Related papers: Self-Kerr effect across the yellow $\mathrm{Cu_2O}…
The nonlinear response of materials, an increasingly important aspect of light-matter interaction, can be challenging to measure in highly absorbing materials. Here, we introduce an interferometric technique that enables a direct…
We have experimentally determined the energies of the ground and first four excited excitonic states of the fundamental optical transition in monolayer WS2, a model system for the growing class of atomically thin two-dimensional…
Resonance fluorescence spectra of a driven Kerr nonlinear resonator is investigated both theoretically and experimentally. When the Kerr nonlinear resonator is driven strongly such that the induced Rabi frequency is comparable to or larger…
Recent experiments show that optically generated Rydberg excitons in cuprous oxide can neutralize charged impurities, strongly reducing stray electric fields and effectively purifying the crystal. Here, we develop a multichannel theory of…
We study coherent backscattering of a quasi-monochromatic laser by a dilute gas of cold two-level atoms. We consider the perturbative regime of weak intensities, where nonlinear effects arise from {\em inelastic} two-photon scattering…
We report the first unambiguous observational evidence of Rydberg Enhanced Recombination (RER), a potentially important recombination mechanism that has hitherto been unexplored in low-temperature photoionized plasmas. RER shares…
We present a novel spectroscopic method for probing the \insitu~density of quantum gases. We exploit the density-dependent energy shift of highly excited {Rydberg} states, which is of the order $10$\MHz\,/\,1E14\,cm$^{\text{-3}}$ for…
We report a novel experimental technique to investigate ultrafast dynamics in photoexcited molecules by probing the third-order nonlinear optical susceptibility. A non-colinear 3-pulse scheme is developed to probe the ultrafast dynamics of…
In this paper, we report on numerical calculations of the spontaneous emission rates and Lamb shifts of a $^{87}\text{Rb}$ atom in a Rydberg-excited state $\left(n\leq30\right)$ located close to a silica optical nanofiber. We investigate…
The nonlinear optical response of an excitonic insulator coupled to lattice degrees of freedom is shown to depend in strong and characteristic ways on whether the insulating behavior originates primarily from electron-electron or…
The dynamics of the modulation instability induced by cross phase modulation is studied by considering the influence of the walk-off and noninstantaneous response effects for two copropagating optical fields travelling in the anomalous…
A resonant inelastic x-ray scattering study of the electronic structure of the semiconductor cuprous oxide, $\rm Cu_2O$, is reported. When the incident x-ray energy is tuned to the Cu K-absorption edge, large enhancements of the spectral…
We investigate the interaction between highly excited Rydberg excitons and charged impurities in the semiconductor Cuprous Oxide. We find that it is long-ranged and based on charge-induced dipole interactions. We demonstrate that we can…
Nonlinear optical (NLO) phenomena such as harmonic generation, Kerr, and Pockels effects are of great technological importance for lasers, frequency converters, modulators, switches, etc. Recently, two-dimensional (2D) materials have drawn…
We report the experimental observation of strong two-color optical nonlinearity in an ultracold gas of $^{85}\mathrm{Rb}$-$^{87}\mathrm{Rb}$ atom mixture. By simultaneously coupling two probe transitions of $^{85}$Rb and $^{87}$Rb atoms to…
We demonstrate the interaction-induced blockade effect in an ultracold $^{88}$Sr gas via studying the time dynamics of a two-photon excitation to the triplet Rydberg series $5\mathrm{s}n\mathrm{s}\, ^3\textrm{S}_1$ for five different…
In the regime of Rydberg electromagnetically induced transparency, we study the correlated behaviors between the transmission spectra of a pair of probe fields passing through respective parallel one-dimensional cold Rydberg ensembles. Due…
We analyze the Hall conductivity $\sigma_{xy}(\omega)$ of a charge ordered state with momentum $\mathbf{Q}=(0,2Q)$ and calculate the intrinsic contribution to the Kerr angle $\Theta_K$ using the fully reconstructed tight-binding band…
Dispersive shock waves (DSWs) are fascinating wave phenomena occurring in media when nonlinearity overwhelms dispersion (or diffraction). Creating DSWs with low generation power and realizing their active controls is desirable but remains a…
Controlling nonequilibrium responses in optically driven quantum materials is essential for advancing applications in energy conversion, ultrafast electronics, and quantum computation. Nonlinear optical spectroscopy serves as a powerful…