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Arrays of optically trapped nanoparticles have emerged as a promising platform for the study of complex non-equilibrium phenomena. Analogous to atomic many-body systems, one of the crucial ingredients is the ability to precisely control the…

A novel approach for the state-specific enantiomeric enrichment and the spatial separation of enantiomers is presented. Our scheme utilizes techniques from strong-field laser physics, specifically an optical centrifuge in conjunction with a…

Chemical Physics · Physics 2019-12-18 Andrey Yachmenev , Jolijn Onvlee , Emil Zak , Alec Owens , Jochen Küpper

A highly-efficient method for optical detection and separation of left- and right-handed chiral molecules is presented. The method utilizes a closed-loop three-state system in which the population dynamics depends on the phases of the three…

Quantum Physics · Physics 2019-05-08 Nikolay V. Vitanov , Michael Drewsen

We present an optomechanical model that describes the stochastic motion of an overdamped chiral nanoparticle diffusing in the optical bistable potential formed in the standing-wave of two counter-propagating Gaussian beams. We show how…

Quantum Physics · Physics 2022-01-05 Gabriel Schnoering , Samuel Albert , Antoine Canaguier-Durand , Cyriaque Genet

Advanced photonic nanostructures have enabled the maximization of synthetic chiroptic activities. The unique structuring of these building blocks has empowered chiral selective interactions with electromagnetic waves in plasmonic structures…

The recoil optical force that acts on emitters near a surface or waveguide relies on near-field directionality and conservation of momentum. It features desirable properties uncommon in optical forces, such as the ability to produce it via…

Optics · Physics 2020-07-02 J. A. Girón-Sedas , Francisco J. Rodríguez-Fortuño

All-dielectric "magnetic light" nanophotonics based on high refractive index nanoparticles allows controlling magnetic component of light at nanoscale without having high dissipative losses. The artificial magnetic optical response of such…

State-selective enantiomeric excess is realized using microwave-driven coherent population transfer. The method selectively promotes either R or S molecules to a higher rotational state by phase-controlled microwave pulses that drive…

Chemical Physics · Physics 2017-03-23 Sandra Eibenberger , John Doyle , David Patterson

A novel optical method for distinguishing chiral molecules is proposed and validated within a quantum simulator employing a trapped-ion qudit. This approach correlates the sign disparity of the dipole moment of chiral molecules with…

Quantum Physics · Physics 2024-03-11 Teng Liu , Fa Zhao , Pengfei Lu , Qifeng Lao , Min Ding , Ji Bian , Feng Zhu , Le Luo

Molecular chirality plays an important role in chemistry and biology, allows control of biological interactions, affects drugs efficacy and safety, and promotes synthesis of new materials. In general, chirality manifests itself in optical…

Optics · Physics 2026-04-10 Yuanyang Xie , Alexey V. Krasavin , Anatoly V. Zayats

Chirality is an intriguing property of certain molecules, materials or artificial nanostructures, which allows them to interact with the spin angular momentum of the impinging light field. Due to their chiral geometry, they can distinguish…

Optics · Physics 2016-11-03 Peter Banzer , Pawel Wozniak , Uwe Mick , Israel De Leon , Robert W. Boyd

We introduce and theoretically analyze the concept of manipulating optical chirality via strong coupling of the optical modes of chiral nanostructures with excitonic transitions in molecular layers or semiconductors. With chirality being…

Many nanophotonic applications require precise control and characterization of electromagnetic field properties at the nanoscale. The chiral properties of the field are among its key characteristics, yet measurement of optical chirality at…

Optics · Physics 2022-02-18 Abid Anjum Sifat , Filippo Capolino , Eric O. Potma

We analyze how chirality can generate pulling optical forces and left-handed torques by cross-coupling linear-to-angular momenta between the light field and the chiral object. In the dipolar regime, we reveal that such effects can emerge…

Optics · Physics 2015-03-10 Antoine Canaguier-Durand , Cyriaque Genet

We report for the first time the theory of optical tweezers of spherical dielectric particles embedded in a chiral medium. We develop a partial-wave (Mie) expansion to calculate the optical force acting on a dielectric microsphere…

Optics · Physics 2020-09-28 Rfaqat Ali , R. S. Dutra , F. A. Pinheiro , F. S. S. Rosa , P. A. Maia Neto

Optical forces acting on nano-sized particles are typically too small to be useful for particle manipulation. We theoretically and numerically demonstrate a mechanism that can significantly enhance the optical force acting on a small…

Optics · Physics 2016-03-15 Shubo Wang , C. T. Chan

Selective sensing of chiral molecules is a key aspect in fields spanning biology, chemistry, and pharmacology. However, conventional optical methods, such as circular dichroism (CD), encounter limitations owing to weak chiral light-matter…

Silicon nanoparticles possess unique size-dependent optical properties due to their strong electric and magnetic resonances in the visible range. However, their widespread application has been limited, in comparison to other (e.g. metallic)…

Three-wave mixing spectroscopy of chiral molecules, which exist in left-handed and right-handed conformations, allows for enantio-selective population transfer despite random orientation of the molecules. This is based on constructive…

Quantum Physics · Physics 2019-07-09 Monika Leibscher , Thomas F. Giesen , Christiane P. Koch

We propose a method to realize enantiodiscrimination of chiral molecules based on quantum correlation function in a driven cavity-molecule system, where the chiral molecule is coupled with a quantized cavity field and two classical light…

Quantum Physics · Physics 2022-08-12 Fen Zou , Yu-Yuan Chen , Bo Liu , Yong Li
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