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Ferromagnetic van der Waals (vdW) insulators are of great scientific interest for their promising applications in spintronics. It has been indicated that in the two materials within this class, CrI$_3$ and VI$_3$, the magnetic ground state,…

Strongly Correlated Electrons · Physics 2020-12-15 Asish K. Kundu , Yu Liu , C. Petrovic , T. Valla

CrI3, which belongs to a rare category of two-dimensional (2D) ferromagnetic semiconductors, is of great interest for spintronic device applications. Unlike CrCl3 whose magnetism presents a 2D-Heisenberg behavior, CrI3 exhibits a larger van…

Materials Science · Physics 2018-03-14 G. T. Lin , X. Luo , F. C. Chen , J. Yan , J. J. Gao , Y. Sun , W. Tong , P. Tong , W. J. Lu , Z. G. Sheng , W. H. Song , X. B. Zhu , Y. P. Sun

CrI3 is a layered ferromagnetic insulator that has recently attracted enormous interest as it was the first example of a stand-alone monolayer ferromagnet, paving the way towards the study of two-dimensional magnetic materials and their use…

Magnetic insulators are a key resource for next-generation spintronic and topological devices. The family of layered metal halides promises ultrathin insulating multiferroics, spin liquids, and ferromagnets, but new characterization methods…

We report on a combined experimental and theoretical study on CrI3 single crystals by employing the polarization dependence of resonant inelastic X-ray scattering (RIXS). Our investigations reveal multiple Cr 3d orbital splitting (dd…

Graphene-based heterostructures are a promising material system for designing the topologically nontrivial Chern insulating devices. Recently, a two-dimensional (2D) monolayer ferromagnetic insulator CrI$_{3}$ was successfully synthesized…

Materials Science · Physics 2018-02-07 Jiayong Zhang , Bao Zhao , Tong Zhou , Yang Xue , Chunlan Ma , Zhongqin Yang

Two-dimensional CrI3 has attracted much attention as it is reported to be a ferromagnetic semiconductor with the Curie temperature around 45K. By performing first-principles calculations, we find that the magnetic ground state of CrI3 is…

Computational Physics · Physics 2019-01-09 Zewen Wu , Jin Yu , Shengjun Yuan

Manipulating physical properties using the spin degree of freedom constitutes a major part of modern condensed matter physics and is very important for spintronics devices. Using the newly discovered two dimensional van der Waals…

Materials Science · Physics 2018-05-29 Peiheng Jiang , Lei Li , Zhaoliang Liao , Y. X. Zhao , Zhicheng Zhong

The development of room-temperature magnetic semiconductors is critical for advancing spintronic technologies, yet van der Waals magnets like CrI3 exhibit intrinsically low Curie temperatures (Tc = 45 K). This study employs first-principles…

Materials Science · Physics 2025-08-12 Qing-Han Yang , Jia-Wen Li , Xin-Wei Yi , Xiang Li , Jing-Yang You , Gang Su , Bo Gu

Using density functional theory combined with a Hubbard model (DFT+U ), the electronic band structure of CrI3 multilayers, both free-standing and enclosed between graphene contacts, is calculated. We show that the DFT+U approach, together…

Materials Science · Physics 2020-10-21 Soumyajit Sarkar , Peter Kratzer

CrI3 is a prototypical van der Waals ferromagnet with a magnetic honeycomb lattice. Previous inelastic neutron scattering studies have suggested topological nature of its magnetic excitations with a magnon gap at the Dirac points, which are…

Materials Science · Physics 2024-03-14 Chunqiang Xu , Heda Zhang , Caitlin Carnahan , Pengpeng Zhang , Di Xiao , Xianglin Ke

Two-dimensional (2D) layered magnetic materials are generating a great amount of interest for the next generation of electronic devices thanks to their remarkable properties associated to spin dynamics. The recently discovered layered…

The recently reported magnetic ordering in insulating two-dimensional (2D) materials, such as chromium triiodide (CrI$_3$) and chromium tribromide (CrBr$_3$), opens new possibilities for the fabrication of magneto-electronic devices based…

We report structural, physical properties and electronic structure of van der Waals (vdW) crystal VI3. Detailed analysis reveals that VI3 exhibits a structural transition from monoclinic C2/m to rhombohedral R-3 at Ts ~ 79 K, similar to…

Materials Science · Physics 2019-06-19 Shangjie Tian , Jian-Feng Zhang , Chenghe Li , Tianping Ying , Shiyan Li , Xiao Zhang , Kai Liu , Hechang Lei

The integration of diverse electronic phenomena, such as magnetism and nontrivial topology, into a single system is normally studied either by seeking materials that contain both ingredients, or by layered growth of contrasting materials.…

Low dimensional magnetism has been powerfully boosted as a promising candidate for numerous applications. The stability of the long-range magnetic order is directly dependent on the electronic structure and the relative strength of the…

Materials Science · Physics 2020-04-27 Adolfo O. Fumega , S. Blanco-Canosa , H. Babu-Vasili , Jian-Shi Zhou , F. Rivadulla , Victor Pardo

We present comprehensive measurements of the structural, magnetic and electronic properties of layered van-der-Waals ferromagnet VI$_3$ down to low temperatures. Despite belonging to a well studied family of transition metal trihalides,…

Recently intrinsic ferromagnetism in two-dimensional(2D) van der Waals materials was discovered [1, 2, 3]. A monolayer of Chromiun triiodide(CrI3) is ferromagnetic while a bilayer structure was reported to be anti-ferro magnetic, moreover…

Materials Science · Physics 2018-11-30 E. Suarez Morell , Andrea León , R. Hiroki Miwa , P. Vargas

Two-dimensional (2D) ferromagnets with high Curie temperature have long been the pursuit for electronic and spintronic applications. CrI3 is a rising star of intrinsic 2D ferromagnets, however, it suffers from weak exchange coupling. Here…

Materials Science · Physics 2020-09-22 Yu Guo , Nanshu Liu , Yanyan Zhao , Xue Jiang , Si Zhou , Jijun Zhao

Recent years have seen a vast increase in research into van der Waals magnetic materials. In many of these systems, magnetism is introduced via light 3\textit{d}-transition metal elements, combined with chalcogenides or halogens. Despite…

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