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We investigate the spin-nonconserving relaxation channel of excitons by their couplings with phonons in two-dimensional transition metal dichalcogenides using $\textit{ab initio}$ approaches. Combining $\text{GW}$-Bethe-Salpeter equation…

Materials Science · Physics 2022-04-14 Xiaowei Zhang , Ting Cao

Hexagonal boron nitride (hBN) is a wide band gap material with both strong excitonic light emission in the ultraviolet and strong exciton-phonon coupling. Luminescence experiments performed on the recently synthesized monolayer form (m-hBN)…

Materials Science · Physics 2023-02-28 Pierre Lechifflart , Fulvio Paleari , Davide Sangalli , Claudio Attaccalite

Ab initio techniques for studying the optical and vibrational properties of materials are well-established, but only a few recent studies have focused on the interaction between excitons and atomic vibrations. In this paper, we revisit the…

Materials Science · Physics 2026-03-17 Rafael R. Del Grande , David A. Strubbe

Excitons are elementary optical excitation in semiconductors. The ability to manipulate and transport these quasiparticles would enable excitonic circuits and devices for quantum photonic technologies. Recently, interlayer excitons in 2D…

Mesoscale and Nanoscale Physics · Physics 2022-04-06 Ruoming Peng , Adina Ripin , Yusen Ye , Jiayi Zhu , Changming Wu , Seokhyeong Lee , Huan Li , Takashi Taniguchi , Kenji Watanabe , Ting Cao , Xiaodong Xu , Mo Li

We study the binding energies and optical properties of direct and indirect excitons in monolayers and double layer heterostructures of Xenes: silicene, germanene, and stanene. It is demonstrated that an external electric field can be used…

Mesoscale and Nanoscale Physics · Physics 2018-09-19 Matthew N Brunetti , Oleg L. Berman , Roman Ya. Kezerashvili

Time-dependent density functional theory (TDDFT) has been applied to the calculation of absorption spectra for two-dimensional atomic layer materials. We reveal that the character of the first bright exciton state of bi-layer hexagonal…

Materials Science · Physics 2020-01-08 Yasumitsu Suzuki , Kazuyuki Watanabe

Heterostructures made from 2D transition-metal dichalcogenides are known as ideal platforms to explore excitonic phenomena ranging from correlated moir\'e excitons to degenerate interlayer exciton ensembles. So far, it is assumed that the…

We introduce theoretical methods for describing the optical response of two-dimensional (2D) materials patterned at the nanoscale into both arrays of ribbons along a planar surface and spherical particles. Fourier-Floquet decompositions of…

Mesoscale and Nanoscale Physics · Physics 2025-12-16 Christian Nicolaisen Hansen , Line Jelver , Christos Tserkezis

Using an equation of motion (EOM) approach, we calculate excitonic properties of monolayer transition metal dichalcogenides (TMDs) perturbed by an external magnetic field. We compare our findings to the widely used Wannier model for…

Materials Science · Physics 2019-01-16 J. Have , G. Catarina , T. G. Pedersen , N. M. R. Peres

Twisted hexagonal boron nitride (thBN) exhibits emergent ferroelectricity due to the formation of moir\'e superlattices with alternating AB and BA domains. These domains possess electric dipoles, leading to a periodic electrostatic…

Recent theoretical and experimental studies suggest that van der Waals heterostructures with n- and p-doped bilayers of transition metal dichalcogenides are promising facilitators of exciton superfluidity. Exciton superfluidity in such…

Mesoscale and Nanoscale Physics · Physics 2023-08-10 Rune Højlund , Emil Grovn , Sahar Pakdel , Kristian S. Thygesen , Fredrik Nilsson

Recent measurements have shown that a continuously tunable bandgap of up to 250 meV can be generated in biased bilayer graphene [Y. Zhang et al., Nature 459, 820 (2009)], opening up pathway for possible graphene-based nanoelectronic and…

Materials Science · Physics 2010-02-11 Cheol-Hwan Park , Steven G. Louie

Metamaterial homogenization theories usually start with crude approximations that are valid in certain limits in zero order, such as small frequencies, wave vectors and material fill fractions. In some cases they remain surprisingly robust…

Optics · Physics 2022-01-25 Antonio Günzler , Cedric Schumacher , Matthias Saba

The excitonic spectra of single layer GeS and GeSe are predicted by ab initio GW-Bethe Salpeter equation calculations. G 0 W 0 calculations for the band structures find a fundamental band gap of 2.85 eV for GeS and 1.70 eV for GeSe…

Mesoscale and Nanoscale Physics · Physics 2016-10-26 Lidia C. Gomes , P. E. Trevisanutto , A. Carvalho , A. S. Rodin , A. H. Castro Neto

Heterostructures of layered transition metal dichalcogenides (TMDs) host long-lived, tunable excitons, making them intriguing candidates for material-based quantum information applications. Light absorption in these systems induces a…

Materials Science · Physics 2023-08-25 Tomer Amit , Sivan Refaely-Abramson

The properties of excitons, or correlated electron-hole pairs, are of paramount importance to optoelectronic applications of materials. A central component of exciton physics is the electron-hole interaction, which is commonly treated as…

Transition-metal dichalcogenide heterostructures exhibit moir\'e patterns that spatially modulate the electronic structure across the material's plane. For certain material pairs, this modulation acts as a potential landscape with deep,…

Mesoscale and Nanoscale Physics · Physics 2021-03-12 David A. Ruiz-Tijerina , Isaac Soltero , Francisco Mireles

We present a hybrid approach for GW/Bethe-Salpeter Equation (BSE) calculations of core excitation spectra, including x-ray absorption (XAS), electron energy loss spectra (EELS), and non-resonant inelastic x-ray scattering (NRIXS). The…

Materials Science · Physics 2015-05-20 J. Vinson , E. L. Shirley , J. J. Rehr , J. J. Kas

Biased bilayer graphene (BBG) is a variable band gap semiconductor, with a strongly field-dependent band gap of up to $300 \, \text{meV}$, making it of particular interest for graphene-based nano-electronic and -photonic devices. The…

Mesoscale and Nanoscale Physics · Physics 2022-03-21 Mikkel Ohm Sauer , Thomas Garm Pedersen

The electronic band structure of V$_2$O$_5$ is calculated using an all-electron quasiparticle self-consistent (QS) $GW$ method, including electron-hole ladder diagrams in the screening of $W$. The optical dielectric function calculated with…

Materials Science · Physics 2024-07-31 Claudio Garcia , Santosh Kumar Radha , Swagata Acharya , Walter R. L. Lambrecht
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