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Motivation: A major challenge in metabolomics is annotation: assigning molecular structures to mass spectral fragmentation patterns. Despite recent advances in molecule-to-spectra and in spectra-to-molecular fingerprint prediction (FP),…

Quantitative Methods · Quantitative Biology 2025-06-10 Apurva Kalia , Yan Zhou Chen , Dilip Krishnan , Soha Hassoun

Detecting and quantifying products of cellular metabolism using Mass Spectrometry (MS) has already shown great promise in many biological and biomedical applications. The biggest challenge in metabolomics is annotation, where measured…

Machine Learning · Computer Science 2020-10-12 Hao Zhu , Liping Liu , Soha Hassoun

Compound identification and structure annotation from mass spectra is a well-established task widely applied in drug detection, criminal forensics, small molecule biomarker discovery and chemical engineering. We propose SpecTUS: Spectral…

Machine Learning · Computer Science 2026-02-23 Adam Hájek , Michal Starý , Elliott Price , Filip Jozefov , Helge Hecht , Aleš Křenek

Identifying a small molecule from its mass spectrum is the primary open problem in computational metabolomics. This is typically cast as information retrieval: an unknown spectrum is matched against spectra predicted computationally from a…

Machine Learning · Computer Science 2023-01-30 Michael Murphy , Stefanie Jegelka , Ernest Fraenkel , Tobias Kind , David Healey , Thomas Butler

Electrospray tandem mass spectrometry (ESI-MS/MS) is commonly used in high throughput metabolomics. One of the key obstacles to the effective use of this technology is the difficulty in interpreting measured spectra to accurately and…

Computational Engineering, Finance, and Science · Computer Science 2014-06-10 F. Allen , R. Greiner , D. Wishart

Accurately identifying metabolites i.e. small molecules from mass spectrometry data remains a core challenge in metabolomics, with broad applications in drug discovery, environmental analysis, and clinical research. We address the Molecule…

Deep learning based approaches have achieved significant progresses in different tasks like classification, detection, segmentation, and so on. Ensemble learning is widely known to further improve performance by combining multiple…

Computer Vision and Pattern Recognition · Computer Science 2019-05-17 Danlu Chen , Xu-Yao Zhang , Wei Zhang , Yao Lu , Xiuli Li , Tao Mei

Multi-task learning for molecular property prediction is becoming increasingly important in drug discovery. However, in contrast to other domains, the performance of multi-task learning in drug discovery is still not satisfying as the…

Biomolecules · Quantitative Biology 2022-10-07 Shengchao Liu , Meng Qu , Zuobai Zhang , Huiyu Cai , Jian Tang

Graph neural networks (GNNs) have shown considerable promise in computational chemistry. However, the limited availability of molecular data raises concerns regarding GNNs' ability to effectively capture the fundamental principles of…

Machine Learning · Computer Science 2025-03-12 Junyi An , Chao Qu , Yun-Fei Shi , XinHao Liu , Qianwei Tang , Fenglei Cao , Yuan Qi

Molecular property prediction (MPP) is a fundamental but challenging task in the computer-aided drug discovery process. More and more recent works employ different graph-based models for MPP, which have made considerable progress in…

Machine Learning · Computer Science 2023-12-29 Bangyi Zhao , Weixia Xu , Jihong Guan , Shuigeng Zhou

Untargeted metabolomic studies are revealing large numbers of naturally occurring metabolites that cannot be characterized because their chemical structures and MS/MS spectra are not available in databases. Here we present iMet, a…

Quantitative Methods · Quantitative Biology 2017-03-17 Antoni Aguilar-Mogas , Marta Sales-Pardo , Miriam Navarro , Ralf Tautenhahn , Roger Guimerà , Oscar Yanes

A key prerequisite to optimal reasoning under uncertainty in intelligent systems is to start with good class probability estimates. This paper improves on the current best probability estimation trees (Bagged-PETs) and also presents a new…

Machine Learning · Computer Science 2012-07-19 Rodney Nielsen

This work studies ensemble learning for graph neural networks (GNNs) under the popular semi-supervised setting. Ensemble learning has shown superiority in improving the accuracy and robustness of traditional machine learning by combining…

Machine Learning · Computer Science 2024-05-07 Xin Zhang , Daochen Zha , Qiaoyu Tan

Metabolite structure identification has become the major bottleneck of the mass spectrometry based metabolomics research. Till now, number of mass spectra databases and search algorithms have been developed to address this issue. However,…

Quantitative Methods · Quantitative Biology 2021-01-12 Hansen Zhao , Xu Zhao , Huan Yao , Jiaxin Feng , Sichun Zhang , Xinrong Zhang

Machine learning methods for identifying molecular structures from tandem mass spectra (MS/MS) have advanced rapidly, yet current approaches still exhibit significant error rates. In high-stakes applications such as clinical metabolomics…

Machine Learning · Computer Science 2026-03-12 Mira Jürgens , Gaetan De Waele , Morteza Rakhshaninejad , Willem Waegeman

In recent years, multi-label classification problem has become a controversial issue. In this kind of classification, each sample is associated with a set of class labels. Ensemble approaches are supervised learning algorithms in which an…

Machine Learning · Computer Science 2018-01-09 Amirreza Mahdavi-Shahri , Mahboobeh Houshmand , Mahdi Yaghoobi , Mehrdad Jalali

Untargeted metabolomics generates large volumes of tandem mass spectrometry (MS/MS) data and computational annotations that can reveal molecular mechanisms across organisms and environments. Public reuse has improved through harmonized…

Databases · Computer Science 2026-05-26 Matthieu Féraud , Dina Boukhajou , Fabien Gandon , Louis-Félix Nothias

Active learning generally involves querying the most representative samples for human labeling, which has been widely studied in many fields such as image classification and object detection. However, its potential has not been explored in…

Computer Vision and Pattern Recognition · Computer Science 2020-12-10 Jun Wang , Shaoguo Wen , Kaixing Chen , Jianghua Yu , Xin Zhou , Peng Gao , Changsheng Li , Guotong Xie

Supervised machine-learning models often underperform in predicting user behaviors from conversational text, hindered by poor crowdsourced label quality and low NLP task accuracy. We introduce the Metadata-Sensitive Weighted-Encoding…

Machine Learning · Computer Science 2025-05-29 Lynnette Hui Xian Ng , Kokil Jaidka , Kaiyuan Tay , Hansin Ahuja , Niyati Chhaya

Molecular Property Prediction (MPP) task involves predicting biochemical properties based on molecular features, such as molecular graph structures, contributing to the discovery of lead compounds in drug development. To address data…

Machine Learning · Computer Science 2023-12-07 Xu Yao , Shuang Liang , Songqiao Han , Hailiang Huang
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