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Optical activity is ubiquitous across natural and artificial media and is conventionally understood in terms of scattering from electric and magnetic moments. Here we demonstrate experimentally and confirm numerically a type of optical…

Toroidal multipoles are the terms missing in the standard multipole expansion; they are usually overlooked due to their relatively weak coupling to the electromagnetic fields. Here we propose and theoretically study all-dielectric…

Toroidal dipole, first described by Ia. B. Zeldovich [Sov. Phys. JETP 33, 1184 (1957)], is a distinct electromagnetic excitation that differs both from the electric and the magnetic dipoles. It has a number of intriguing properties: static…

Optics · Physics 2013-10-02 V. Savinov , V. A. Fedotov , N. I. Zheludev

We demonstrate that the toroidal dipolar response can be realized in the optical regime by designing a feasible nanostructured metamaterial, comprising asymmetric double-bar magnetic resonators assembled into a toroid-like configuration. It…

Optics · Physics 2015-03-13 Zheng-Gao Dong , J. Zhu , Junsuk Rho , Jia-Qi Li , Changgui Lu , Xiaobo Yin , X. Zhang

In this short article, we overview a concept of electronic toroidal multipoles, and their ordering with associated physical properties in non-magnetic and magnetic materials. The toroidal multipoles are introduced as microscopic electronic…

Materials Science · Physics 2024-09-12 Hiroaki Kusunose , Satoru Hayami

Natural optical activity is the paradigmatic example of an effect originating in the weak spatial inhomogeneity of the electromagnetic field on the atomic scale. In molecules, such effects are well described by the multipole theory of…

Materials Science · Physics 2023-05-31 Óscar Pozo , Ivo Souza

In the frame of the algebraic Riemann Rotational Model one computes the longitudinal, transverse and toroidal multipoles corresponding to the excitations of low-lying levels in the ground state band of several even-even nuclei by inelastic…

Nuclear Theory · Physics 2009-10-28 S. Misicu

We present a general formalism of multipole descriptions under the space-time inversion group. We elucidate that two types of atomic toroidal multipoles, i.e., electric and magnetic, are fundamental pieces to express electronic order…

Strongly Correlated Electrons · Physics 2018-02-26 Satoru Hayami , Hiroaki Kusunose

We present a theory describing interaction of structured light, such as light carrying orbital angular momentum, with molecules. The light-matter interaction Hamiltonian we derive is expressed through couplings between spherical gradients…

The electromagnetic response of matter is governed by three fundamental multipole families: electric, magnetic, and toroidal. While the electric and magnetic are cornerstones of physics, the toroidal dipole (TD) has eluded direct,…

Quantum Physics · Physics 2025-11-04 Alexandru-Lucian Nastasia , Mircea Dolineanu , Dragos-Victor Anghel

It is shown that a new type of metamaterial, a 3D-array of toroidal solenoids, displays a significant toroidal response that can be readily measured. This is in sharp contrast to materials that exist in nature, where the toroidal component…

Classical Physics · Physics 2007-09-25 K. Marinov , A. D. Boardman , V. A. Fedotov , N. Zheludev

Maxwell's equations in curved space-time are invariant under electromagnetic duality transformations. We exploit this property to constraint the design parameters of metamaterials used for transformations optics. We show that a general…

Optics · Physics 2013-10-21 Ivan Fernandez-Corbaton , Gabriel Molina-Terriza

Living in a world of resonances, there have been significant progresses in the field of excitation high-quality and multifunctional moments across a wide range of optical frequencies. Among all acknowledged resonances, the toroidal…

Optics · Physics 2018-10-17 Burak Gerislioglu , Arash Ahmadivand

The interaction between light and matter is fundamental to developments in quantum optics and information. Over recent years enormous progress has been made in controlling the interface between light and single emitters including ions,…

Multipoles are paramount for describing electromagnetic fields in many areas of nanoscale optics, playing an essential role for the design of devices in plasmonics and all-dielectric nanophotonics. Challenging the traditional division into…

Photons carrying a well-defined orbital angular momentum have been proven to modify spectroscopic selection rules in atomic matter. Excitation profiles of electric quadrupole transitions have been measured with single trapped $^{40}$Ca$^+$…

Molecular hydrogen ions are of metrological relevance due to the possibility of precise theoretical evaluation of their spectrum and of external-field-induced shifts. In homonuclear molecular ions the electric dipole $E1$ transitions are…

Atomic Physics · Physics 2021-01-20 P. Danev , D. Bakalov , V. I. Korobov , S. Schiller

Molecular absorption of infrared radiation is generally due to ro-vibrational electric-dipole transitions. Electric-quadrupole transitions may still occur, but they are typically a million times weaker than electric-dipole transitions,…

In the last decade, much theoretical research has focused on studying the strong coupling between organic molecules (or quantum emitters, in general) and light modes. The description and prediction of polaritonic phenomena emerging in this…

Spatially-structured laser beams, eventually carrying orbital angular momentum, affect electronic transitions of atoms and their motional states in a complex way. We present a general framework, based on the spherical tensor decomposition…

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