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Spins confined in quantum dots are a leading candidate for solid-state quantum bits that can be coherently controlled by optical pulses. There are, however, many challenges to developing a scalable multibit information processing device…

Mesoscale and Nanoscale Physics · Physics 2012-09-26 Sophia E. Economou , Juan I. Climente , Antonio Badolato , Allan S. Bracker , Daniel Gammon , Matthew F. Doty

Spin-bearing molecules are promising building blocks for quantum technologies as they can be chemically tuned, assembled into scalable arrays, and readily incorporated into diverse device architectures. In molecular systems, optically…

Quantum Physics · Physics 2021-01-27 S. L. Bayliss , D. W. Laorenza , P. J. Mintun , B. Diler , D. E. Freedman , D. D. Awschalom

Optically addressable electronic spins in polyatomic molecules are a promising platform for quantum information science with the potential to enable scalable qubit design and integration through atomistic tunability and nanoscale…

Optically addressable spins at material surfaces have represented a long-standing ambition in quantum sensing, providing atomic resolution and quantum-limited sensitivity. However, they are constrained by a finite depth at which the quantum…

Optically addressable molecular triplet spins provide a chemically tunable platform for quantum application, but their coherence is often limited by interactions with surrounding spin baths. Here we demonstrate controlled suppression of…

Quantum technologies offer ways to solve certain tasks more quickly, efficiently, and with greater precision than their classical counterparts. Yet substantial challenges remain in the construction of sufficiently error-free and scalable…

Quantum Physics · Physics 2026-01-13 Calysta A. Tesiman , Mark Oxborrow , Max Attwood

Optically connecting quantum bits can effectively reduce decoherence and facilitate long-distance communication. Optically addressable spin-bearing molecules have been demonstrated to have a good potential for quantum computing. In this…

Quantum Physics · Physics 2023-03-28 Jiawei Chang , Tianhong Huang , Lin Ma , Taoyu Zou , Hai Wang , Wei Wu

Optical interfaces that connect long-lived spin qubits to photons are a central requirement for quantum networking and distributed quantum information processing. Currently, solid-state atomic defects are leading candidates due to their…

Exciting progress towards spin-based quantum computing has recently been made with qubits realized using nitrogen-vacancy (N-V) centers in diamond and phosphorus atoms in silicon, including the demonstration of long coherence times made…

Benefiting from both molecular tunability and versatile methods for deployment, optically interfaced molecular spins are a promising platform for quantum technologies such as sensing and imaging. Room-temperature optically detected coherent…

Creating a quantum-coherent architecture at the atomic scale has long been an ambition in quantum science and nanotechnology. This ultimate length scale requires the use of fundamental quantum properties of atoms, such as the spin of…

A key challenge in quantum computation is the implementation of fast and local qubit control while simultaneously maintaining coherence. Qubits based on hole spins offer, through their strong spin-orbit interaction, a way to implement fast…

Mesoscale and Nanoscale Physics · Physics 2021-03-04 F. N. M. Froning , L. C. Camenzind , O. A. H. van der Molen , A. Li , E. P. A. M. Bakkers , D. M. Zumbühl , F. R. Braakman

A key virtue of spin qubits is their sub-micron footprint, enabling a single silicon chip to host the millions of qubits required to execute useful quantum algorithms with error correction. With each physical qubit needing multiple control…

Optically addressable solid-state spins have been extensively studied for quantum technologies, offering unique advantages for quantum computing, communication, and sensing. Advancing these applications is generally limited by finding…

Hole spin qubits are frontrunner platforms for scalable quantum computers because of their large spin-orbit interaction which enables ultrafast all-electric qubit control at low power. The fastest spin qubits to date are defined in long…

Mesoscale and Nanoscale Physics · Physics 2022-10-18 Stefano Bosco , Daniel Loss

The states of a boron acceptor near a Si/SiO2 interface, which bind two low-energy Kramers pairs, have exceptional properties for encoding quantum information and, with the aid of strain, both heavy hole and light hole-based spin qubits can…

Mesoscale and Nanoscale Physics · Physics 2016-06-22 Joe Salfi , Mengyang Tong , Sven Rogge , Dimitrie Culcer

Manipulation of spin states at the single-atom scale underlies spin-based quantum information processing and spintronic devices. Such applications require protection of the spin states against quantum decoherence due to interactions with…

Mesoscale and Nanoscale Physics · Physics 2018-11-13 Yujeong Bae , Kai Yang , Philip Willke , Taeyoung Choi , Andreas J. Heinrich , Christopher P. Lutz

Long coherence time and compatibility with semiconductor fabrication make spin qubits in silicon an attractive platform for quantum computing. In recent years, hole spin qubits are being developed as they have the advantages of weak…

Mesoscale and Nanoscale Physics · Physics 2023-04-14 Shihang Zhang , Yu He , Peihao Huang

Molecules present a versatile platform for quantum information science, and are candidates for sensing and computation applications. Robust spin-optical interfaces are key to harnessing the quantum resources of materials. To date,…

Optically addressed atomic defects in the solid-state are widely used as single-photon sources and memories for quantum network applications. The solid-state environment allows for a high density of electron and nuclear spins with the…

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