Related papers: Second-Harmonic Generation in Bulk Diamond Based o…
We develop a quantitative mathematical theory that offers new perspectives on nonlinear harmonic generation in plasmonic structures arising from symmetry breaking. Focusing on second harmonic generation--the most fundamental process and the…
Ensembles of negatively charged nitrogen vacancy centers (NV-) in diamond have been proposed for sensing of magnetic fields and paramagnetic agents, and as a source of spin-order for the hyperpolarization of nuclei in magnetic resonance…
Nanophotonics research has focused recently on the ability of non-linear optical processes to mediate and transform optical signals in a myriad of novel devices, including optical modulators, transducers, color filters, photodetectors,…
Second-harmonic generation (SHG) is a fundamental tool in modern laser technology, enabling coherent frequency conversion to remote optical bands, serving as the basis for self-referenced femtosecond lasers and quadrature-squeezed light…
We analytically investigate the effect of a non-centrosymmetric geometry in the optical second harmonic (SH) generation from a particle made of a centrosymmetric material, in the interior of which quadratic optical processes are suppressed.…
Nonlinear optical processes associated with even-order nonlinear susceptibilities are critical for both classical and quantum technologies. Inversion symmetry, however, prevents nonlinear optical responses mediated by even-order…
We experimentally explore the fingerprint of the microscopic electron dynamics in second-order harmonic generation (SHG). It is shown that the interbond electron hopping induces a novel source of nonlinear polarization and plays an…
Second-harmonic generation (SHG) is a well-known nonlinear spectroscopy method to probe electronic structure, specifically, in transition metal dichalcogenide (TMDC) monolayers. This work investigates the nonlinear dynamics of a strongly…
Boosting nonlinear frequency conversion in extremely confined volumes remains a key challenge in nano-optics, nanomedicine, photocatalysis, and background-free biosensing. To this aim, field enhancements in plasmonic nanostructures are…
We demonstrate that high-harmonic generation (HHG) in solids dominantly originates from strongly localized surface states through non-perturbative processes. Measurements reveal that HHG from bulk states is suppressed by at least 1-2 orders…
In our previous work [2], it has been found that sizable charmonium events via the channel $e^+e^- \to \gamma^*/Z^0 \to H(|c\bar{c}\rangle) +\gamma$ can be produced at the suggested super $Z$ factory, where $H(|c\bar{c}\rangle)$ represents…
We report the first observation of nonlinear harmonic generation and sum frequency generation (SFG) coupled with stimulated Raman scattering (SRS) via the second-order (\chi^{(2)}) and the third-order (\chi^{(3)}) nonlinearities in a silica…
Silicon photonics lacks a second-order nonlinear optical response in general because the typical constituent materials are centro-symmetric and lack inversion symmetry, which prohibits second-order nonlinear processes such as second…
Chip-scale nonlinear optics enables strong light-matter interactions within compact devices, serving as a fundamental platform for multifunctional integrated photonics from classical optical signal processing to quantum information…
We analytically and numerically investigate the emission of high-harmonic radiation from model solids by intense few-cycle mid-infrared laser pulses. In single-active-electron approximation, we expand the active electron's wavefunction in a…
Dynamical control of the nonlinear optical properties of solids -- with light itself -- will be essential for future ultrafast photonic technologies. Previously, methods to modulate nonlinear processes including second-harmonic generation…
Optical coating, an integral part of many optical systems, is prone to damage from environmental exposure and laser irradiation. This underscores the need for reliable and sensitive coating diagnostics. We introduce second harmonic…
High-harmonic generation (HHG) in solids has been touted as a way to probe ultrafast dynamics and crystal symmetries in condensed matter systems. Here, we investigate the polarization properties of high-order harmonics generated in…
High-harmonic generation (HHG) is a strong-field phenomenon that is sensitive to the attosecond dynamics of tunnel ionization and coherent transport of electron-hole pairs in solids. While the foundations of solid HHG have been established,…
Parametric oscillation is a fundamental concept that underlies nonlinear wave-matter interactions, leading to generation or amplification of new frequency components. Using a temporal modulation generated by the heterodyne interference of a…