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Pyrene-functional PMMAs were prepared via ATRP-controlled polymerization and click reaction, as efficient dispersing agents for the exfoliation of few-layered graphene sheets (GS) in easily processable low boiling point chloroform. In…

Polycyclic Aromatic Hydrocarbons (PAHs) are organic molecules which comprise the smallest particles of dust in the interstellar medium (ISM). Due to their broad/complex emission profiles, obtaining kinematics is a challenge with traditional…

Astrophysics of Galaxies · Physics 2024-05-24 Fergus R. Donnan , Dimitra Rigopoulou , Ismael García-Bernete

Studying the anharmonicity in the infrared (IR) spectra of polycyclic aromatic hydrocarbons (PAHs) at elevated temperatures is important to understand vibrational features and chemical properties of interstellar dust, especially in the…

The high interstellar abundances of polycyclic aromatic hydrocarbons (PAHs) and their size distribution are the result of complex chemical processes implying dust, UV radiation, and the main gaseous components (H, C+, and O). These…

Astrophysics of Galaxies · Physics 2021-07-07 A. Omont , H. F. Bettinger

This joint theoretical and experimental study establishes that the adsorption of polycyclic aromatic hydrocarbons (PAHs) onto the amorphous ice surface provokes a broadening and redshift of the "dangling" OH (dOH) ice spectral feature, the…

Chemical Physics · Physics 2020-03-05 E Michoulier , C Toubin , A Simon , J Mascetti , C Aupetit , J A Noble

Polycyclic aromatic hydrocarbon (PAH) molecules, ubiquitously seen in the interstellar medium (ISM) of our own and external galaxies, might have been incorporated into comets if they are formed from relatively unprocessed interstellar…

Astrophysics · Physics 2009-11-13 Aigen Li

Polycyclic Aromatic Hydrocarbons are prevalent in the universe and interstellar medium but are primarily attributed to anthropogenic sources on Earth, such as fossil fuel combustion and firewood burning. Drawing upon the idea of PAHs as…

Earth and Planetary Astrophysics · Physics 2025-01-14 Dwaipayan Dubey , Ravi Kopparapu , Barbara Ercolano , Karan Molaverdikhani

We demonstrate a novel in situ polymerization technique to develop localized polymer coatings on the surface of dispersed pristine graphene sheets. Graphene sheets show great promise as strong, conductive fillers in polymer nanocomposites;…

Soft Condensed Matter · Physics 2011-04-29 Sriya Das , Ahmed S. Wajid , John L. Shelburne , Yen-Chi Liao , Micah J. Green

The use of a novel three-dimensional graphene structure allows circumventing the limitations of the two-dimensional nature of graphene and its application in hydrogen absorption. Here we investigate hydrogen-bonding on monolayer graphene…

Recurrent fluorescence (RF) is an important relaxation mechanism in polycyclic aromatic hydrocarbons (PAHs), which could stabilize them and contribute to the production of aromatic infrared bands that are observed in the infrared spectra of…

Chemical Physics · Physics 2026-04-01 Damien Borja , Florent Calvo , Pascal Parneix , Cyril Falvo

We investigate the microscopic processes leading to graphene growth by the chemical vapor deposition of propane in the argon atmosphere at the SiC surface. Experimentally, it is known that the presence of argon fastens the dehydrogenation…

Materials Science · Physics 2017-09-13 Malgorzata Wierzbowska , Adam Dominiak , Kamil Tokar

We design and train a neural network (NN) model to efficiently predict the infrared spectra of interstellar polycyclic aromatic hydrocarbons (PAHs) with a computational cost many orders of magnitude lower than what a first-principles…

Astrophysics of Galaxies · Physics 2020-10-20 Peter Kovacs , Xiaosi Zhu , Jesus Carrete , Georg K. H. Madsen , Zhao Wang

The growth of controlled 1D carbon-based nanostructures on metal surfaces is a multistep process whose path, activation energies and intermediate metastable states strongly depend on the employed substrate. Whereas this process has been…

Man-made artificial graphene has attracted significant attention in the past few years due to the possibilities to construct designer Dirac fermions with unexpected topological properties and applications in nanoelectronics. Here we use a…

Materials Science · Physics 2014-12-10 Matti Ropo , Sami Paavilainen , Jaakko Akola , Esa Räsänen

The infrared signatures of polycyclic aromatic hydrocarbons (PAHs) are observed in a variety of astrophysical objects, including the circumnuclear medium of active galactic nuclei (AGNs). These are sources of highly energetic photons (0.2…

The infrared signature of polycyclic aromatic hydrocarbons (PAHs) are present in many protostellar disks and these speciesare thought to play an important role in heating of the gas in the photosphere. We aim to consider PAH cluster…

Earth and Planetary Astrophysics · Physics 2021-09-01 K. Lange , C. Dominik , A. G. G. M. Tielens

Energetic and geometric aspects of the permeation of low-Z atoms through graphene sheets are investigated. Energy barriers and deformations are calculated via density functional theory for the permeation of H, He, Li and Be atoms at several…

Chemical Physics · Physics 2012-10-02 Stefan E. Huber , Andreas Mauracher , Michael Probst

In this work, we study the photodissociation processes of small PAH clusters (e.g., pyrene clusters). The experiments are carried out using a quadrupole ion trap in combination with time-of-flight (QIT-TOF) mass spectrometry. The results…

Instrumentation and Methods for Astrophysics · Physics 2018-09-27 Junfeng Zhen , Tao Chen , Alexander G. G. M. Tielens

The growth of graphene on copper by atmospheric pressure chemical vapor deposition in a system free of pumping equipment is investigated. The emphasis is put on the necessity of hydrogen presence during graphene synthesis and cooling. In…

In order to find out capable molecular source of astronomically well observed infrared (IR) spectrum, asymmetric molecular configuration polycyclic aromatic hydrocarbon (PAH) was analyzed by the density functional theory (DFT) analysis.…

Astrophysics of Galaxies · Physics 2015-10-27 Norio Ota