Related papers: Strong-field chiral imaging with twisted photoelec…
We report the first observation of free-electron angular momentum wave packets generated by atomic multiphoton ionization with bichromatic three-dimensional (3D) polarization-tailored ultrashort laser fields. These fields, created by the…
Imaging is of great importance in everyday life and various fields of science and technology. Conventional imaging is achieved by bending light rays originating from an object with a lens. Such ray bending requires space-variant structures,…
Intense laser ionization expands Einstein's photoelectric effect rules giving a wealth of phenomena widely studied over the last decades. In all cases, so far, photons were assumed to carry one unit of angular momentum. However it is now…
Chirality is a concept that one object is not superimposable on its mirror image by translation and rotation. In particular, chiral plasmonics have been widely investigated due to their excellent optical chiral properties, and have led to…
Light waves possess multiple degrees of freedom besides intensity, including phase and polarization, that often contain important information but require complex and bulky systems for their measurement. Here we report a pair of compact…
Owing to the ubiquity and easy-to-shape property of optical intensity, the intensity gradient force of light has been most spectacularly exploited in optical manipulation of small particles. Manifesting the intensity gradient as an optical…
The ability to create surface structures with precisely controlled chirality remains a major challenge in laser-matter interaction experiments. In this work, we theoretically study the interaction of vortex laser beams, characterized by…
Sensing chirality is of fundamental importance to many fields, including analytical and biological chemistry, pharmacology, and fundamental physics. Recent developments have extended optical chiral sensing using microwaves, fs pulses,…
Strong-field physics is currently experiencing a shift towards the use of mid-IR driving wavelengths. This is because they permit conducting experiments unambiguously in the quasi-static regime and enable exploiting the effects related to…
A method for the generation of ultrarelativistic electron beams with high spin polarization is put forward, where a tightly-focused linearly-polarized ultraintense laser pulse interacts with a nonprepolarized transverse-size-tailored solid…
We have recorded the coherent diffraction images of individual xenon clusters with intense extreme ultraviolet pulses to elucidate the influence of light-induced electronic changes on the diffraction pattern. Using the FLASH free-electron…
The transverse component of the spin angular momentum of evanescent waves gives rise to lateral optical forces on chiral particles, which have the unusual property of acting in a direction in which there is neither a field gradient nor wave…
We present energy-resolved measurements of electron emission from sharp metal tips driven with low energy pulses from a few-cycle laser oscillator. We observe above-threshold photoemission with a photon order of up to 9. At a laser…
We show how a spin polarization can be generated through the photo-induced electron transfer of an achiral donor-acceptor complex following chiral light excitation. In particular, we illustrate the basic energetic and symmetry requirements…
A new pathway of strong laser field induced ionization of an atom is identified which is based on recollisions under the tunneling barrier. With an amended strong field approximation, the interference of the direct and the under-the-barrier…
We theoretically show that a single free electron in circular/spiral motion radiates an electromagnetic wave possessing helical phase structure and carrying orbital angular momentum. We experimentally demonstrate it by double-slit…
We report on strong field ionization of S- and R-propylene oxide in circularly polarized two-color laser fields. We find that the relative helicity of the two single color laser fields affects the photoelectron circular dichroism (PECD).…
We consider the process of atomic ionization driven by a laser pulse with varying ellipticity. We study distribution of the momenta of the photoelectrons, ionized by a strong laser field, emitted in the direction perpendicular to the…
We theoretically propose a multidimensional high-harmonic echo spectroscopy technique which utilizes strong optical fields to resolve coherent electron dynamics spanning an energy range of multiple electron Volts. Using our recently…
Twisted atomic bilayers are emerging platforms for manipulating chiral light-matter interaction at the extreme nanoscale, due to their inherent magnetoelectric responses induced by the finite twist angle and quantum interlayer coupling…