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Related papers: Charge-state dependent vibrational relaxation in a…

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The dephasing time in coupled mesoscopic conductors is caused by the fluctuations of the dipolar charge permitted by the long range Coulomb interaction. We relate the phase breaking time to elementary transport coefficients which describe…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 Markus Buttiker , Andrew M. Martin

Ballistic transport occurs whenever electrons propagate without collisions deflecting their trajectory. It is normally observed in conductors with a negligible concentration of impurities, at low temperature, to avoid electron-phonon…

Mesoscale and Nanoscale Physics · Physics 2018-04-25 Youngwoo Nam , Dong-Keun Ki , David Soler-Delgado , Alberto F. Morpurgo

Non-equilibrium transport through a quantum dot with one spin-split single-particle level is studied in the cotunneling regime at low temperatures. The Coulomb diamond can be subdivided into parts differing in at least one of two respects:…

Mesoscale and Nanoscale Physics · Physics 2009-12-07 Daniel Becker , Daniela Pfannkuche

Quantum interference in nano-electronic devices could lead to reduced-energy computing and efficient thermoelectric energy harvesting. When devices are shrunk down to the molecular level it is still unclear to what extent electron…

Pristine monolayer graphene exhibits very poor screening because the density of states vanishes at the Dirac point. As a result, charge relaxation is controlled by the effects of zero-point motion (rather than by the Coulomb interaction)…

Mesoscale and Nanoscale Physics · Physics 2017-01-25 Eugene B. Kolomeisky , Joseph P. Straley

We analyze the interplay between vibrational and electronic degrees of freedom in charge transport across a molecular single-electron transistor. We focus on the wide class of molecules which possess quasi-degenerate vibrational…

Soft Condensed Matter · Physics 2007-05-23 Andrea Donarini , Milena Grifoni , Klaus Richter

We expand iterative numerically-exact influence functional path-integral tools and present a method capable of following the nonequilibrium time evolution of subsystems coupled to multiple bosonic and fermionic reservoirs simultaneously.…

Mesoscale and Nanoscale Physics · Physics 2015-06-15 Lena Simine , Dvira Segal

As a step towards a more realistic modeling of vibrations in single-molecule devices, we investigate the effects of charge-dependent vibrational frequencies and anharmonic potentials on electronic transport. For weak phonon relaxation, we…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Jens Koch , Felix von Oppen

Tunnel transport of interacting spin-polarized electrons through a single-level vibrating quantum dot in external magnetic field is studied. By using density matrix method, the current-voltage characteristics and the dependence of…

Mesoscale and Nanoscale Physics · Physics 2021-03-23 A. D. Shkop , O. M. Bahrova , S. I. Kulinich , I. V. Krive

Vibrationally inelastic electron transport through a flexible molecular junction is investigated. The study is based on a mechanistic model for a biphenyl molecule between two metal electrodes. Employing methods from electron-molecule…

Mesoscale and Nanoscale Physics · Physics 2023-07-26 Martin Cizek , Michael Thoss , Wolfgang Domcke

The role of the discontinuity of the exchange-correlation potential of density functional theory is studied in the context of electron transport and shown to be intimately related to Coulomb blockade. By following the time evolution of an…

Mesoscale and Nanoscale Physics · Physics 2010-06-08 S. Kurth , G. Stefanucci , E. Khosravi , C. Verdozzi , E. K. U. Gross

The realization of molecular-based electronic devices depends to a large extent on the ability to mechanically stabilize the involved molecular bonds, while making use of efficient resonant charge transport through the device. Resonant…

Mesoscale and Nanoscale Physics · Physics 2018-09-11 David Gelbwaser-Klimovsky , Alán Aspuru-Guzik , Michael Thoss , Uri Peskin

The characteristics of molecular electronic devices are critically determined by metal-organic interfaces, which influence the arrangement of the orbital levels that participate in charge transport. Studies on self-assembled monolayers…

We develop a theory of far from the equilibrium transport in arrays of tunnel junctions. We find that if the rate of the electron-electron interactions exceeds the rate of the electron-phonon energy exchange, the energy relaxation ensuring…

Mesoscale and Nanoscale Physics · Physics 2009-12-10 N. M. Chtchelkatchev , V. M. Vinokur , T. I. Baturina

We investigate ballistic vibrational energy transport through optical phonon band in oligomeric chains in the presence of decoherence. An exact solution is obtained for the excitation density in the space-time representation in the…

Chemical Physics · Physics 2015-05-20 Arkady A. Kurnosov , Igor V. Rubtsov , Alexander L. Burin

Due to the electron correlation, a fast removal of an electron from a molecule may create a coherent superposition of cationic states and in this way initiate pure electronic dynamics in which the hole-charge left by ionization migrates…

Chemical Physics · Physics 2023-04-03 J. Vester , V. Despré , A. I. Kuleff

Quantum transport through single molecules is very sensitive to the strength of the molecule-electrode contact. Here, we investigate the behavior of a model molecular junction weakly coupled to external electrodes in the case where charging…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Bo Song , Dmitry A. Ryndyk , Gianaurelio Cuniberti

The electronic bound states and resonances in the vicinity of the Dirac point energy due to the adsorption of calcium dimers on a suspended graphene monolayer are explored theoretically using density functional theory (DFT) and an improved…

Mesoscale and Nanoscale Physics · Physics 2015-06-23 Alireza Saffarzadeh , George Kirczenow

The rate-equation approach is used to describe sequential tunneling through a molecular junction in the Coulomb blockade regime. Such device is composed of molecular quantum dot (with discrete energy levels) coupled with two metallic…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Kamil Walczak

Transport through molecular devices with strong coupling to a single vibrational mode is considered in the case where the vibration is damped by coupling to the environment. We focus on the weak tunneling limit, for which a rate equation…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Stephan Braig , Karsten Flensberg