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We study theoretically the excitonic nonlinearity in hybrid organic-inorganic Ruddlesden-Popper perovskite thin films. The composite layered structure of these materials allows for flexible modulation of their excitonic response between the…

Mesoscale and Nanoscale Physics · Physics 2022-11-14 D. A. Baghdasaryan , E. S. Hakobyan , D. B. Hayrapetyan , I. V. Iorsh , I. A. Shelykh , V. Shahnazaryan

Exciton-polaritons, hybrid light-matter elementary excitations arising from the strong coupling regime between excitons in semiconductors and photons in photonic nanostructures, offer a fruitful playground to explore the physics of quantum…

The Mott transition from a dipolar excitonic liquid to an electron-hole plasma is demonstrated in a wide GaN/(Al,Ga)N quantum well at $T=7$K by means of spatially-resolved magneto-photoluminescence spectroscopy. Increasing optical…

Mesoscale and Nanoscale Physics · Physics 2021-02-03 F. Chiaruttini , T. Guillet , C. Brimont , D. Scalbert , S. Cronenberger , B. Jouault , P. Lefebvre , B. Damilano , M. Vladimirova

A recent single quantum wire is of sufficient quality to reveal new details of the photoluminescence (PL) evolution with increasing electron--hole (e--h) pair density. At a pair density of 3.6 $\times$ 10$^{3}$ cm$^{-1}$, the PL is…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Masahiro Yoshita , Yuhei Hayamizu , Hidefumi Akiyama , Loren N. Pfeiffer , Ken W. West , Kenichi Asano , Tetsuo Ogawa

Photoluminescence is commonly used to identify the electronic structure of individual nanotubes. But, nanotubes naturally occur in bundles. Thus, we investigate photoluminescence of nanotube bundles. We show that their complex spectra are…

Materials Science · Physics 2015-05-13 P. H. Tan , A. G. Rozhin , T. Hasan , P. Hu , V. Scardaci , W. I. Milne , A. C. Ferrari

We use path integral Monte Carlo to study the energetics of excitons in layered, hybrid organic-inorganic perovskites in order to elucidate the relative contributions of dielectric confinement and electron-phonon coupling. While the…

Materials Science · Physics 2025-03-26 Rohit Rana , David T. Limmer

Spin or valley degrees of freedom in condensed matter have been proposed as efficient information carriers towards next generation spintronics. It is therefore crucial to develop effective strategies to generate and control spin or…

Mesoscale and Nanoscale Physics · Physics 2023-04-26 Ying Shi , Yusong Gan , Yuzhong Chen , Yubin Wang , Sanjib Ghosh , Alexey Kavokin , Qihua Xiong

The evolution of charge carriers in photoexcited room temperature ZnO nanoparticles in solution is investigated using ultrafast ultraviolet photoluminescence spectroscopy, ultrafast Zn K-edge absorption spectroscopy and ab-initio molecular…

The effectiveness of molecular-based light harvesting relies on transport of optical excitations, excitons, to charg-transfer sites. Measuring exciton migration has, however, been challenging because of the mismatch between nanoscale…

Materials Science · Physics 2017-11-22 Samuel B. Penwell , Lucas D. S. Ginsberg , Rodrigo Noriega , Naomi S. Ginsberg

Excitons, Coulomb-bound electron and hole pairs, are elementary photo-excitations in semiconductors, that can couple directly to light through radiative relaxation. In contrast to these bright excitons, dark excitons X$\rm{_D}$ with…

Materials Science · Physics 2018-02-14 Kyoung-Duck Park , Tao Jiang , Genevieve Clark , Xiaodong Xu , Markus B. Raschke

Excitons, composite electron-hole quasiparticles, are known to play an important role in optoelectronic phenomena in many semiconducting materials. Recent experiments and theory indicate that the band-gap optics of the newly discovered…

Mesoscale and Nanoscale Physics · Physics 2015-09-02 Yuri N. Gartstein , Xiao Li , Chuanwei Zhang

Carrier multiplication by singlet exciton fission enhances photovoltaic conversion efficiencies in organic solids. This decay of one singlet exciton into two triplet states promises to overcome the Shockley-Queisser limit as up to two…

Materials Science · Physics 2016-12-16 K. Kolata , S. Marquardt , N. W. Rosemann , A. Mager , A. Hansmann , U. Höfer , R. Berger , T. Breuer , G. Witte , S. Chatterjee

Exciton-polaritons offer a versatile platform for realization of all-optical integrated logic gates due to the strong effective optical nonlinearity resulting from the exciton-exciton interactions. In most of the current excitonic materials…

Excitons play an essential role in the optical response of two-dimensional materials. These are bound states showing up in the band gaps of many-body systems and are conceived as quasiparticles formed by an electron and a hole. By…

In high performance perovskite based solar cells, CH3NH3PbI3 is the key material. We carried out a study on charge diffusion in spin-coated CH3NH3PbI3 perovskite thin film by transient fluorescent spectroscopy. A thickness-dependent…

Chemical Physics · Physics 2015-10-02 Yu Li , Weibo Yan , Yunlong Li , Shufeng Wang , Wei Wang , Zuqiang Bian , Lixin Xiao , Qihuang Gong

Exciton-phonon interactions govern the energy level spectrum and thus the optical response in semiconductors. In this respect, lead-halide perovskite nanocrystals represent a unique system, for which the interaction with optical phonons is…

Following the ultrafast photoexcitation of a semiconductor, it embodies competing dynamics among photocarriers, many-body transient states of highly energetic excitons, and electron-hole liquid. Here, we show that femtosecond optical pulse…

Materials Science · Physics 2026-03-30 Neetesh Dhakar , Sunil Kumar

Excitons play major roles in optical processes in modern semiconductors, such as single-wall carbon nanotubes (SWCNTs), transition metal dichalcogenides, and 2D perovskite quantum wells. They possess extremely large binding energies…

Tightly bound excitons in monolayer semiconductors represent a versatile platform to study two-dimensional propagation of neutral quasiparticles. Their intrinsic properties, however, can be severely obscured by spatial energy fluctuations…