Related papers: Self-Kerr effect across the yellow $\mathrm{Cu_2O}…
We show how to compute the nonlinear optical functions (absorption, reflection, and transmission) for a medium with Rydberg excitons, including the effect of the coherence between the electron-hole pair and the electromagnetic field. Using…
We investigate the nonlinear refraction and the nonlinear Kerr phase shift which are due to Rydberg excitons induced in Cu2O crystal by short-time pulses. We observe the phenomenon of quantum beats, analogous to that observed in exciton…
The quantum confiment of Rydberg excitons (REs) in quantum structures opens the way towards considering nonlinear interactions in such systems. We present a theoretical calculation of optical functions in the case of a nonlinear coupling…
Rydberg excitons (analogues of Rydberg atoms in condensed matter systems) are highly excited bound electron-hole states with large Bohr radii. The interaction between them as well as exciton coupling to light may lead to strong optical…
Microwave-optical conversion is key to future networks of quantum devices, such as those based on superconducting technology. Conversion at the single quantum level requires strong nonlinearity, high bandwidth, and compatibility with a…
We theoretically investigate the nonlinear optical transmission through a cuprous oxide crystal for wavelengths that cover the series of highly excited excitons, observed in recent experiments. Since such Rydberg excitons have strong van…
Hosting giant Rydberg excitons with principal quantum numbers up to n = 30, cuprous oxide (Cu2O) provides a rare solid-state setting for exploring Rydberg physics, as exemplified by the blockade effect. Here we access the strongly…
Cuprous oxide (Cu${}_2$O) has recently been proposed as a promising solid-state host for excitonic Rydberg states with large principal quantum numbers ($n$), whose exaggerated wavefunction sizes ($\propto n^2)$ facilitate gigantic…
We investigate the Kerr and magneto-optical effects for a probe laser field with two orthogonally polarized components, propagating in a cold Rydberg atomic gas with an inverted-Y-type level configuration via double electromagnetically…
We use two-color pump-probe spectroscopy to study Rydberg excitons in Cu$_2$O in the presence of free carriers injected by above-band-gap excitation. Already at plasma densities $\rho_\text{eh}$ below one hundredth electron-hole pair per…
We report the experimental observation of a cross-Kerr nonlinearity in a free-space medium based on resonantly-excited, interacting Rydberg atoms and electromagnetically induced transparency. The nonlinearity is used to implement…
We study the ultrastrong driving of Rydberg excitons in Cu$_2$O by a microwave field. The effect of the field is studied using optical absorption spectroscopy, and through the observation of sidebands on the transmitted laser light. A model…
The recent observation of high-lying Rydberg states of excitons in semiconductors with relatively high binding energy motivates exploring their applications in quantum nonlinear optics and quantum information processing. Here, we study…
Rydberg states of excitons can reach microns in size and require extremely pure crystals. We introduce an experimental method for the rapid and spatially-resolved characterization of Rydberg excitons in copper oxide (Cu2O) with sub-micron…
The quantum confinement of Rydberg excitons is an important step towards exploiting their large nonlinearities for quantum applications. We observe Rydberg excitons in natural nanoparticles of Cu$_2$O. We resolve up to the principal quantum…
Rydberg excitons in Cu2O can be an emergent platform for solid-state quantum information processing by utilizing the exaggerated properties of high-lying excited states within the material. To develop practical quantum systems,…
The excitation dynamics of a laser-driven Rydberg gas exhibits a cooperative effect due to the interatomic Rydberg-Rydberg interaction, but the large many-body system with inhomogeneous Rydberg coupling is hard to exactly solved or…
Rydberg excitons in the semiconductor Cu$_2$O have been observed in absorption experiments up to a principal quantum number of n = 28 at millikelvin temperatures [1]. Here, we extend the experimental parameter space by variing both…
High-power optical pulses experience self-focusing when propagating in a gaseous medium due to the manifestation of the cubic (Kerr-like) nonlinearity. The magnitude of this effect depends on the Kerr nonlinearity coefficient n2, which in…
Rydberg excitons are, with their ultrastrong mutual interactions, giant optical nonlinearities, and very high sensitivity to external fields, promising for applications in quantum sensing and nonlinear optics at the single-photon level. To…