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Multiple exciton generation (MEG) is a widely studied phenomenon in semiconductor nanocrystals and quantum dots, aimed at improving the energy conversion efficiency of solar cells. MEG is the process wherein incident photon energy is…

Strongly Correlated Electrons · Physics 2023-10-24 S. R. Sahu , S. Khan , A. Tripathy , K. Dey , N. Bano , S. Raj Mohan , M. P. Joshi , S. Verma , B. T. Rao , V. G. Sathe , D. K. Shukla

We have shown theoretically that efficient multiple exciton generation (MEG) by a single photon can be observed in small nanocrystals (NCs). Our quantum simulations that include hundreds of thousands of exciton and multi-exciton states…

Mesoscale and Nanoscale Physics · Physics 2010-09-23 Wayne M. Witzel , Andrew Shabaev , C. Stephen Hellberg , Verne L. Jacobs , Alexander L. Efros

Multiple exciton generation (MEG) is a process in which more than one exciton is generated upon the absorption of a high energy photon, typically higher than two times the band gap, in semiconductor nanocrystals. It can be observed…

Multiple exciton generation (MEG) in nanometer-sized hydrogen-passivated silicon nanowires (NWs), and quasi two-dimensional nanofilms strongly depends on the degree of the core structural disorder as shown by the many-body perturbation…

Mesoscale and Nanoscale Physics · Physics 2014-11-25 Andrei Kryjevski , Dmitri Kilin

Utilizing the excess energy of photoexcitation that is otherwise lost as thermal effects can improve the efficiency of next-generation light-harvesting devices. Multiple exciton generation (MEG) in semiconducting materials yields two or…

Materials Science · Physics 2022-12-06 Ashish Soni , Dushyant Kushavah , Li-Syuan Lu , Wen-Hao Chang , Suman Kalyan Pal

We use Boltzmann transport equation (BE) to study time evolution of a photo-excited state in a nanoparticle including phonon-mediated exciton relaxation and the multiple exciton generation (MEG) processes, such as exciton-to-biexciton…

Mesoscale and Nanoscale Physics · Physics 2017-11-22 Andrei Kryjevski , Deyan Mihaylov , Svetlana Kilina , Dmitri Kilin

We show that bi-exciton formation can be highly efficient in a solar cell with the semiconductor absorber filled with an array of metallic nanoparticles having plasmonic resonance tuned to the semiconductor gap energy. This process can be…

Materials Science · Physics 2019-06-12 Jiantao Kong , Xueyuan Wu , Xin Wang , Michael J Naughton , Krzysztof Kempa

Multiple exciton generation is a process in which more than one electron hole pair is generated per absorbed photon. It allows us to increase the efficiency of solar energy harvesting. Experimental studies have shown the multiple exciton…

Mesoscale and Nanoscale Physics · Physics 2016-08-11 Fikeraddis A. Damtie , Khadga J. Karki , Tõnu Pullerits , Andreas Wacker

We study the coherent mixing between two-particle (single exciton) and four-particle (biexciton) states of a semiconductor nanocrystal resulting from the coulomb coupling between states with different numbers of electron-hole pairs. Using a…

Mesoscale and Nanoscale Physics · Physics 2016-02-26 P. Kowalski , P. Machnikowski

Magnetoelectroluminescence (MEL) of organic semiconductor has been experimentally tuned by adopting blended emitting layer consisting of both hole and electron transporting materials. A theoretical model considering intermolecular quantum…

Materials Science · Physics 2015-05-14 B. F. Ding , Y. Yao , X. Y. Sun , Z. Y. Sun , X. D. Gao , Z. T. Xie , Z. J. Wang , X. M. Ding , Y. Z. Wu , X. F. Jin , C. Q. Wu , X. Y. Hou

Unique properties of lead chalcogenides have enabled multiple exciton generation (MEG) in their nanocrystals that can be beneficial in enhancing the efficiency of the third generation solar cells. Although the intrinsic electric field plays…

Atomic and Molecular Clusters · Physics 2017-09-07 Mahdi Gordi , Mohammad Kazem Moravvej-Farshi , Hamidreza Ramezani

The two-dimensional semiconductor MoS2 in its mono- and few-layer form is expected to have a significant exciton binding energy of several 100 meV, leading to the consensus that excitons are the primary photoexcited species. Nevertheless,…

This paper reviews both experimental and theoretical work on nanostructures showing high quantum yields due to the phenomenon of multiple exciton generation. It outlines the aims and barriers to progress in identifying further such…

Mesoscale and Nanoscale Physics · Physics 2018-06-06 Nicholas Siemons , Alessio Serafini

We study the exciton dynamics in an optically excited nanocrystal quantum dot. Multiple exciton formation is more efficient in nanocrystal quantum dots compared to bulk semiconductors due to enhanced Coulomb interactions and the absence of…

Mesoscale and Nanoscale Physics · Physics 2016-05-02 Fikeraddis A. Damtie , Andreas Wacker

We present detailed analysis of the non-Poissonian population of excitons produced by MEG effect in quantum dots on the base of statistic theory of MEG and synergetic approach for chemical reactions. From the analysis we can conclude that a…

Quantum Physics · Physics 2015-05-28 N. N. Turaeva , B. L. Oksengendler , I. Uralov

Multiple exciton generation solar cells exhibit a low power conversion efficiency owing to nonradiative recombination even if numerous electron and hole pairs are generated per incident photon. This paper elucidates the non-idealities of…

Applied Physics · Physics 2021-04-14 Jongwon Lee

Although van der Waals layered transition metal dichalcogenides from transient absorption spectroscopy have successfully demonstrated an ideal carrier multiplication (CM) performance with an onset of nearly 2Eg,interpretation of the CM…

Mesoscale and Nanoscale Physics · Physics 2021-04-20 Jun Suk Kim , Minh Dao Tran , Sung-Tae Kim , Daehan Yoo , Sang-Hyun Oh , Ji-Hee Kim , Young Hee Lee

The statistical theory of multiple exciton generation in quantum dots which is based on the Fermi approach to the problem of multiple particle in nucleon-nucleon collisions is presented. Our estimates of the multiple exciton generation…

Mesoscale and Nanoscale Physics · Physics 2011-02-07 B. L. Oksengendler , N. N. Turaeva , S. S. Rashidova

Photogenerated excitonic ensembles confined in coupled GaAs quantum wells are probed by a complementary approach of emission spectroscopy and resonant inelastic light scattering. Lateral electrostatic trap geometries are used to create…

The conversion of light into free electron-hole pairs constitutes the key process in the fields of photodetection and photovoltaics. The efficiency of this process depends on the competition of different relaxation pathways and can be…

Mesoscale and Nanoscale Physics · Physics 2013-04-24 K. J. Tielrooij , J. C. W. Song , S. A. Jensen , A. Centeno , A. Pesquera , A. Zurutuza Elorza , M. Bonn , L. S. Levitov , F. H. L. Koppens
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