Related papers: Electron transfer under the Floquet modulation in …
Floquet systems are governed by periodic, time-dependent, Hamiltonians. Prima facie they should absorb energy from the external drives involved in modulating their couplings and heat up to infinite temperature. However this unhappy state of…
The rate of electron transfer between a molecular species and a metal, each at a different local temperature, is examined theoretically through implementation of a bithermal (characterized by two temperatures) Marcus formalism. Expressions…
We study qubit-mediated energy transfer between two electron reservoirs by adopting a numerically-exact influence functional path-integral method. This non-perturbative technique allows us to study the system's dynamics beyond the weak…
The influence of an intramolecular proton transfer reaction on the conductance of a molecular junction is investigated employing a generic model, which includes the effects of the electric field of the gate and leads electrodes and the…
The effect of solvation on the electron transfer (ET) rate processes is investigated on the basis of the exact theory constructed in J. Phys. Chem. B Vol. 110, (2006); quant-ph/0604071. The nature of solvation is studied in a close relation…
"Floquet engineering" - designing band structures "on-demand" through the application of coherent time-periodic drives - has recently emerged as a powerful tool for creating new topological and anomalous phases of matter. In this…
Interband and intraband transitions are fundamental concepts in the study of electronic properties of materials, particularly semiconductors and nanomaterials. These transitions involve the movement of electrons between distinct energy…
We provide physically intuitive mechanisms for the effect of noise on excitation energy transfer (EET) in networks. Using these mechanisms of dephasing-assisted transport (DAT) in a hybrid basis of both excitons and sites, we develop a…
It is shown how the exchange interaction, the dipole-dipole interaction, and the Dzyaloshinsky-Moriya interaction between electronic spin-density fluctuations emerge naturally from a field-theoretic framework that couples electrons to the…
We experimentally observe Floquet Raman transitions in the weakly driven solid state spin system of nitrogen-vacancy center in diamond. The periodically driven spin system simulates a two-band Wannier-Stark ladder model, and allows us to…
Nanoscale molecular-electronic devices and machines are emerging as promising functional elements, naturally flexible and efficient, for next generation technologies. A deeper understanding of carrier dynamics in molecular junctions is…
We present a real-time path integral theory for the rate of electron transfer reactions. Using graph theoretic techniques, the dynamics is expressed in a formally exact way as a set of integral equations. With a simple approximation for the…
We consider the phenomenon of electric Mott transition (EMT), which is an electric induced insulator to metal transition. Experimentally, it is observed that depending on the magnitude of the electric excitation the final state may show a…
The realization of single-molecule thermal conductance measurements has driven the need for theoretical tools to describe conduction processes that occur over atomistic length scales. In macroscale systems, the principle that is typically…
By means of a Floquet analysis, we study the quantum dynamics of a fully connected Lipkin-Ising ferromagnet in a periodically driven transverse field showing that thermalization in the steady state is intimately connected to properties of…
Emulation of energy transfer processes in natural systems on quantum platforms can further our understanding of complex dynamics in nature. One notable example is the demonstration of vibrationally assisted energy transfer (VAET) on a…
The Forster resonant energy transfer mechanism (FRET) is investigated in optically driven and electrically gated tunnel coupled quantum dot molecules. Two novel FRET induced optical signatures are found in the dressed excitonic spectrum.…
We propose a method to study the time evolution of correlated electrons driven by an harmonic perturbation. Combining Floquet formalism to include the time-dependent field and Cluster Perturbation Theory to solve the many-body problem in…
Excited-state charge-transfer complexes (exciplexes) have been actively exploited in organic optoelectronic devices to improve performance; however, diffusion of exciplexes has not been actively studied despite its influence on performance…
Controlling the direction and magnitude of both heat and electronic currents using rectifiers has significant implications for the advancement of molecular circuit design. In order to facilitate the implementation of new transport phenomena…