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Related papers: Exploring canyons in glassy energy landscapes usin…

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We introduce simple models, inspired by previous models for froths and covalent glasses, with trivial equilibrium properties but dynamical behaviour characteristic of strong glass forming systems. These models are also a generalization of…

Statistical Mechanics · Physics 2009-11-07 Arnaud Buhot , Juan P. Garrahan , David Sherrington

The aging dynamics of a simple model glass is numerically investigated observing how it takes place in the potential energy landscape $V$. Partitioning the landscape in basins of minima of $|\nabla V|^2$, we are able to elucidate some…

Soft Condensed Matter · Physics 2017-08-23 R. Di Leonardo , L. Angelani , G. Parisi , G. Ruocco , A. Scala , F. Sciortino

Based on a recently introduced metric for measuring distances between configurations, we in- troduce distance-energy (DE) plots to characterize the potential energy surface (PES) of clusters. Producing such plots is computationally feasible…

Atomic and Molecular Clusters · Physics 2013-11-19 Sandip De , Bastian Schaefer , Ali Sadeghi , Michael Sicher , D. G. Kanhere , Stefan Goedecker

An equilibrated model glass-forming liquid is studied by mapping successive configurations produced by molecular dynamics simulation onto a time series of inherent structures (local minima in the potential energy). Using this ``inherent…

Soft Condensed Matter · Physics 2012-03-27 Thomas B. Schroeder , Srikanth Sastry , Jeppe C. Dyre , Sharon C. Glotzer

We focus on the energy landscape of a simple mean-field model of glasses and analyze activated barrier-crossing by combining the Kac-Rice method for high-dimensional Gaussian landscapes with dynamical field theory. In particular, we…

Disordered Systems and Neural Networks · Physics 2021-01-06 V. Ros , G. Biroli , C. Cammarota

The `lid' algorithm performs an exhaustive exploration of neighborhoods of local energy minima of energy landscapes. This paper describes an implementation of the algorithm, including issues of parallel performance and scalability. To…

Computational Physics · Physics 2009-10-31 Paolo Sibani , Ruud van der Pas , J. Christian Schoen

We introduce multistate metadynamics for automatic exploration of conical intersection seams between adiabatic Born-Oppenheimer potential energy surfaces in molecular systems. By choosing the energy gap between the electronic states as a…

Chemical Physics · Physics 2018-05-10 Joachim O. Lindner , Merle I. S. Röhr , Roland Mitrić

Enhanced sampling techniques have become an essential tool in computational chemistry and physics, where they are applied to sample activated processes that occur on a time scale that is inaccessible to conventional simulations. Despite…

Chemical Physics · Physics 2022-01-13 F. Giberti , G. A. Tribello , M. Ceriotti

We present a three-dimensional lattice-gas model with trivial thermodynamics, but nontrivial dynamics. The model is characterized by each particle having its own random energy landscape. The equilibrium dynamics of the model were…

Soft Condensed Matter · Physics 2012-03-27 Ulf R. Pedersen , Tina Hecksher , Jeppe C. Dyre , Thomas B. Schrøder

We report Molecular Dynamics simulations for a new model of tetrahedral network glass-former, based on short-range, spherical potentials. Despite the simplicity of the forcefield employed, our model reproduces some essential physical…

Statistical Mechanics · Physics 2016-09-08 D. Coslovich , G. Pastore

We present molecular dynamics simulations of a model glass-forming liquid (the binary Kob-Anderson Lennard-Jones model) and consider the distributions of inherent energies and metabasins during aging. In addition to the typical protocol of…

Disordered Systems and Neural Networks · Physics 2016-08-14 Christian Rehwald , Nicoletta Gnan , Andreas Heuer , Thomas Schrøder , Jeppe C. Dyre , Gregor Diezemann

While diffusion in crystalline solids is quantitatively understood through defect-mediated atomic hops, no comparable quantitative framework exists for glasses. In these systems, the origin of large diffusion activation energies remains…

Materials Science · Physics 2026-03-20 Ajay Annamareddy , Bu Wang , Paul M. Voyles , Izabela Szlufarska , Dane Morgan

We study the relation of the potential energy landscape (PEL) topography to relaxation dynamics of a small model glass former of Lennard-Jones type. The mechanism under investigation is the hopping betweem superstructures of PEL mimima,…

Disordered Systems and Neural Networks · Physics 2009-11-07 Burkhard Doliwa , Andreas Heuer

We analyse the relationship between dynamics and configuration space structure of Ising spin glass systems. The exact knowledge of the structure of the low--energy landscape is used to study the relaxation of the system by random walk in…

Disordered Systems and Neural Networks · Physics 2009-11-07 S. Kobe , J. Krawczyk

We numerically investigate the aging dynamics of a monatomic Lennard-Jones glass, focusing on the topology of the potential energy landscape which, to this aim, has been partitioned in basins of attraction of stationary points (saddles and…

Disordered Systems and Neural Networks · Physics 2009-10-31 L. Angelani , R. Di Leonardo , G. Parisi , G. Ruocco

An analytical model of non-Gaussian energy landscape of low-temperature fluids is developed based on the thermodynamics of the fluid of dipolar hard spheres. The entire excitation profile of the liquid, from the high temperatures to the…

Soft Condensed Matter · Physics 2009-11-13 Dmitry V. Matyushov

We present the study of the landscape structure of athermal soft spheres both as a function of the packing fraction and of the energy. We find that, on approaching the jamming transition, the number of different configurations available to…

Statistical Mechanics · Physics 2020-05-20 Claudia Artiaco , Paolo Baldan , Giorgio Parisi

Given discrete degrees of freedom (spins) on a graph interacting via an energy function, what can be said about the energy local minima and associated inherent structures? Using the lid algorithm in the context of a spin glass energy…

Disordered Systems and Neural Networks · Physics 2009-11-11 Z. Burda , A. Krzywicki , O. C. Martin , Z. Tabor

We present results from molecular dynamics simulations exploring the supercooled dynamics of the Gaussian Core Model in the low- and intermediate-density regimes. In particular, we discuss the transition from the low-density…

Soft Condensed Matter · Physics 2024-03-18 Vittoria Sposini , Christos N. Likos , Manuel Camargo

We propose a way to analyze the landscape geometry explored by a glassy system after a quench solely based on time series of energy values recorded during a simulation. Entry and exit times for landscape `valleys' are defined operationally…

Statistical Mechanics · Physics 2007-05-23 Paolo Sibani , Jesper Dall