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Ordered crystalline compounds exhibiting ultralow and glass-like thermal conductivity are both fundamentally and technologically important, where phonon quasi-particles dominate their heat transport. Understanding the microscopic mechanisms…

Materials Science · Physics 2025-09-04 Shantanu Semwal , Yi Xia , Chris Wolverton , Koushik Pal

The occurrence of thermal transport phenomena is widespread, exerting a pivotal influence on the functionality of diverse electronic and thermo-electric energy-conversion devices. The traditional first-principles theory governing the…

Materials Science · Physics 2026-05-20 Soham Mandal , Manish Jain , Prabal K. Maiti

We extended and corrected Mott's two-band model for the composition-dependence of thermal and electrical conductivity in binary metal alloys based on high-throughput time-domain thermoreflectance (TDTR) measurements on diffusion multiples…

Materials Science · Physics 2016-10-04 Changdong Wei , Nikolas Antolin , Oscar D. Restrepo , Wolfgang Windl , Ji-Cheng Zhao

Semiconductor alloys exhibit a strong dependence of effective thermal conductivity on measurement frequency. So far this quasi-ballistic behaviour has only been interpreted phenomenologically, providing limited insight into the underlying…

Materials Science · Physics 2015-02-13 Bjorn Vermeersch , Jesus Carrete , Natalio Mingo , Ali Shakouri

Structural defects in one-dimensional heat conductors couple longitudinal (stretching) and transverse (bending) vibrations. This coupling results in the scattering of longitudinal phonons to transverse phonons and backwards. We show that…

Chemical Physics · Physics 2025-05-27 Alexander L. Burin

We present a first-principles study of the cross-plane thermal conductivity $\kappa_{\perp}$ in a wide variety of semiconductor thin films. We introduce a simple suppression model that matches variance-reduced Monte Carlo simulations with…

Mesoscale and Nanoscale Physics · Physics 2016-05-11 Bjorn Vermeersch , Jesus Carrete , Natalio Mingo

Semiconductors with very low lattice thermal conductivities are highly desired for applications relevant to thermal energy conversion and management, such as thermoelectrics and thermal barrier coatings. Although the crystal structure and…

Materials Science · Physics 2021-07-13 Jiangang He , Yi Xia , Wenwen Lin , Koushik Pal , Yizhou Zhu , Mercouri G. Kanatzidis , Chris Wolverton

We conduct comprehensive investigations of both thermal and electrical transport properties of SnSe and SnS using first-principles calculations combined with the Boltzmann transport theory. Due to the distinct layered lattice structure,…

Materials Science · Physics 2015-10-14 Ruiqiang Guo , Xinjiang Wang , Youdi Kuang , Baoling Huang

We investigate the evolution of the cross-plane thermal conductivity $\kappa$ of superlattices (SLs) as interfaces change from perfectly abrupt to totally intermixed, by using non-equilibrium molecular dynamics simulations in combination…

Materials Science · Physics 2019-08-19 Xiaolong Yang , Wu Li

A density functional theory based two-terminal scattering formalism that includes spin-orbit coupling and spin non-collinearity is described. An implementation using tight-binding muffin-tin orbitals combined with extensive use of sparse…

Mesoscale and Nanoscale Physics · Physics 2018-06-15 Anton A. Starikov , Yi Liu , Zhe Yuan , Paul J. Kelly

High-entropy alloys are characterized by high configurational entropy. Since the discovery of high-entropy alloys (HEA) in 2004, entropy engineering has provided a promising direction for exploiting composition, lattice disorder, band…

Materials Science · Physics 2019-11-12 S. Joseph Poon , Jian He

We investigate the semiclassical electronic transport properties of the bilayer silicene-like system in the presence of charged impurity. The trigonal warping due to the interlayer hopping, and its effect to the band structure of bilayer…

Mesoscale and Nanoscale Physics · Physics 2018-09-18 Chen-Huan Wu

Recent theoretical and experimental research suggests that $\theta$-TaN is a semimetal with high thermal conductivity ($\kappa$), primarily due to the contribution of phonons ($\kappa_\texttt{ph}$). By using first-principles calculations,…

Materials Science · Physics 2024-03-20 Ashis Kundu , Yani Chen , Xiaolong Yang , Fanchen Meng , Jesús Carrete , Mukul Kabir , Georg K. H. Madsen , Wu Li

Recently, $\mathrm{BaSn_2}$ is predicted to be a strong topological insulator by the first-principle calculations. It is well known that topological insulator has a close connection to thermoelectric material, such as $\mathrm{Bi_2Te_3}$…

Materials Science · Physics 2016-12-21 San-Dong Guo , Liang Qiu

Phonon surface scattering has been at the core of heat transport engineering in nanoscale structures and devices. Herein, we demonstrate that this phonon pathway can be the sole mechanism only below a characteristic, size-dependent…

Phonon size effects induce ballistic transport in nanomaterials, challenging Fourier's law. Nondiffusive heat transport is captured by the Peierls-Boltzmann transport equation (BTE), commonly solved under the relaxation time approximation…

Mesoscale and Nanoscale Physics · Physics 2020-03-10 Giuseppe Romano

Two-dimensional (2-D) transition metal dichalcogenides (TMDs) have shown numerous interesting physical and chemical properties, making them promising materials for electronic, optoelectronic, and energy applications. Tuning thermal…

Materials Science · Physics 2016-09-07 Xiaokun Gu , Ronggui Yang

We combine first-principles calculations and Boltzmann transport theory to study the electrical transport properties of intermetallic compound YbAl3. To accurately predict the electronic relaxation time, we use the density functional…

Mesoscale and Nanoscale Physics · Physics 2016-09-20 Jinghua Liang , Dengdong Fan , Peiheng Jiang , Huijun Liu , Wenyu Zhao

Numerical calculations of lattice thermal conductivity are reported for the binary alloys NiPd and NiPt. The present work is a continuation of an earlier paper by us [PRB, 72, 214207 (2005)]which had developed a theoretical framework for…

Materials Science · Physics 2013-12-25 Aftab Alam , Abhijit Mookerjee

We study a theoretical model for the magnetothermal conductivity of a spin-1/2 ladder with low exchange coupling ($J\ll\Theta_D$) subject to a strong magnetic field $B$. Our theory for the thermal transport accounts for the contribution of…

Strongly Correlated Electrons · Physics 2015-06-05 Ofer Shlagman , Efrat Shimshoni