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Ultrastable vapor-deposited glasses display uncommon material properties. Most remarkably, upon heating they are believed to melt via a liquid front that originates at the free surface and propagates over a mesoscopic crossover length,…

Soft Condensed Matter · Physics 2019-10-24 Elijah Flenner , Ludovic Berthier , Patrick Charbonneau , Christopher J. Fullerton

The influence of strain amplitude, glass stability and thermal fluctuations on shear band formation and yielding transition is studied using molecular dynamics simulations. The model binary mixture is first gradually cooled below the glass…

Soft Condensed Matter · Physics 2020-08-03 Nikolai V. Priezjev

The interplay between the structural relaxation and the rheological response of a binary LJ glass former is studied via MD simulations. In the quiescent state, the model is well known for its sluggish dynamics and a two step relaxation of…

Soft Condensed Matter · Physics 2015-05-14 Fathollah Varnik

We perform molecular dynamics simulations of an idealized polymer melt surrounding a nanoscopic filler particle to probe the effects of a filler on the local melt structure and dynamics. We show that the glass transition temperature $T_g$…

Soft Condensed Matter · Physics 2009-10-31 Francis W. Starr , Thomas B. Schrøder , Sharon C. Glotzer

The process of ageing in rubbers requires monitoring over long periods (days to years). To do so in non-conducting rubbers, small amounts of carbon-black particles were dispersed in a fractal network through the rubber matrix, to make the…

Materials Science · Physics 2009-11-10 H. B. Brom , I. G. Romijn , J. G. Magis , M. van der Vleuten , M. A. J. Michels

We represent a theory of polymer gelation as an analogue of liquid-glass transition in which elastic fields of stress and strain shear components appear spontaneously as a consequence of the cross-linking of macromolecules. This…

Statistical Mechanics · Physics 2015-06-24 Alexander I. Olemskoi , Ivan Krakovsky

We consider the stationary state of a fluid comprised of inelastic hard spheres or disks under the influence of a random, momentum-conserving external force. Starting from the microscopic description of the dynamics, we derive a nonlinear…

Statistical Mechanics · Physics 2013-02-25 W. T. Kranz , M. Sperl , A. Zippelius

A model is derived for the viscoelastic response of glasses at isothermal uniaxial deformation with small strains. A glass is treated as an ensemble of relaxing units with various activation energies for rearrangement. With reference to the…

Materials Science · Physics 2007-05-23 A. D. Drozdov , J. deC. Christiansen

Supercooled liquids undergo a rapid change in dynamics as they are cooled to their glass transition temperature and turn from a flowing liquid into an amorphous solid. Depending on how steeply the viscosity changes with temperature around…

In large area micro hot embossing, the process temperature plays a critical role to both the local fidelity of microstructure formation and global uniformity. The significance of low temperature hot embossing is to improve global flatness…

Other Computer Science · Computer Science 2008-02-22 X. C. Shan , Y. C. Liu , H. J. Lu , Z. F. Wang , Y. C. Lam

We propose that an onset of glass transition can be defined as the point at which a supercooled liquid acquires the stress relaxation mechanism of a solid glass. We translate this condition into the rate equation for local relaxation…

Materials Science · Physics 2009-11-11 Kostya Trachenko

Quantitative understanding of the fracture toughness of metallic glasses, including the associated ductile-to-brittle transitions, is not yet available. Here we use a simple model of plastic deformation in glasses, coupled to an advanced…

Materials Science · Physics 2012-11-12 Chris H. Rycroft , Eran Bouchbinder

Randomly disordered (polydomain) liquid crystalline elastomers align under stress. We study the dynamics of stress relaxation before, during and after the Polydomain-Monodomain transition. The results for different materials show the…

Soft Condensed Matter · Physics 2016-08-31 S. M. Clarke , E. M. Terentjev

The glass transition temperature and its connection to statistical properties of confined and free-standing polymer films of varying thickness containing unentangled to highly entangled bead-spring chains are studied by molecular dynamics…

Soft Condensed Matter · Physics 2023-09-21 Hsiao-Ping Hsu , Kurt Kremer

We study the stress response to a step strain of covalently bonded gelatin gels in the temperature range where triple helix reversible crosslink formation is prohibited. We observe slow stress relaxation towards a $T$-dependent finite…

Soft Condensed Matter · Physics 2016-03-23 O. Ronsin , C. Caroli , T Baumberger

Glass-like materials are nonequilibrium systems where the relaxation time may exceed reasonable time scales of observations. In the present paper a dynamic percolation model is introduced in order to explain the principal properties of…

Condensed Matter · Physics 2007-05-23 A. Vazquez , O. Sotolongo-Costa

Metallic glasses deform elastically under stress. However, the atomic-level origin of elastic properties of metallic glasses remain unclear. In this paper using {\em ab initio} molecular dynamics simulations of the Cu$_{50}$Zr$_{50}$…

Materials Science · Physics 2020-03-10 I. Lobzenko , Y. Shiihara , T. Iwashita

In soft amorphous materials, shear cessation after large shear deformation leads to structures having residual shear stress. The origin of these states and the distribution of the local shear stresses within the material is not well…

Soft Condensed Matter · Physics 2021-08-31 Vishwas V. Vasisht , Pinaki Chaudhuri , Kirsten Martens

By systematically investigating the relaxation behavior of a model metallic glass based on the extensive molecular dynamics (MD) simulations combined with the dynamic mechanical spectroscopy method, a pronounced ultra-low temperature peak…

Materials Science · Physics 2020-02-25 B. Wang , L. J. Wang , B. S. Shang , X. Q. Gao , Y. Yang , H. Y. Bai , M. X. Pan , W. H. Wang , P. F. Guan

Experimentally resolving atomic-scale structural changes of a deformed glass remains challenging owing to the disordered nature of glass structure. Here, we show that the structural anisotropy emerges as a general hallmark for different…

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