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Colloidal building blocks with re-configurable shapes and dynamic interactions can exhibit unusual self-assembly behaviors and pathways. In this work, we consider the phase behavior of colloids coated with surface-mobile polymer brushes…

Soft Condensed Matter · Physics 2024-05-16 Yaxin Xu , Prabhat Jandhyala , Sho C. Takatori

In this work, we investigate the transient rheological behavior of two soft glassy materials: a clay dispersion and a silica gel, emphasizing their unconventional shear stress build-up behavior under conditions of constant imposed strain.…

Soft Condensed Matter · Physics 2025-04-02 Vivek Kumar , Gareth H McKinley , Yogesh M Joshi

The structure and degree of order in soft matter and other materials is intimately connected to the nature of the interactions between the particles. One important research goal is to find suitable control mechanisms, to enhance or suppress…

Soft Condensed Matter · Physics 2020-09-16 A. Scacchi , M. G. Mazza , A. J. Archer

Thermal greases, often used as thermal interface materials, are complex paste-like mixtures composed of a base polymer in which dense metallic (or ceramic) filler particles are dispersed to improve the heat transfer properties of the…

Suspensions are of wide interest and form the basis for many smart fluids. For most suspensions, the viscosity decreases with increasing shear rate, i.e. they shear thin. Few are reported to do the opposite, i.e. shear thicken, despite the…

The origin of the dramatic changes in the behavior of liquids as they approach their vitreous state - increases of many orders of magnitude in transport properties and dynamic time scales - is a major unsolved problem in condensed matter.…

Soft Condensed Matter · Physics 2015-06-23 R. Casalini , D. Fragiadakis , C. M. Roland

The sticking of a soft polystyrene colloidal particle to a planar glass plate was studied by a microrheological technique using an optical tweezer to trap the particle and a piezoelectric-stage to position the plate and to sinusoidally…

Soft Condensed Matter · Physics 2009-08-27 Prerna Sharma , Shankar Ghosh , S. Bhattacharya

The results obtained from molecular dynamics simulations of the friction at an interface between polymer melts and weakly attractive crystalline surfaces are reported. We consider a coarse-grained bead-spring model of linear chains with…

Soft Condensed Matter · Physics 2012-06-12 Nikolai V. Priezjev

The behavior of suspensions of rigid particles in a non-Newtonian fluid is studied in the framework of a nonlinear homogenization method. Estimates for the overall properties of the composite material are obtained. In the case of a…

Soft Condensed Matter · Physics 2010-07-28 Xavier Chateau , Guillaume Ovarlez , Kien Luu Trung

We investigate the structure and equilibrium linear-response dynamics of suspensions of hard colloidal dumbbells using Brownian Dynamics computer simulations. The focus lies on the dense fluid and plastic crystal states of the colloids with…

Soft Condensed Matter · Physics 2015-07-10 Nils Heptner , Joachim Dzubiella

Under an increasing applied shear stress ($\sigma$), viscosity of many dense particulate suspensions increases drastically beyond a stress onset ($\sigma_0$), a phenomenon known as discontinuous shear-thickening (DST). Recent studies point…

Soft Condensed Matter · Physics 2020-01-29 Subhransu Dhar , Sebanti Chattopadhyay , Sayantan Majumdar

The sliding of non-Newtonian drops down planar surfaces results in a complex, entangled balance between interfacial forces and non linear viscous dissipation, which has been scarcely inspected. In particular, a detailed understanding of the…

Soft Condensed Matter · Physics 2017-03-31 Silvia Varagnolo , Daniele Filippi , Giampaolo Mistura , Matteo Pierno , Mauro Sbragaglia

We develop a kinetic-theory framework to investigate the steady rheology of a dilute gas interacting via a repulsive potential under uniform shear flow. Starting from the Boltzmann equation with a restitution coefficient that depends on the…

Soft Condensed Matter · Physics 2026-04-23 Yuria Kobayashi , Makoto R. Kikuchi , Shunsuke Iizuka , Satoshi Takada

Dense suspensions of small strongly interacting particles are complex systems, which are rarely understood on the microscopic level. We investigate properties of dense suspensions and sediments of small spherical Al_2O_3 particles in a…

Soft Condensed Matter · Physics 2007-05-23 Martin Hecht , Jens Harting , Markus Bier , Joerg Reinshagen , Hans J. Herrmann

We investigated the effects of particle shape on shear thickening in densely packed suspensions. Rods of different aspect ratios and non-convex hooked rods were fabricated. Viscosity curves and normal stresses were measured using a…

We identify the sequence of microstructural changes that characterize the evolution of an attractive particulate gel under flow and discuss their implications on macroscopic rheology. Dissipative Particle Dynamics (DPD) is used to monitor…

Soft Condensed Matter · Physics 2017-02-07 Safa Jamali , Gareth H. McKinley , Robert C. Armstrong

The synchronized molecular dynamics simulation via macroscopic heat and momentum transfer is proposed for the non-isothermal flow behaviors of complex fluids. In this method, the molecular dynamics simulations are assigned to small fluid…

Soft Condensed Matter · Physics 2014-10-29 Shugo Yasuda , Ryoichi Yamamoto

Discrete particle simulations are used to study the shear rheology of dense, stabilized, frictional particulate suspensions in a viscous liquid, toward development of a constitutive model for steady shear flows at arbitrary stress. These…

Soft Condensed Matter · Physics 2018-02-14 Abhinendra Singh , Romain Mari , Morton M. Denn , Jeffrey F. Morris

Dense suspensions can exhibit an abrupt change in their viscosity in response to increasing shear rate. The origin of this discontinuous shear thickening (DST) has been ascribed to the transformation of lubricated contacts to frictional,…

Soft Condensed Matter · Physics 2017-08-02 Sumantra Sarkar , Elan Shatoff , Kabir Ramola , Romain Mari , Jeffrey Morris , Bulbul Chakraborty

Introducing a reduced particle stiffness in discrete element method (DEM) allows for bigger time steps and therefore fewer total iterations in a simulation. Although this approach works well for dry non-adhesive particles, it has been shown…

Soft Condensed Matter · Physics 2018-10-17 Sheng Chen , Wenwei Liu , Shuiqing Li