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A quantum spin liquid (QSL) arises from a highly entangled superposition of many degenerate classical ground states in a frustrated magnet, and is characterized by emergent gauge fields and deconfined fractionalized excitations (spinons).…

Strongly Correlated Electrons · Physics 2025-06-24 Bin Gao , Félix Desrochers , David W. Tam , Paul Steffens , Arno Hiess , Yixi Su , Sang-Wook Cheong , Yong Baek Kim , Pengcheng Dai

The identification of fractionalized excitations in quantum spin liquids (QSLs) remains a central challenge in condensed matter physics. In dipolar-octupolar (DO) pyrochlores, such as $\text{Ce}_2\text{Zr}_2\text{O}_7$, the candidate…

Strongly Correlated Electrons · Physics 2026-01-07 Bin Gao , Zhengbang Zhou , Tingjun Zhang , Andrey Podlesnyak , Sang-Wook Cheong , Yong Baek Kim , Pengcheng Dai

Quantum spin liquids (QSLs) are exotic phases with intrinsic massive entanglements. Instead of microscopic spins, fractionalized particles and gauge fluctuations are emergent, revealing QSLs' exotic natures. Quantum spins with strong…

Strongly Correlated Electrons · Physics 2019-01-16 Sangjin Lee , Eun-Gook Moon

Recently there have been a number of experiments on Ce$_2$Zr$_2$O$_7$ and Ce$_2$Sn$_2$O$_7$, suggesting that these materials host a three-dimensional quantum spin liquid with emergent photons and fractionalized spinon excitations. However,…

Strongly Correlated Electrons · Physics 2020-11-02 Adarsh S. Patri , Masashi Hosoi , Yong Baek Kim

Decisive experimental confirmation of the $U(1)$ quantum spin liquid phase in quantum spin ice remains an outstanding challenge. In this work, we propose stray-field magnetometry as a direct probe of the emergent photons -- the gapless…

Strongly Correlated Electrons · Physics 2025-12-18 Gautam K. Naik , Jonathan N. Hallén , Nishan C. Jayarama , Roderich Moessner , Chris R. Laumann

Electronic spins can form long-range entangled phases of condensed matter named quantum spin liquids. Their existence is conceptualized in models of two- or three-dimensional frustrated magnets that evade symmetry-breaking order down to…

We propose a readily achievable experimental setting where an external magnetic field is used to tune the emergent quantum electrodynamics (eQED) of dipolar-octupolar quantum spin ice (DO-QSI). In $U(1)_\pi$ DO-QSI -- the proposed ground…

Strongly Correlated Electrons · Physics 2024-07-16 Alaric Sanders , Han Yan , Claudio Castelnovo , Andriy H. Nevidomskyy

Recent investigations on the dipolar-octupolar compounds Ce$_2$Zr$_2$O$_7$ and Ce$_2$Sn$_2$O$_7$ suggest that they may stabilize so-called $\pi$-flux octupolar quantum spin ice ($\pi$-O-QSI), a novel three-dimensional quantum spin liquid…

Strongly Correlated Electrons · Physics 2024-02-13 Félix Desrochers , Yong Baek Kim

Quantum spin liquid (QSL) is an exotic quantum phase of matter whose ground state is quantum-mechanically entangled without any magnetic ordering. A central issue concerns emergent excitations that characterize QSLs, which are…

Strongly Correlated Electrons · Physics 2018-05-08 Y. Tokiwa , T. Yamashita , D. Terazawa , K. Kimura , Y. Kasahara , T. Onishi , Y. Kato , M. Halim , P. Gegenwart , T. Shibauchi , S. Nakatsuji , E. -G. Moon , Y. Matsuda

We consider a class of d- and f-electron systems in which dipolar-octupolar Kramers doublets arise on the sites of the pyrochlore lattice. For such doublets, two components of the pseudospin transform like a magnetic dipole, while the other…

Strongly Correlated Electrons · Physics 2014-04-29 Yi-Ping Huang , Gang Chen , Michael Hermele

We present a new mechanism for Raman scattering of phonons, which is based on the linear magnetoelastic coupling present in non-Kramers magnetic ions. This provides a direct coupling of Raman-active phonons to the magnet's quasiparticles.…

Strongly Correlated Electrons · Physics 2022-08-17 Arnab Seth , Subhro Bhattacharjee , Roderich Moessner

Recent experiments on the dipolar-octupolar pyrochlore compound Ce$_2$Zr$_2$O$_7$ indicate that it may realize a three-dimensional quantum spin liquid (QSL). In particular, the analyses of available data suggest that the system is in a…

Strongly Correlated Electrons · Physics 2022-06-30 Félix Desrochers , Li Ern Chern , Yong Baek Kim

Many unconventional quantum phases host special non-magnetic excitations such as photons and visons. We discuss two possible ways to detect these excitations experimentally. Firstly, spin-lattice coupling mixes the excitations with phonons.…

Strongly Correlated Electrons · Physics 2015-05-30 Zhihao Hao

Gapless fracton quantum spin liquids are exotic phases of matter described by higher-rank U(1) gauge theories which host gapped and immobile fracton matter excitations as well as gapless photons. Despite well-known field theories, no spin…

Strongly Correlated Electrons · Physics 2025-08-12 Nils Niggemann , Meghadeepa Adhikary , Yannik Schaden-Thillmann , Johannes Reuther

Recent experiments on Ce$_2$Zr$_2$O$_7$ suggest that this material may host a novel form of quantum spin ice, a three-dimensional quantum spin liquid with an emergent photon. The Ce$^{3+}$ local moments on the pyrochlore lattice are…

Strongly Correlated Electrons · Physics 2023-01-26 Masashi Hosoi , Emily Z. Zhang , Adarsh S. Patri , Yong Baek Kim

We investigate resonant photoluminescence arising from incompressible quantum liquids formed in two-dimensional electron systems. We demonstrate that, for excitons composed of a photoexcited electron occupying the upper spin sublevel of the…

Mesoscale and Nanoscale Physics · Physics 2025-07-21 D. A. Shchigarev , A. V. Larionov , L. V. Kulik , E. M. Budanov , I. V. Kukushkin , V. Umansky

Understanding the nature and behaviour of excitations in quantum spin liquids, and in topological phases of matter in general, is of fundamental importance and has proven crucial for experimental detection and characterisation of candidate…

Strongly Correlated Electrons · Physics 2019-08-07 Attila Szabó , Claudio Castelnovo

In a quantum spin liquid, the magnetic moments of the constituent electron spins evade classical long-range order to form an exotic state that is quantum entangled and coherent over macroscopic length scales [1-2]. Such phases offer…

Recent excitement in the quantum spin ice community has come from the experimental discovery of pseudospin-$1/2$ breathing pyrochlores, including Ba$_3$Yb$_2$Zn$_5$O$_{11}$, in which inversion symmetry is broken by the `up' and `down'…

Strongly Correlated Electrons · Physics 2024-05-14 Alaric Sanders , Claudio Castelnovo

The search for quantum spin liquids (QSL) -- topological magnets with fractionalized excitations -- has been a central theme in condensed matter and materials physics. While theories are no longer in short supply, tracking down materials…

Strongly Correlated Electrons · Physics 2022-05-11 Anish Bhardwaj , Shu Zhang , Han Yan , Roderich Moessner , Andriy H. Nevidomskyy , Hitesh J. Changlani
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