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Dielectric metasurfaces provide a unique platform for efficient harmonic generation and optical wavefront manipulation at the nanoscale. While several approaches are available for performing wavefront shaping, the one exploiting geometric…

We propose an extensive discussion on the homogenization and scattering analysis of second-order nonlinear metasurfaces. Our developments are based on the generalized sheet transition conditions (GSTCs) which are used to model the…

Recent experiments and calculations in topological semimetals have observed anomalously strong second-order optical nonlinearity, but yet whether the enhancement also occurs at surfaces of topological semimetals in general remains an open…

Mid-infrared nanophotonics can be realized using sub-diffractional light localization and field enhancement with surface phonon polaritons in polar dielectric materials. We experimentally demonstrate second harmonic generation due to the…

We study second-harmonic generation (SHG) arising from surface nonlinearity at a metal-dielectric interface using a spectral decomposition method. Since our method avoids the need to consider the generalized boundary condition across the…

Here we employ the quasi-bound state in the continuum (quasi-BIC) resonance in all-dielectric metasurfaces for efficient nonlinear processes in consideration of the backward frequency conversion. We theoretically study the second-harmonic…

Optics · Physics 2024-06-28 Xu Tu , Siqi Feng , Jiajun Li , Yangguang Xing , Feng Wu , Tingting Liu , Shuyuan Xiao

Generation of even-order optical harmonics requires noncentrosymmetric structures being conventionally observed in crystals lacking the center of inversion. In centrosymmetric systems, even-order harmonics may arise, e.g., at surfaces but…

A systematic approach is presented to exploit the rich field transformation capabilities of Electromagnetic (EM) metasurfaces for creating a variety of illusions using the concept of metasurface holograms. A system level approach to…

Computational Physics · Physics 2020-02-20 Tom. J. Smy , Scott A. Stewart , Shulabh Gupta

The discovery of second harmonic generation in 1961 marked the birth of nonlinear optics, unlocking a range of applications from frequency conversion to quantum light generation. Yet, phase matching in bulk nonlinear crystals remains a key…

We generalize the concept of optical scattering matrix ($S$-matrix) to characterize harmonic generation and frequency mixing in planar metasurfaces in the limit of undepleted pump approximation. We show that the symmetry properties of such…

Optics · Physics 2024-05-03 Kirill Koshelev , Ivan Toftul , Yongsop Hwang , Yuri Kivshar

We theoretically investigate second harmonic generation that originates from the nonlinear, magnetic Lorentz force term from single and multiple apertures carved on thick, opaque metal substrates. The linear transmission properties of…

Efficient frequency conversion techniques are crucial to the development of plasmonic metasurfaces for information processing and signal modulation. In principle, nanoscale electric-field confinement in nonlinear materials enables higher…

Nonlinear light sources are central to a myriad of applications, driving a quest for their miniaturisation down to the nanoscale. In this quest, nonlinear metasurfaces hold a great promise, as they enhance nonlinear effects through their…

We analyze third-harmonic generation from high-index dielectric nanoparticles and discuss the basic features and multipolar nature of the parametrically generated electromagnetic fields near the Mie-type optical resonances. By combining…

Second-harmonic emission at a frequency that is twice the laser frequency is an important diagnostic for nonlinear laser-plasma interaction. It is forbidden for centrosymmetric materials such as the bulk of sapphire. The symmetry, however,…

Resonant metasurfaces have received extensive attention due to their sharp spectral feature and extraordinary field enhancement. In this work, by breaking the in-plane symmetry of silicon nanopillars, we achieve a sharp Fano resonance. The…

Optics · Physics 2020-04-06 Chaobiao Zhou , Shiyu Li , Cheng Gong , Yi Wang , Xiaojun Liu , Mingsheng Zhan

The nonlinear process of second harmonic generation (SHG) in monolayer (1L) transition metal dichalcogenides (TMD), like $WS_2$, strongly depends on the polarization state of the excitation light. Combining plasmonic nanostructures with…

Optics · Physics 2021-10-08 Florian Spreyer , Claudia Ruppert , Philip Georgi , Thomas Zentgraf

Light with light control of surface plasmon polaritons is theoretically demonstrated. A barely simple and compact source of these waves consists in a finite number of slits (evenly spaced) perforating a metal film. The system scatters…

Applied Physics · Physics 2018-08-08 Sergio G. Rodrigo

Second harmonic generation has been applied to study lattice, electronic and magnetic proprieties in atomically thin materials. However, inversion symmetry breaking is usually required for the materials to generate a large signal. In this…

Materials Science · Physics 2022-05-12 Zhuoliang Ni , Nan Huang , Amanda V. Haglund , David G. Mandrus , Liang Wu

By combining analytical and numerical approaches, we study resonantly enhanced second-harmonic generation (SHG) by individual high-index dielectric nanoparticles made of centrosymmetric materials. Considering both bulk and surface…

Optics · Physics 2018-01-08 Daria Smirnova , Alexander I. Smirnov , Yuri S. Kivshar