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All solid state Li-ion batteries employing metallic lithium as an anode offer higher energy densities while also being safer than conventional liquid electrolyte based Li-ion batteries. However, the growth of tiny filaments of lithium…

Applied Physics · Physics 2020-01-20 Vikalp Raj , Varun R Kankanallu , Bibhatsu Kuiri , Naga Phani B Aetukuri

Rechargeable lithium metal batteries have been widely investigated recently, driven by the global trend for the electrification of transportation. Understanding the dynamics of lithium metal electrodeposition is crucial to design safe and…

Materials Science · Physics 2022-07-15 Shoutong Jin , Linming Zhou , Yongjun Wu , Shang Zhu , Qilong Zhang , Hui Yang , Yuhui Huang , Zijian Hong

Next-generation lithium-ion batteries with silicon anodes have positive characteristics due to higher energy densities compared to state-of-the-art graphite anodes. However, the large volume expansion of silicon anodes can cause high…

Numerical Analysis · Mathematics 2024-04-03 R. Schoof , G. F. Castelli , W. Dörfler

Battery interfaces critically influence lithium-metal battery performance through their role in ion diffusion and dendrite formation. However, structural characterization of these interfaces has remained challenging due to limitations in…

Materials Science · Physics 2025-05-08 Hyeongjun Koh , Eric Detsi , Eric A. Stach

Next generation batteries based on lithium (Li) metal anodes have been plagued by the dendritic electrodeposition of Li metal on the anode during cycling, resulting in short circuit and capacity loss. Suppression of dendritic growth through…

Recently some critical problems and challenges have been exposed, hindering the development and practical application of SSLBs, such as the low room temperature ionic conductivity of solid electrolyte, the risk of short circuit caused by…

Materials Science · Physics 2023-08-01 L. J. Zhang

Li metal is an ideal anode material for use in state-of-the-art secondary batteries. However, Li-dendrite growth is a safety concern and results in low coulombic efficiency, which significantly restricts the commercial application of Li…

Whereas in typical standardized tests batteries are almost exclusively loaded with constant current or relatively slowly changing cycles, real applications involve rapid load ripple, which do not contribute to the net energy. The trend to…

Systems and Control · Electrical Eng. & Systems 2022-09-20 Tomas Kacetl , Jan Kacetl , Nima Tashakor , Stefan Goetz

We report the lithium plating associated capacity loss during fast charging of compressively loaded lithium-ion batteries (LIBs). The charging and discharging of LIB under compressive loading during service may affect the cell performance…

Materials Science · Physics 2024-02-23 Prashant P. Gargh , Abhishek Sarkar , Ikenna C. Nlebedim , Pranav Shrotriya

Rechargeable lithium, sodium, and aluminum metal-based batteries are among the most versatile platform for high-energy, cost effective electrochemical energy storage. Non-uniform metal deposition and dendrite formation on the negative…

Materials Science · Physics 2015-01-27 Yingying Lu , Zhengyuan Tu , Lynden Archer

Lithium metal batteries are promising for next-generation high-energy-density batteries, especially when lithium is directly plated on a current collector. However, lithium whiskers can form in the early stages of electroplating. These…

Chemical Physics · Physics 2025-03-28 Martin Werres , Dariusz Niedziela , Arnulf Latz , Birger Horstmann

The path toward Li-ion batteries with higher energy-densities will likely involve use of thin lithium metal (Li) anode (<50 $\mu$m in thickness), whose cyclability today remains limited by dendrite formation and low Coulombic efficiency.…

Rechargeable lithium metal batteries (LMBs) with an ultrahigh theoretical energy density have attracted more and more attentions for their crucial applications of portable electronic devices, electric vehicles, and smart grids. However, the…

Materials Science · Physics 2024-10-22 Yanchen Fana , Xiang Chenb , Dominik Legut , Qianfan Zhang

An important objective of designing lithium-ion rechargeable battery cells is to maximize their rate performance without compromising the energy density, which is mainly achieved through computationally expensive numerical simulations at…

Materials Science · Physics 2020-05-05 Fan Wang , Ming Tang

Interfacial deposition stability between Li metal and a solid electrolyte (SE) is important in preventing interfacial contact loss, mechanical fracture, and dendrite growth in Li-metal solid-state batteries (SSB). In this work, we…

Applied Physics · Physics 2020-06-08 Qingsong Tu , Luis Barroso-Luque , Tan Shi , Gerbrand Ceder

The development of sustainable transportation and communication systems requires an increase in both energy density and capacity retention of Li-batteries. Using substrates forming a solid solution with body centered cubic Li enhances the…

Mechanical degradation in electrode materials during successive electrochemical cycling is critical for battery lifetime and aging properties. A common strategy to mitigate electrode mechanical degradation is to suppress the volume…

Materials Science · Physics 2024-06-10 Maxime Maréchal , Romain Berthelot , Patrick Rozier , Matthieu Saubanère

We study numerically localised short circuits in Li||Bi liquid metal batteries. In the prototype of a classical, three liquid-layer system, we assume a perceptible local deformation of the Li-salt interface. We find that there always exists…

Fluid Dynamics · Physics 2021-08-27 Sabrina Bénard , Norbert Weber , Gerrit Maik Horstmann , Steffen Landgraf , Tom Weier

It is widely believed that the origin of a significant cause for the voltage and capacity fading observed in lithium (Li)-ion batteries is related to structural modifications occurring in the cathode material during the Li-ion…

Lithium metal batteries (LMB) are vital devices for high-energy-density energy storage, but Li metal anode is highly reactive with electrolyte and forms uncontrolled dendrite that can cause undesirable parasitic reactions thus poor cycling…