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We demonstrate the integration of a thin BaTiO$_3$ (BTO) membrane with monolayer MoSe$_2$ in a dual gate device that enables in-situ manipulation of the BTO ferroelectric polarization with a voltage pulse. While two-dimensional (2D)…

Semiconducting transition metal dichalcogenides (TMDs), such as MoSe$_2$ and WSe$_2$, exhibit unique optical and electronic properties. Vertical stacking of layers of one or more TMDs, to create heterostructures, has expanded the fields of…

In this paper we discuss the optical response due to the excitonic effect of two types of hBN bilayers: AB and AA'. Understanding the properties of these bilayers is of great utility to the study of twisted bilayers at arbitrary angles,…

Mesoscale and Nanoscale Physics · Physics 2022-03-21 J. C. G. Henriques , B. Amorim , R. M. Ribeiro , N. M. R. Peres

Using the tight-binding model, we report a gap opening in the energy spectrum of the twisted bilayer graphene under the application of pressure, that can be further amplified by the presence of a perpendicular bias voltage. The valley edges…

Mesoscale and Nanoscale Physics · Physics 2025-03-27 V. G. M. Duarte , D. R. da Costa , N. M. R. Peres , L. K. Teles , A. J. Chaves

We report resonant inelastic X-ray scattering (RIXS) measurements on the prototypical hexagonal boron nitride hBN layered compound. The RIXS results at the B and N K edges have been combined with electron energy loss spectroscopy (EELS)…

Previous calculations of the dielectric and optical properties of 2D materials often overlooked or circumvented the influence of vacuum spacing introduced in periodic calculations, which gave rise to mispredictions of the intrinsic…

Materials Science · Physics 2021-10-26 Guang Yang , Shang-Peng Gao

We calculate the binding energy, transition energies, oscillator strength, and absorption coefficient of indirect excitons in transition metal dichalcogenide (TMDC) double layers separated by an integer number of hexagonal boron nitride…

Mesoscale and Nanoscale Physics · Physics 2018-09-19 Matthew N. Brunetti , Oleg L. Berman , Roman Ya. Kezerashvili

Two-dimensional (2D) MXenes are a rapid growing family of 2D materials with rich physical and chemical properties where their surface termination plays an essential role. Among the various 2D MXenes, functionalization of the…

Materials Science · Physics 2022-09-22 Zafer Kandemir , Engin Torun , Fulvio Paleari , Celal Yelgel , Cem Sevik

Monolayer transition metal dichalcogenides host a variety of optically excited quasiparticles species that stem from two-dimensional confinement combined with relatively large carrier effective masses and reduced dielectric screening. The…

Symmetric electron-hole bilayer systems have been studied at zero temperature using the diffusion quantum Monte Carlo method. A flexible trial wave function is used that can describe fluid, excitonic and biexcitonic phases. We calculate…

Strongly Correlated Electrons · Physics 2013-09-10 Ryo Maezono , Pablo López Ríos , Tetsuo Ogawa , Richard J. Needs

Two-dimensional silicon carbide stands out among 2D materials, primarily due to its notable band gap, unlike its carbon-based counterparts. However, the binary nature and non-layered structure of bulk SiC present challenges in fabricating…

Materials Science · Physics 2024-11-26 Arushi Singh , Vikram Mahamiya , Alok Shukla

One of the most striking features of novel 2D semiconductors (e.g., transition metal dichalcogenide monolayers or phosphorene) is a strong Coulomb interaction between charge carriers resulting in large excitonic effects. In particular, this…

Mesoscale and Nanoscale Physics · Physics 2015-11-18 Kirill A. Velizhanin , Avadh Saxena

We investigate how external screening shapes excitons in two-dimensional (2d) semiconductors embedded in laterally structured dielectric environments. An atomic scale view of these elementary excitations is developed using models which…

We develop a systematic theory for excitons subject to Fermi-Hubbard physics in moir\'e twisted transition metal dichalcogenides (TMDs). Specifically, we consider excitons in moir\'e systems for which the valence band is in the…

Strongly Correlated Electrons · Physics 2023-06-07 T. -S. Huang , Yang-Zhi Chou , C. L. Baldwin , Fengcheng Wu , Mohammad Hafezi

We demonstrated the potential of the fractional dimensional approach to understand exciton parameters in the exemplary atomically thin semiconductor material, a monolayer of WS$_2$. This approach has proved to be successful in finding the…

Mesoscale and Nanoscale Physics · Physics 2024-03-19 Lakshminarayan Sharma , Carlos Rodriguez-Fernandez , Humeyra Caglayan

Monolayer transition metal dichalcogenide (TMDC) semiconductors exhibit strong excitonic optical resonances which serve as a microscopic, non-invasive probe into their fundamental properties. Like the hydrogen atom, such excitons can…

Metasurfaces enable flat optical elements by leveraging optical resonances in metallic or dielectric nanoparticles to obtain accurate control over the amplitude and phase of the scattered light. While highly efficient, these resonances are…

Optics · Physics 2022-09-07 Jason Lynch , Ludovica Guarneri , Deep Jariwala , Jorik van de Groep

Transient X-ray and extreme ultraviolet (XUV) spectroscopies have become invaluable tools for studying photoexcited dynamics due to their sensitivity to carrier occupations and local chemical or structural changes. One of the most studied…

Materials Science · Physics 2022-04-14 Isabel M. Klein , Hanzhe Liu , Danika Nimlos , Alex Krotz , Scott K. Cushing

Van der Waals heterostructures of two-dimensional transition metal dichalcogenides provide a unique platform to engineer optoelectronic devices tuning their optical properties via stacking, twisting, or straining. Using ab initio Many-Body…

Mesoscale and Nanoscale Physics · Physics 2025-03-21 R. Reho , A. R. Botello-Méndez , D. Sangalli , M. J. Verstraete , Zeila Zanolli

Ab initio electronic structure calculations of two-dimensional layered structures are typically performed using codes that were developed for three-dimensional structures, which are periodic in all three directions. The introduction of a…

Strongly Correlated Electrons · Physics 2016-06-22 Paolo E. Trevisanutto , Giovanni Vignale