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We report magneto-optical trapping (MOT) of a polyatomic molecule, calcium monohydroxide (CaOH). The MOT contains $2.0(5)\times 10^4$ CaOH molecules at a peak density of $3.0(8)\times10^{6}$ cm$^{-3}$. CaOH molecules are further sub-Doppler…

Calcium monofluoride (CaF) molecules are loaded into an optical dipole trap (ODT) and subsequently laser cooled within the trap. Starting with magneto-optical trapping, we sub-Doppler cool CaF and then load $150(30)$ CaF molecules into an…

Direct laser cooling and trapping of molecules to temperature below Doppler limit and density exceeding $10^8$ are challenging due to the sub-Doppler heating effects of molecular magneto-optical trap (MOT). In our previous paper [1], we…

Atomic Physics · Physics 2023-05-29 S. Xu , R. Li , Y. Zhai , Y. Xia , M. Siercke , S. Ospelkaus

The grating magneto-optical trap (GMOT) requires only one beam and three planar diffraction gratings to form a cloud of cold atoms above the plane of the diffractors. Despite the complicated polarization arrangement, we demonstrate…

Atomic Physics · Physics 2013-10-15 J. Lee , J. A. Grover , L. A. Orozco , S. L. Rolston

We study theoretically the behavior of laser-cooled calcium monofluoride (CaF) molecules in an optical molasses and magneto-optical trap (MOT), and compare our results to recent experiments. We use multi-level optical Bloch equations to…

Atomic Physics · Physics 2021-05-18 J. A. Devlin , M. R. Tarbutt

We demonstrate significantly improved magneto-optical trapping of molecules using a very slow cryogenic beam source and RF modulated and DC magnetic fields. The RF MOT confines $1.1(3) \times 10^5$ CaF molecules at a density of $4(1) \times…

We have experimentally studied sub-Doppler laser cooling in a magneto-optical trap for thulium atoms working at the wavelength of 410.6\,nm. Without any dedicated molasses period of sub-Doppler cooling, the cloud of $3\times 10^6$ atoms at…

Quantum Physics · Physics 2015-05-20 D. Sukachev , A. Sokolov , K. Chebakov , A. Akimov , S. Kanorsky , N. Kolachevsky , V. Sorokin

Recent experiments have demonstrated direct cooling and trapping of diatomic and triatomic molecules in magneto-optical traps (MOTs). However, even the best molecular MOTs to date still have density $10^{-5}$ times smaller than in typical…

Atomic Physics · Physics 2023-04-19 Thomas K. Langin , David DeMille

Magneto-optical trapping forces for molecules are far weaker than for alkali atoms because the photon scattering rate is reduced when there are multiple ground states, and because of optical pumping into dark states. The force is further…

Atomic Physics · Physics 2021-12-14 M. R. Tarbutt , T. C. Steimle

Ultracold atoms at temperatures close to the recoil limit have been achieved by extending Doppler cooling to forbidden transitions. A cloud of ^40Ca atoms has been cooled and trapped to a temperature as low as 6 \mu K by operating a…

Atomic Physics · Physics 2015-11-30 T. Binnewies , G. Wilpers , U. Sterr , F. Riehle , J. Helmcke , T. E. Mehlstäubler , E. M. Rasel , W. Ertmer

In red-detuned magneto-optical traps (MOTs) of molecules, sub-Doppler heating competes with Doppler cooling, resulting in high temperature and low density. A solution is offered by the blue-detuned MOT where sub-Doppler cooling dominates…

Atomic Physics · Physics 2026-01-30 Qinshu Lyu , M. R. Tarbutt

Laser cooling and trapping are central to modern atomic physics. The workhorse technique in cold-atom physics is the magneto-optical trap (MOT), which combines laser cooling with a restoring force from radiation pressure. For a variety of…

Atomic Physics · Physics 2014-10-20 J. F. Barry , D. J. McCarron , E. B. Norrgard , M. H. Steinecker , D. DeMille

We demonstrate optical cycling and sub-Doppler laser cooling of a cryogenic buffer-gas beam of calcium monohydride (CaH) molecules. We measure vibrational branching ratios for laser cooling transitions for both excited electronic states A…

Atomic Physics · Physics 2022-08-24 S. F. Vázquez-Carson , Q. Sun , J. Dai , D. Mitra , T. Zelevinsky

The ability to cool atoms below the Doppler limit -- the minimum temperature reachable by Doppler cooling -- has been essential to most experiments with quantum degenerate gases, optical lattices and atomic fountains, among many other…

Atomic Physics · Physics 2018-01-17 S. Truppe , H. J. Williams , M. Hambach , L. Caldwell , N. J. Fitch , E. A. Hinds , B. E. Sauer , M. R. Tarbutt

Direct laser cooling of molecules has reached a phase space density exceeding 10$^{-6}$ in optical traps, but with rather small molecular numbers. To progress towards quantum degeneracy, a mechanism is needed that combines sub-Doppler…

Atomic Physics · Physics 2023-05-24 Justin J. Burau , Parul Aggarwal , Kameron Mehling , Jun Ye

We theoretically investigate the damping and trapping forces in a three-dimensional magneto-optical trap (MOT), by numerically solving the optical Bloch equations. We focus on the case where there are dark states because the atom is driven…

Atomic Physics · Physics 2017-03-29 J. A. Devlin , M. R. Tarbutt

We demonstrate sub-Doppler cooling of calcium atoms using a two-photon transition from the ${^1}S_0$ ground state to the upper $4s5s~{^1}S_0$ state via the ${^1}P_1$ intermediate state. We achieve temperatures as low as $260~\mu\text{K}$ in…

We investigate cooling mechanisms in magneto-optically and magnetically trapped erbium. We find efficient sub-Doppler cooling in our trap, which can persist even in large magnetic fields due to the near degeneracy of two Lande g factors.…

Atomic Physics · Physics 2009-09-29 Andrew J. Berglund , Siu Au Lee , Jabez J. McClelland

We present the properties of a magneto-optical trap (MOT) of CaF molecules. We study the process of loading the MOT from a decelerated buffer-gas-cooled beam, and how best to slow this molecular beam in order to capture the most molecules.…

Atomic Physics · Physics 2017-12-06 H. J. Williams , S. Truppe , M. Hambach , L. Caldwell , N. J. Fitch , E. A. Hinds , B. E. Sauer , M. R. Tarbutt

We demonstrate loading of SrF molecules into an optical dipole trap (ODT) via in-trap $\Lambda$-cooling. We find that this cooling can be optimized by a proper choice of relative ODT and $\Lambda$ beam polarizations. In this optimized…

Atomic Physics · Physics 2021-10-27 Thomas K. Langin , Varun Jorapur , Yuqi Zhu , Qian Wang , David DeMille
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