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Femtosecond laser ablation is a process that bears both fundamental physics interest and has wide industrial applications. For decades, the lack of probes on the relevant time and length scales has prevented access to the highly…

The use of strongly bent crystals in spectrometers for pulses of a hard x-ray free-electron laser is explored theoretically. Diffraction is calculated in both dynamical and kinematical theories. It is shown that diffraction can be treated…

Instrumentation and Detectors · Physics 2019-05-28 Vladimir Kaganer , Ilia Petrov , Liubov Samoylova

We present a model of x-ray thermal diffuse scattering (TDS) from a cubic polycrystal with an arbitrary crystallographic texture, based on the classic approach of Warren. We compare the predictions of our model with femtosecond x-ray…

Applied Physics · Physics 2025-08-07 P. G. Heighway , D. J. Peake , T. Stevens , J. S. Wark , B. Albertazzi , S. J. Ali , L. Antonelli , M. R. Armstrong , C. Baehtz , O. B. Ball , S. Banerjee , A. B. Belonoshko , C. A. Bolme , V. Bouffetier , R. Briggs , K. Buakor , T. Butcher , S. Di Dio Cafiso , V. Cerantola , J. Chantel , A. Di Cicco , A. L. Coleman , J. Collier , G. Collins , A. J. Comley , F. Coppari , T. E. Cowan , G. Cristoforetti , H. Cynn , A. Descamps , F. Dorchies , M. J. Duff , A. Dwivedi , C. Edwards , J. H. Eggert , D. Errandonea , G. Fiquet , E. Galtier , A. Laso Garcia , H. Ginestet , L. Gizzi , A. Gleason , S. Goede , J. M. Gonzalez , M. G. Gorman , M. Harmand , N. Hartley , C. Hernandez-Gomez , A. Higginbotham , H. Höppner , O. S. Humphries , R. J. Husband , T. M. Hutchinson , H. Hwang , D. A. Keen , J. Kim , P. Koester , Z. Konopkova , D. Kraus , A. Krygier , L. Labate , A. E. Lazicki , Y. Lee , H-P. Liermann , P. Mason , M. Masruri , B. Massani , E. E. McBride , C. McGuire , J. D. McHardy , D. McGonegle , R. S. McWilliams , S. Merkel , G. Morard , B. Nagler , M. Nakatsutsumi , K. Nguyen-Cong , A-M. Norton , I. I. Oleynik , C. Otzen , N. Ozaki , S. Pandolfi , A. Pelka , K. A. Pereira , J. P. Phillips , C. Prescher , T. Preston , L. Randolph , D. Ranjan , A. Ravasio , J. Rips , D. Santamaria-Perez , D. J. Savage , M. Schoelmerich , J-P. Schwinkendorf , S. Singh , J. Smith , R. F. Smith , A. Sollier , J. Spear , C. Spindloe , M. Stevenson , C. Strohm , T-A. Suer , M. Tang , M. Toncian , T. Toncian , S. J. Tracy , A. Trapananti , T. Tschentscher , M. Tyldesley , C. E. Vennari , T. Vinci , S. C. Vogel , T. J. Volz , J. Vorberger , J. T. Willman , L. Wollenweber , U. Zastrau , E. Brambrink , K. Appel , M. I. McMahon

A growing number of shock compression experiments, especially those involving laser compression, are taking advantage of in situ x-ray diffraction as a tool to interrogate structure and microstructure evolution. Although these experiments…

Time-resolved soft-x-ray-diffraction experiments give access to microscopic processes in a broad range of solid-state materials by probing ultrafast dynamics of ordering phenomena. While laboratory-based high-harmonic generation (HHG) light…

Ultrafast lattice deformation of tens to hundreds of nanometer thick metallic crystals, after femtosecond laser excitation, was measured directly using 8.04 keV subpicosecond x-ray and 59 keV femtosecond electron pulses. Coherent phonons…

Materials Science · Physics 2018-03-09 Runze Li , Kyle Sundqvist , Jie Chen , H. E. Elsayed-Ali , Peter M. Rentzepis

A new experimental setup combining X-Ray Photon Correlation Spectroscopy (XPCS) in the hard x-ray regime and a high-pressure sample environment is developed to monitor the pressure dependence of the internal motion of complex systems down…

Femtosecond, 8.04 KeV x-ray pulses are used to probe the lattice dynamics of 150 nm Cu (111) single crystal on mica substrate irradiated with 400 nm, 100 fs laser pulses. For pump fluencies below the damage and melting threshold, we…

Materials Science · Physics 2017-03-08 Runze Li , Omar A. Ashour , Jie Chen , H. E. Elsayed-Ali , Peter M. Rentzepis

In single particle coherent x-ray diffraction imaging experiments, performed at x-ray free-electron lasers (XFELs), samples are exposed to intense x-ray pulses to obtain single-shot diffraction patterns. The high intensity induces…

Atomic and Molecular Clusters · Physics 2013-01-29 U. Lorenz , N. M. Kabachnik , E. Weckert , I. A. Vartanyants

Scanning transmission electron microscopy (STEM) has advanced rapidly in the last decade thanks to the ability to correct the major aberrations of the probe forming lens. Now atomic-sized beams are routine, even at accelerating voltages as…

The multi-wavelength anomalous diffraction (MAD) method is used to determine phase information in x-ray crystallography by employing dispersion corrections from heavy atoms on coherent x-ray scattering. X-ray free-electron lasers (FELs)…

Atomic Physics · Physics 2011-11-18 Sang-Kil Son , Henry N. Chapman , Robin Santra

Knowledge of molecular structure is paramount in understanding, and ultimately influencing, chemical reactivity. For nearly a century, diffractive imaging has been used to identify the structures of many biologically-relevant gas-phase…

Chemical Physics · Physics 2020-03-09 Kasra Amini , Jens Biegert

Volume Free Electron Laser (VFEL) was proposed in [1-4]. It can operate in the wide spectral range from microwaves to X-rays. To simulate the processes which take place in VFEL the superradiance from a short electron pulse moving in a…

Optics · Physics 2016-09-08 Vladimir G. Baryshevsky , Konstantin G. Batrakov

The free-free opacity in plasmas is fundamental to our understanding of energy transport in stellar interiors and for inertial confinement fusion research. However, theoretical predictions in the challenging dense plasma regime are…

Silicon (Si) is one of the most abundant elements on Earth, and it is the most important and widely used semiconductor, constituting the basis of modern electronic devices. Despite extensive study, some properties of Si remain elusive. For…

The interaction of light with objects and media moving at relativistic and superluminal speeds enables unconventional phenomena such as Fresnel drag, Hawking radiation, and light amplification. Synthetic motion, facilitated by modulated…

Multi-technique high resolution X-ray mapping enhanced by the recent advent of 4th generation synchrotron facilities can produce colossal datasets, challenging traditional analysis methods. Such difficulty is clearly materialized when…

X-ray diffraction from molecules in the ground state produces an image of their charge density, and time-resolved X-ray diffraction can thus monitor the motion of the nuclei. However, the density change of excited valence electrons upon…

Chemical Physics · Physics 2018-06-15 Jérémy R. Rouxel , Markus Kowalewski , Kochise Bennett , Shaul Mukamel

We produce YbF molecules with a density of 10^18 m^-3 using laser ablation inside a cryogenically-cooled cell filled with a helium buffer gas. Using absorption imaging and absorption spectroscopy we study the formation, diffusion,…