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We assess proposals for entangling two distant atoms by measurement of emitted photons, analyzing how their performance depends on the photon detection efficiency. We consider schemes based on measurement of one or two photons and compare…

We image with cameras entangled photon light transmitted through a random medium. Near-field and far-field spatial quantum correlations show that entangled photon pairs (bi-photons) generated by spontaneous optical parametric…

Quantum Physics · Physics 2019-07-09 Soro Gnatiessoro , Alexis Mosset , Eric Lantz , Fabrice Devaux

Entangled photons can be used to make measurements with an accuracy beyond that possible with classical light. While most implementations of quantum metrology have used states made up of a single colour of photons, we show that entangled…

In molecular aggregates, multiple delocalized exciton states interact with phonons, making the state-resolved spectroscopic monitoring of dynamics challenging. We propose a protocol that combines photon-entanglement-enhanced narrowband…

Quantum Physics · Physics 2026-04-24 Arunangshu Debnath , Shaul Mukamel

Quantum light is increasingly recognized as a promising resource for developing optical measurement techniques. Particular attention has been paid to enhancing the precision of the measurements beyond classical techniques by using…

Chemical Physics · Physics 2023-10-03 Yuta Fujihashi , Kuniyuki Miwa , Masahiro Higashi , Akihito Ishizaki

A quantum system composed of two or more subsystems can be in an entangled state, i.e. a state in which the properties of the global system are well defined but the properties of each subsystem are not. Entanglement is at the heart of…

In this contribution we analyze virtual-state spectroscopy --- a unique tool for extracting information about the virtual states that contribute to the two-photon excitation of an absorbing medium --- as implemented by means of intense…

Quantum Physics · Physics 2018-03-14 Jiří Svozilík , Jan Peřina , Roberto de J. León-Montiel

Entanglement is a fundamental feature of quantum mechanics, considered a key resource in quantum information processing. Measuring entanglement is an essential step in a wide range of applied and foundational quantum experiments. When a…

Entangling independent photons is not only of fundamental interest but also of crucial importance for quantum information science. Two-photon interference is a major method to entangle independent identical photons. If two photons are…

Quantum Physics · Physics 2015-01-27 Tian-Ming Zhao , Han Zhang , Jian Yang , Zi-Ru Sang , Xiao Jiang , Xiao-Hui Bao , Jian-Wei Pan

High-dimensional entanglement in the form of transverse spatial correlation between a pair of photons generated via spontaneous parametric downconversion is not only a valuable resource in many academic and real-life applications but also…

Quantum Physics · Physics 2025-08-18 Rounak Chatterjee , Vikas S Bhat , Kiran Bajar , Sushil Mujumdar

We demonstrate the control of entanglement of a single photon between several spatial modes propagating through a strongly scattering medium. Measurement of the scattering matrix allows the wavefront of the photon to be shaped to compensate…

We consider a photonic crystal (PC) doped with four-level atoms whose intermediate transition is coupled near-resonantly with a photonic band-gap edge. We show that two photons, each coupled to a different atomic transition in such atoms,…

Quantum Physics · Physics 2009-11-06 David Petrosyan , Gershon Kurizki

Entangled two-photon absorption can enable a linear scaling of fluorescence emission with the excitation power. In comparison to classical two-photon absorption with a quadratic scaling, this can allow fluorescence imaging or…

Hyperentangled photonic states - exhibiting nonclassical correlations in several degrees of freedom - offer improved performance of quantum optical communication and computation schemes. Experimentally, a hyperentanglement of…

Quantum Physics · Physics 2021-06-21 Michał Lipka , Michał Parniak

Recent theoretical studies in quantum spectroscopy have emphasized the potential of non-classical correlations in entangled photon pairs for selectively targeting specific nonlinear optical processes in nonlinear optical responses. However,…

Chemical Physics · Physics 2026-04-21 Yuta Fujihashi , Ozora Iso , Ryosuke Shimizu , Akihito Ishizaki

It has been proposed that entangled two-photon absorption (E2PA) can be observed with up to 10 orders of magnitude lower photon flux than its classical counterpart. However, there is a significant controversy regarding the magnitude of this…

Ultrafast optical spectroscopy is a powerful technique for studying the dynamic processes of molecular systems in condensed phases. However, in molecular systems containing many dye molecules, the spectra can become crowded and difficult to…

Chemical Physics · Physics 2025-02-05 Yuta Fujihashi , Akihito Ishizaki , Ryosuke Shimizu

We study in this paper the efficiency of different two-photon states of light to induce the simultaneous excitation of two atoms of different kinds when the sum of the energies of the two photons matches the sum of the energies of the two…

Quantum Physics · Physics 2013-03-21 Zhan Zheng , Pablo L. Saldanha , Jose R. Rios Leite , Claude Fabre

Quantum entanglement has emerged as a great resource for interactions between molecules and radiation. We propose a new paradigm of stimulated Raman scattering with entangled photons. A quantum ultrafast Raman spectroscopy is developed for…

Quantum Physics · Physics 2023-05-26 Joel Jiahao Fan , Zhe-Yu Jeff Ou , Zhedong Zhang

It has been discussed recently how quantum illumination can be used to increase the accuracy of the value range-delay measurement \cite{Zhuang Shapiro 2022} in the domain of SNR compatible with current radar systems. However, the advantage…

Quantum Physics · Physics 2023-05-10 Ricardo Gallego Torromé