English
Related papers

Related papers: Molecular Orientation-Induced Second Harmonic Gene…

200 papers

Thermotropic liquid crystals are versatile optical materials that exhibit a state of matter intermediate between liquids and solids. Their properties can change significantly with temperature, pressure, or other external factors, leading to…

High-order harmonic generation (HHG) from aligned acetylene molecules interacting with mid infra-red (IR), linearly polarized laser pulses is studied theoretically using a mixed quantum-classical approach in which the electrons are…

Atomic Physics · Physics 2018-05-18 Peter Mulholland , Daniel Dundas

Polarization plays an important role in various time-domain astrophysics to understand the magnetic fields, geometry, and environments of spatially unresolved variable sources. In this paper we present the results of laboratory and on-sky…

Instrumentation and Methods for Astrophysics · Physics 2020-04-29 Manisha Shrestha , Iain A. Steele , Andrez S. Piascik , Helen Jermak , Robert J. Smith , Chris M. Copperwheat

Generation of electromagnetic radiation near the second harmonic of the plasma frequency during the injection of an electron beam into a rippled-density plasma channel is investigated using both analytical theory and particle-in-cell…

Plasma Physics · Physics 2019-05-01 V. V. Annenkov , E. A. Berendeev , E. P. Volchok , I. V. Timofeev

Research of the nonlinear optical characteristics of transition metal dichalcogenides in the presence of photoactive particles, plasmonic nanocavities, waveguides, and metamaterials is still in its early stages. This investigation delves…

A comparative experimental investigation of the dependence of second harmonic generation (SHG) on applied external voltage between the standard nematic liquid crystalline material and an analogue ferromagnetic nematic liquid crystalline…

Soft Condensed Matter · Physics 2019-09-30 Jure Brence , Luka Cmok , Nerea Sebastian , Alenka Mertelj , Darja Lisjak , Irena Drevensek-Olenik

We investigate the effect of phase modulation of laser beams on the coherent and incoherent non-linear signals arising from the interaction of femtosecond pulses with matter. We observe that two collinear beams, whose phases are modulated…

Optics · Physics 2015-05-29 Khadga Jung Karki , Loni Kringle , Andrew H. Marcus , Tõnu Pullerits

When circularly polarized light is scattered from a rotating target, a rotational Doppler shift (RDS) emerges from an exchange of angular momentum between the spinning object and the electromagnetic field. Here, we used coherently spinning…

Metrology in atomic physics has been crucial for a number of advanced determinations of fundamental constants. In addition to very precise frequency measurements, the molar polarizability of an atomic gas has recently also been measured…

Atomic Physics · Physics 2013-09-10 U. D. Jentschura , M. Puchalski , P. J. Mohr

Chiral discrimination with high harmonic generation (cHHG method) has been introduced in the recent work by R. Cireasa et al ( Nat. Phys. 11, 654 - 658, 2015). In its original implementation, the cHHG method works by detecting high harmonic…

Optics · Physics 2015-10-28 Olga Smirnova , Yann Mairesse , Serguei Patchkovskii

We propose and computationally study a method for simultaneously orienting the angular momentum of asymmetric top molecules along: 1) a laboratory-fixed direction; 2) the molecular intermediate moment of inertia axis; 3) the laser field…

Quantum Physics · Physics 2022-11-21 Emil J. Zak

The generation process of second harmonic (SH) radiation from holes periodically arranged on a metal surface is investigated. Three main modulating factors affecting the optical response are identified: the near-field distribution at the…

Mesoscale and Nanoscale Physics · Physics 2015-01-08 Sergio G. Rodrigo , V. Laliena , L. Martín-Moreno

Intense single-cycle THz pulses resonantly interacting with molecular rotations are shown to induce significant field-free orientation under ambient conditions. We calculate and measure the angular distribution associated with THz-driven…

Chemical Physics · Physics 2015-05-28 Sharly Fleischer , Yan Zhou , Robert W. Field , Keith A. Nelson

Light with spatiotemporal orbital angular momentum (ST-OAM) is a recently discovered type of structured and localized electromagnetic field. This field carries characteristic space-time spiral phase structure and transverse intrinsic OAM.…

Context. Polarized dust emission can be used as a probe for magnetic fields at different scales. In particular, the analysis of the relative orientation between the density structures and the magnetic field projected on the plane of the sky…

Astrophysics of Galaxies · Physics 2021-03-24 Elisabetta R. Micelotta , Mika Juvela , Paolo Padoan , Isabelle Ristorcelli , Dana Alina , Johanna Malinen

Comparative analysis of second harmonic generation in ordinary and backward-wave settings is presented. Extraordinary properties of frequency doubling nonlinear optical reflectivity and pulse shaping through phase matching of ordinary and…

Optics · Physics 2016-02-02 Alexander K. Popov , Sergey A. Myslivets

We present an experimental technique using orbital angular momentum (OAM) in a fundamental laser field to drive High Harmonic Generation (HHG). The mixing of beams with different OAM allows to generate two laser foci tightly spaced to study…

Chemical Physics · Physics 2019-07-24 Jan Troßand Carlos A. Trallero-Herrero

Polaritonic states arise when a bright optical transition of a molecular ensemble is resonantly matched to an optical cavity mode frequency. Here, we lay the groundwork to study the behavior of polaritons in clean, isolated systems by…

Chemical Physics · Physics 2023-10-20 Adam D. Wright , Jane C. Nelson , Marissa L. Weichman

Two-dimensional infrared (2DIR) spectroscopy is widely used to study molecular dynamics but it is typically restricted to solid and liquid phase samples and modest spectral resolution. Only recently, its potential to study gas-phase…

Optics · Physics 2022-11-01 Grzegorz Kowzan , Thomas K. Allison