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We propose a scheme for retrieving the ultrafast valley polarization (VP) dynamics in two-dimensional hexagonal materials via attosecond circular dichroism (CD) transient absorption spectroscopy. This approach builds on the CD transition…

Local energy extrema of the bands in momentum space, or valleys, can endow electrons in solids with pseudo-spin in addition to real spin. In transition metal dichalcogenides this valley pseudo-spin, like real spin, is associated with a…

Mesoscale and Nanoscale Physics · Physics 2015-06-22 Grant Aivazian , Zhirui Gong , Aaron M Jones , Rui-Lin Chu , Jiaqiang Yan , David G Mandrus , Chuanwei Zhang , David Cobden , Wang Yao , Xiaodong Xu

Coherent control and manipulation of quantum degrees of freedom such as spins forms the basis of emerging quantum technologies. In this context, the robust valley degree of freedom and the associated valley pseudospin found in…

Mesoscale and Nanoscale Physics · Physics 2022-11-17 Mandeep Khatoniar , Nicholas Yama , Areg Ghazaryan , Sriram Guddala , Pouyan Ghaemi , Kausik Majumdar , Vinod Menon

Using the valley degree of freedom as a carrier of information for storage and processing, valley polarization plays a crucial role. A variety of mechanisms for valley polarization have been proposed, among which the valley-layer coupling…

Materials Science · Physics 2025-05-29 San-Dong Guo , Liguo Zhang , Xiao-Shu Guo , Gangqiang Zhu

Electron valleys in transition-metal dichalcogenide monolayers drive novel physics and allow designing multifunctional architectures for applications. We propose to manipulate the electron valleys in these systems for spin/valley filter and…

Mesoscale and Nanoscale Physics · Physics 2021-11-15 Ao Zhang , Kaike Yang , Yun Zhang , Anlian Pan , Mingxing Chen

A femtosecond laser pulse is able to switch the magnetic state of a 3d-4f ferrimagnetic material on a pico-second time scale. Devices based on this all-optical switching (AOS) mechanism are competitive candidates for ultrafast memory…

Applied Physics · Physics 2022-01-12 Pingzhi Li , Mark J. G. Peeters , Youri L. W. van Hees , Reinoud Lavrijsen , Bert Koopmans

Valley, as a new degree of freedom for electrons, has drawn considerable attention due to its significant potential for encoding and storing information. Lifting the energy degeneracy to achieve valley polarization is necessary for…

Materials Science · Physics 2020-03-11 Pei Zhaos , Yandong Ma , Hao Wang , Baibiao Huang , Liangzhi Kou , Ying Dai

Single-layer semiconducting transition-metal dichalcogenides, lacking point inversion symmetry, provide an efficient platform for valleytronics, where the electronic, magnetic, valley and lattice degrees of freedom can be selectively…

Mesoscale and Nanoscale Physics · Physics 2024-11-19 Emmanuele Cappelluti , Habib Rostami , Federico Cilento

Controlling the polarization state of light with sub-picosecond speed and subwavelength precision remains a key challenge for next-generation nanophotonic devices. Conventional methods such as birefringent crystals, liquid crystals, or…

Two-dimensional semimetals with tilted Dirac cones in the electronic band structure are shown to exhibit spatial separation of carriers belonging to different valleys under illumination. In stark contrast to gapped Dirac materials this…

Mesoscale and Nanoscale Physics · Physics 2023-11-08 A. Wild , E. Mariani , M. E. Portnoi

All-optical helicity dependent switching (AO-HDS), deterministic control of magnetization by circularly polarized laser pulses, allows to efficiently manipulate spins without the need of a magnetic field. However, AO-HDS in ferromagnetic…

Efficient electric manipulation of valley degrees of freedom is critical and challenging for the advancement of valley-based information science and technology. We put forth an electrical scheme, based on a two-band Dirac model, that can…

Mesoscale and Nanoscale Physics · Physics 2024-06-17 Yaqing Yang , Xiaoyu Cheng , Liantuan Xiao , Suotang Jia , Jun Chen , Lei Zhang , Jian Wang

Exciton polaritons based on atomically thin semiconductors are essential building blocks of quantum optoelectronic devices. Their properties are governed by an ultrafast and oscillatory energy transfer between their excitonic and photonic…

Despite much anticipation of valleytronics as a candidate to replace the ageing CMOS-based information processing, its progress is severely hindered by the lack of practical ways to manipulate valley polarization all-electrically in an…

Mesoscale and Nanoscale Physics · Physics 2017-12-15 Yee Sin Ang , Shengyuan A. Yang , C. Zhang , Zhongshui Ma , L. K. Ang

One of the key challenges for spintronic and novel quantum technologies is to achieve active control of the spin angular momentum of electrons in nanoscale materials on ultrafast, femtosecond timescales. While conventional ferromagnetic…

Mesoscale and Nanoscale Physics · Physics 2024-05-13 Benito Arnoldi , Sara L. Zachritz , Sebastian Hedwig , Martin Aeschlimann , Oliver L. A. Monti , Benjamin Stadtmüller

It is well established that light can control magnetism in matter, e.g. via the inverse Faraday effect or ultrafast demagnetization. However, such control is typically limited to magnetization transverse to light's polarization plane, or…

Optics · Physics 2025-12-17 Shuang Liu , Oren Cohen , Peng Chen , Ofer Neufeld

The dispersion scan (d-scan) technique is extended to measurement of the timedependent polarization state of ultrashort laser pulses. In the simplest implementation for linearly polarized ultrashort pulses, the d-scan technique records the…

Using symmetry breaking strain to tune the valley occupation of a two-dimensional (2D) electron system in an AlAs quantum well, together with an applied in-plane magnetic field to tune the spin polarization, we independently control the…

Strongly Correlated Electrons · Physics 2014-02-03 O. Gunawan , T. Gokmen , K. Vakili , M. Padmanabhan , E. P. De Poortere , M. Shayegan

The electron's charge and spin degrees of freedom are at the core of modern electronic devices. With the in-depth investigation of two-dimensional materials, another degree of freedom, valley, has also attracted tremendous research…

Materials Science · Physics 2023-09-06 Ping Li , Bang Liu , Wei-Xi Zhang , Zhi-Xin Guo

The direct gap interband transitions in transition metal dichalcogenides monolayers are governed by chiral optical selection rules. Determined by laser helicity, optical transitions in either the $K^+$ or $K^-$ valley in momentum space are…

Mesoscale and Nanoscale Physics · Physics 2016-10-26 G. Wang , X. Marie , B. L. Liu , T. Amand , C. Robert , F. Cadiz , P. Renucci , B. Urbaszek
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