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The breakdown of the quasiparticle approximation (QPA) for phonons in strongly anharmonic materials necessitates advanced first-principles frameworks for accurate lattice dynamics and thermal transport predictions. We develop a…

Materials Science · Physics 2025-12-23 Yi Xia

Crystalline solids are generally known as excellent heat conductors, amorphous materials or glasses as thermal insulators. It has thus come as a surprise that certain crystal structures defy this paradigm. A prominent example are type-I…

Strongly Correlated Electrons · Physics 2019-02-22 M. Ikeda , H. Euchner , X. Yan , P. Tomes , A. Prokofiev , L. Prochaska , G. Lientschnig , R. Svagera , S. Hartmann , E. Gati , M. Lang , S. Paschen

We describe a theoretical and computational approach to calculate the vibrational, elastic, and thermal properties of materials from the low-temperature quantum regime to the high-temperature anharmonic regime. This approach is based on…

Materials Science · Physics 2024-09-20 Dylan A. Folkner , Zekun Chen , Giuseppe Barbalinardo , Florian Knoop , Davide Donadio

The thermal transport properties of single-wall carbon nanotubes (SWCNTs) are re-investigated using the iterative solution of the Boltzmann transport equation by including four-phonon scattering. Using only three-phonon scattering, the…

Materials Science · Physics 2023-11-07 Ankit Jain

Ordered crystalline compounds exhibiting ultralow and glass-like thermal conductivity are both fundamentally and technologically important, where phonon quasi-particles dominate their heat transport. Understanding the microscopic mechanisms…

Materials Science · Physics 2025-09-04 Shantanu Semwal , Yi Xia , Chris Wolverton , Koushik Pal

Within the framework of the unified theory thermal transport model, the competing contributions of coherent and incoherent terms create a trade-off relationship, posing substantial challenges to achieving a reduction in overall $\rm…

Materials Science · Physics 2025-04-04 Wenjie Xiong , Hao Huang , Yu Wu , Xinji Xu , Geng Li , Zonglin Gu , Shuming Zeng

We propose a method to engineer the phonon thermal transport properties of low dimensional systems. The method relies on introducing a predetermined combination of molecular adsorbates, which give rise to antiresonances at frequencies…

Mesoscale and Nanoscale Physics · Physics 2018-10-02 Koray Sevim , Hâldun Sevinçli

We have carried out temperature-dependent x-ray diffraction and Raman scattering experiments on powder $Cs_3Bi_2Br_9$. Trigonal to monoclinic structural transition at around 95 K is discussed and shown to be driven by the softening of the…

Third order anharmonic scattering in light-matter systems can drive a wide variety of practical and physically interesting processes from lasing to polariton condensation. Motivated by recent experimental results in the nonlinear optics of…

Mesoscale and Nanoscale Physics · Physics 2017-11-06 Christopher R. Gubbin , Simone De Liberato

We present here a theoretical method to determine the phononic contribution to the thermal conductance of nanoscale systems in the phase-coherent regime. Our approach makes use of classical molecular dynamics (MD) simulations to calculate…

Mesoscale and Nanoscale Physics · Physics 2022-11-09 Fabian Müller , Peter Nielaba , Juan Carlos Cuevas , Fabian Pauly

The van der Waals (vdW) interactions exist in reality universally and play an important role in physics. Here, we show the study on the mechanism of vdW interactions on phonon transport in atomic scale, which would boost developments in…

Mesoscale and Nanoscale Physics · Physics 2021-01-13 Xiaoxiang Yu , Dengke Ma , Chengcheng Deng , Xiao Wan , Meng An , Han Meng , Xiaobo Li , Xiaoming Huang , Nuo Yang

Interface impedes heat flow in heterostructures and the interfacial thermal resistance (ITR) has become a critical issue for thermal dissipation in electronic devices. To explore the mechanism leading to the ITR, in this work, the dynamic…

Applied Physics · Physics 2023-06-28 Quanjie Wang , Jie Zhang , Vladimir Chernysh , Xiangjun Liu

In this paper, we provide an analytical study of the transmission eigenvalue problem in the context of biharmonic scattering with a penetrable obstacle. We will assume that the underlying physical model is given by an infinite elastic…

Analysis of PDEs · Mathematics 2025-10-10 Rafael Ceja Ayala , Isaac Harris , Andreas Kleefeld

We report a Raman study of the effect of temperature on the self-energies of optical phonons in a number of transition metals with hexagonal-close-packed structure. Anisotropic softening of phonon energies and narrowing of phonon linewidths…

Materials Science · Physics 2017-01-04 Yu. S. Ponosov , S. V. Streltsov

The anharmonicity of the acoustic phonon dispersion of graphene has been studied by the harmonic linear response (HLR) approach at finite temperature. This is a non-perturbative method based on the linear response of the system to applied…

Materials Science · Physics 2020-08-20 R. Ramirez , C. P. Herrero

In this work, using the scattering matrix method, we have investigated the transmission coefficients and the thermal conductivity in a double-bend waveguide structure. The transmission coefficients show strong resonances due to the…

Mesoscale and Nanoscale Physics · Physics 2007-10-05 Yi Ming , Zhexian Wang , Zejun Ding

The temperature dependence of the phonon spectrum in the superconducting transition metal dichalcogenide 2H-NbS$_2$ is measured by diffuse and inelastic x-ray scattering. A deep, wide and strongly temperature dependent softening, of the two…

Knowledge of lattice anharmonicity is essential to elucidate distinctive thermal properties in crystalline solids. Yet, accurate \textit{ab initio} investigations of lattice anharmonicity encounter difficulties owing to the cumbersome…

Materials Science · Physics 2022-04-13 Zhen Zhang , Dong-Bo Zhang , Tao Sun , Renata M. Wentzcovitch

The problem of phonon scattering by grain boundaries is studied within the wedge disclination dipole (WDD) model. It is shown that a specific q-dependence of the phonon mean free path for biaxial WDD results in a low-temperature crossover…

Materials Science · Physics 2009-10-31 V. A. Osipov , S. E. Krasavin

We study thermal transport in a chain of coupled atoms, which can vibrate in longitudinal as well as transverse directions. The particles interact through anharmonic potentials upto cubic order. The problem is treated quantum mechanically.…

Statistical Mechanics · Physics 2010-04-19 Santhosh G , Deepak Kumar