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Resonant soft X-ray Raman scattering measurements on NiO have been made at photon energies across the Ni 2p absorption edges. The details of the spectral features are identified as Raman scattering due to d-d and charge-transfer…

Materials Science · Physics 2012-01-04 M. Magnuson , S. M. Butorin , A. Agui , J. Nordgren

We develop a formalism to calculate the L-edge resonant x-ray scattering (RIXS) spectra from transition-metal compounds. Using a multi-orbital tight-binding model, we derive useful formulas to calculate the spectra by collecting up the…

Strongly Correlated Electrons · Physics 2015-06-16 Jun-ichi Igarashi , Tatsuya Nagao

The magnetic properties of rare earth compounds are usually well captured by assuming a fully localized f shell and only considering the Hund's rule ground state multiplet split by a crystal electrical field (CEF). Currently, the standard…

Strongly Correlated Electrons · Physics 2018-07-06 A. Amorese , N. Caroca-Canales , S. Seiro , C. Krellner , G. Ghiringhelli , N. B. Brookes , D. V. Vyalikh , C. Geibel , K. Kummer

We develop a formalism for calculating resonant inelastic x-ray scattering (RIXS) spectra in systems of itinerant electrons with arbitrary band structures, accounting for the effect of the positively-charged core hole exactly. We apply this…

Superconductivity · Physics 2013-12-24 David Benjamin , Israel Klich , Eugene Demler

Resonant Inelastic X-Ray Scattering (RIXS) is a well-established tool for probing excitations in a wide range of materials. The measured spectra strongly depend on the scattering geometry, via its influence on the polarization of the…

Strongly Correlated Electrons · Physics 2026-05-18 Michelangelo Tagliavini , Fabian Wenzel , Maurits W. Haverkort

We analyze resonant inelastic x-ray scattering (RIXS) at the Cu K edge in a typical orbital-ordered compound KCuF3 on the basis of a microscopic theory. Spectral shape and its dependence on polarization direction and momentum transfer of…

Strongly Correlated Electrons · Physics 2014-06-20 Takuji Nomura

The capability to probe the dispersion of elementary spin, charge, orbital, and lattice excitations has positioned resonant inelastic x-ray scattering (RIXS) at the forefront of photon science. Here we develop the scattering theory for RIXS…

Superconductivity · Physics 2015-04-10 Pasquale Marra , Steffen Sykora , Krzysztof Wohlfeld , Jeroen van den Brink

We study resonant x-ray scattering (RXS) at Np M_{4,5} edges in the triple-\textbf{k} multipole ordering phase in NpO_{2}, on the basis of a localized electron model. We derive an expression for RXS amplitudes to characterize the spectra…

Strongly Correlated Electrons · Physics 2015-06-25 Tatsuya Nagao , Jun-ichi Igarashi

Young's archetypal double-slit experiment forms the basis for modern diffraction techniques: the elastic scattering of waves yields an interference pattern that captures the real-space structure. Here, we report on an inelastic incarnation…

We present a relativistic time-dependent density functional theory (TDDFT) approach for the simulation of resonant inelastic X-ray scattering (RIXS) spectra, based on both a full four-component (4c) Dirac-Coulomb Hamiltonian and a modern…

Chemical Physics · Physics 2026-04-17 Lukas Konecny , Muhammed A. Dada , Daniel R. Nascimento , Michal Repisky

Low-energy electron excitation spectra were measured on a single crystal of a typical iron-based superconductor PrFeAsO$_{0.7}$ using resonant inelastic X-ray scattering (RIXS) at the Fe-$L_3$ edge. Characteristic RIXS features are clearly…

Strongly Correlated Electrons · Physics 2016-07-18 T. Nomura , Y. Harada , H. Niwa , K. Ishii , M. Ishikado , S. Shamoto , I. Jarrige

We present two different theories for Raman scattering and Resonant Inelastic X-ray Scattering (RIXS) in the low temperature ferromagnetic phase of YTiO$_3$ and compare this to the available experimental data. For description of the orbital…

Strongly Correlated Electrons · Physics 2010-03-30 L. J. P. Ament , G. Khaliullin

We theoretically analyze the intensity of the resonant inelastic X-ray scattering (RIXS) based on Ansatz that the electron is fractionalized into two components. By fitting the angle resolved photoemission spectroscopy (ARPES) data of a…

Strongly Correlated Electrons · Physics 2021-07-26 Masatoshi Imada

We have investigated the electronic structure of Sr2IrO4 within the density-functional theory using the generalized gradient approximation while taking into account strong Coulomb correlations in the framework of the fully relativistic…

Strongly Correlated Electrons · Physics 2023-10-13 V. N. Antonov , D. A. Kukusta , L. V. Bekenov

We analyze the resonant inelastic x-ray scattering (RIXS) spectra at the Ni $K$ edge in an antiferromagnetic insulator NiO by applying the theory developed by the present authors. It is based on the Keldysh Green's function formalism, and…

Strongly Correlated Electrons · Physics 2009-11-11 Manabu Takahashi , Jun-ichi Igarashi , Takuji Nomura

We study the magnetic excitation spectra of Cu L_{2,3}-edge resonant inelastic x-ray scattering (RIXS) from the spin-liquid ground state in two-leg spin ladder cuprates. Applying the projection method developed by the present authors, we…

Strongly Correlated Electrons · Physics 2015-06-05 Tatsuya Nagao , Jun-ichi Igarashi

This paper presents a simple formalism for calculating X-ray absorption (XAS) and resonant inelastic x-ray scattering (RIXS) that has as input orbital-resolved density of states from a single-particle or many-body \textit{ab initio}…

Strongly Correlated Electrons · Physics 2023-04-18 M. R. Norman , A. S. Botana , J. Karp , A. Hampel , H. LaBollita , A. J. Millis , G. Fabbris , Y. Shen , M. P. M. Dean

This paper provides a brief overview of applications of advanced X-ray spectroscopic techniques that take advantage of the resonant inelastic X-ray scattering (RIXS) in the hard and tender x-ray range and have recently become available for…

Materials Science · Physics 2014-01-08 K. O. Kvashnina , S. M. Butorin

We present a novel derivation of resonant inelastic x-ray scattering (RIXS) which yields an expression for the RIXS cross section in terms of emission pathways between intermediate and final many-body states. Thereby electron-hole…

Materials Science · Physics 2020-10-14 Christian Vorwerk , Francesco Sottile , Claudia Draxl

We report resonant inelastic x-ray scattering (RIXS) excited by circularly polarized x-rays on Mn-Zn ferrite at the Mn L2,3-resonances. We demonstrate that crystal field excitations, as expected for localized systems, dominate the RIXS…

Materials Science · Physics 2012-01-04 M. Magnuson , L. -C. Duda , S. M. Butorin , P. Kuiper , J. Nordgren