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Second harmonic generation (SHG) is a fundamental nonlinear optical phenomenon widely used both for experimental probes of materials and for application to optical devices. Even-order nonlinear optical responses including SHG generally…

Mesoscale and Nanoscale Physics · Physics 2021-10-13 Kazuaki Takasan , Takahiro Morimoto , Joseph Orenstein , Joel E. Moore

The topological Weyl semimetals with peculiar band structure exhibit novel nonlinear optical enhancement phenomena even for light at optical wavelengths. While many intriguing nonlinear optical effects were constantly uncovered in type-I…

While all media can exhibit first-order conductivity describing current linearly proportional to electric field, $E$, the second-order conductivity, $\sigma^{(2)}$ , relating current to $E^2$, is nonzero only when inversion symmetry is…

Second harmonic generation (SHG) is a nonlinear optical response arising exclusively from broken inversion symmetry in the electric-dipole limit. Recently, SHG has attracted widespread interest as a versatile and noninvasive tool for…

We study nonlinear optical responses in superconducting systems with inversion ($\mathcal{I}$) symmetry-breaking order parameters. We first show that any superconducting system with $\mathcal{I}$ and time-reversal ($\mathcal{T}$) symmetries…

Superconductivity · Physics 2019-12-11 Tianrui Xu , Takahiro Morimoto , Joel E. Moore

Broken symmetries and electronic topology are nicely manifested together in the second order nonlinear optical responses from topologically nontrivial materials. While second order nonlinear optical effects from the electric dipole (ED)…

Materials Science · Physics 2023-10-25 Youngjun Ahn , Xiaoyu Guo , Rui Xue , Kejian Qu , Kai Sun , David Mandrus , Liuyan Zhao

Second-harmonic generation (SHG) is a well-known nonlinear spectroscopy method to probe electronic structure, specifically, in transition metal dichalcogenide (TMDC) monolayers. This work investigates the nonlinear dynamics of a strongly…

We develop a multipolar theory of second-harmonic generation (SHG) by dielectric nanoparticles made of noncentrosymmetric materials with bulk quadratic nonlinearity. We specifically analyze two regimes of optical excitation: illumination by…

Second-harmonic generation (SHG) is a direct measure of the strength of second-order nonlinear optical effects, which also include frequency mixing and parametric oscillations. Natural and artificial materials with broken…

We report about the experimental observation and characterization of nonlinear optical properties of individual silicon nanowires of different dimensions. Our results show that the nonlinear light has different components, one of them…

Mesoscale and Nanoscale Physics · Physics 2017-04-13 Peter R. Wiecha , Arnaud Arbouet , Houssem Kallel , Priyanka Periwal , Thierry Baron , Vincent Paillard

Second harmonic generation (SHG), as one of the most significant \c{hi}(2) nonlinear optical processes, plays crucial roles in a broad variety of optical and photonic applications. Designing various delicate schemes to achieve highly…

Optics · Physics 2021-09-01 Lei Wang , XiuQuan Zhang , Feng Chen

The second-order nonlinear optical (NLO) processes, such as the photogalvanic effect and second-order harmonic generation (SHG), play crucial roles in probing and controlling light-matter interactions for energy and device applications. To…

Materials Science · Physics 2020-08-05 Ruixiang Fei , Wenshen Song , Li Yang

Diode effects are of great interest for both fundamental physics and modern technologies. Electrical diode effects (nonreciprocal transport) have been observed in Weyl systems. Optical diode effects arising from the Weyl fermions have been…

Intense laser-driven nonlinear optical phenomena in two-dimensional (2D) nodal-line semimetals (NLS) exhibit complex mechanisms, particularly in the NbSi$_{x}$Te$_{2}$ material systems characterized by nonsymmorphic symmetry-protected band…

Optics · Physics 2025-08-25 Navdeep Rana , M. S. Mrudul , Amar Bharti , Sucharita Giri , Gopal Dixit

This research will examine the computational methods to calculate the nonlinear optical process of second harmonic generation (SHG) that will be hypothesized to be present during lithium ion insertion into silicon nanowires. First it will…

Optics · Physics 2021-10-19 Donald C. Boone

Nonreciprocal devices that allow the light propagation in only one direction are indispensable in photonic circuits and emerging quantum technologies. Contemporary optical isolators and circulators, however, require large size or strong…

Materials Science · Physics 2021-10-12 Shingo Toyoda , Manfred Fiebig , Taka-hisa Arima , Yoshinori Tokura , Naoki Ogawa

Recent experiments and calculations in topological semimetals have observed anomalously strong second-order optical nonlinearity, but yet whether the enhancement also occurs at surfaces of topological semimetals in general remains an open…

A new concept for second-harmonic generation (SHG) in an optical nanocircuit is proposed. We demonstrate both theoretically and experimentally that the symmetry of an optical mode alone is sufficient to allow SHG even in centro-symmetric…

The response functions of a material characterize its behavior under external stimuli, such as electromagnetic radiation. Such responses may grow linearly with the amplitude of the incident radiation, as is the case of absorption, or may be…

Mesoscale and Nanoscale Physics · Physics 2019-08-07 Liang Z. Tan , Andrew M. Rappe

Weyl semimetals (WSM) have been discovered in time-reversal symmetric materials, featuring monopoles of Berry's curvature in momentum space. WSM have been distinguished between Type-I and II where the velocity tilting of the cone in the…

Mesoscale and Nanoscale Physics · Physics 2018-01-19 Xu Yang , Kenneth Burch , Ying Ran
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