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The combination of high-order harmonic generation (HHG) with resonant XUV excitation of a core electron into the transient valence vacancy that is created in the course of the HHG process is investigated theoretically. In this setup, the…

Atomic Physics · Physics 2023-01-10 Christian Buth , Markus C. Kohler , Joachim Ullrich , Christoph H. Keitel

Isolated attosecond pulses (IAPs) produced through laser-driven high-harmonic generation (HHG) hold promise for unprecedented insight into biological processes via attosecond x-ray diffraction with tabletop sources. However, efficient…

We report a novel quasi-phase matching technique for high-order harmonic generation in low-density gases. Numerical simulations show that in few-optical cycle pulsed Bessel beams it is possible to control the pulse envelope and phase…

In our recent study [Commun. Phys. 3, 92 (2020)], we have developed an approach for energy-scaling of high-order harmonic generation in water-window region under neutral-medium condition. More specifically, we obtained nanojoule-class…

We perform an experimental two-color high-order harmonic generation study in argon with the fundamental of an ytterbium ultrashort pulse laser and its second harmonic. The intensity of the second harmonic and its phase relative to the…

The laser interaction with an electron-positron-ion mixed plasma is studied, from the perspective of the associated high-order harmonic generation. For an idealized mixed plasma which is assumed with a sharp plasma-vacuum interface and…

Plasma Physics · Physics 2021-01-20 W. L. Zhang , T. Grismayer , K. M. Schoeffler , R. A. Fonseca , L. O. Silva

We present theoretical investigations of high-order harmonic generation (HHG) resulting from the interaction of noble gases with localized surface plasmons. These plasmonic fields are produced when a metal nanoparticle is subject to a…

Plasmon resonances are known to amplify the electromagnetic fields near metallic nanostructures. Therefore, they are considered to provide a promising scheme to generate extreme-ultraviolet harmonics, using low power drivings. During…

We observe a new regime of coherent XUV radiation generation in noble gases induced by femtosecond pulses at very high intensities. This XUV emission has both a reduced divergence and spectral width as compared to high-order harmonic…

We report here experimental results of perturbative nonlinear optical wave-mixing processes in the extreme ultraviolet region by using two-color and three-color laser fields. Besides the usual odd-harmonic spectrum of high harmonic…

Optics · Physics 2019-04-02 Khoa Anh Tran , Khuong Ba Dinh , Peter Hannaford , Lap Van Dao

We employ the R-matrix with time-dependence method to investigate extreme-ultraviolet-initiated high-harmonic generation (XIHHG) in Ar$^{+}$. Using a combination of extreme-ultraviolet (XUV, $92\textrm{ nm}$, $3\times…

Atomic Physics · Physics 2018-03-14 D. D. A. Clarke , H. W. van der Hart , A. C. Brown

Based upon our previous works (Eur.Phys.J.D 6, 319(1999); Chin.Phys.Lett. 18, 236(2001)), we develop a classical approach to calculate the high-order harmonic generation of the laser driven atoms and molecules. The Coulomb singularities in…

Atomic Physics · Physics 2007-05-23 Chaohong Lee , Yiwu Duan , Wing-Ki Liu , Jian-Min Yuan , Lei Shi , Xiwen Zhu , Kelin Gao

Intense extreme-ultraviolet (XUV) pulses enable the investigation of XUV-induced nonlinear processes and are a prerequisite for the development of attosecond pump - attosecond probe experiments. While highly nonlinear processes in the XUV…

In this report, a novel methodology based on the static coherent states approach is introduced with the capability of calculating various strong-field laser-induced nonlinearities in full dimensional single-electron molecular systems; an…

Quantum Physics · Physics 2019-10-10 Mohammadreza Eidi , Mohsen Vafaee , Hamed Koochaki Kelardeh , Alexandra Landsman

High harmonic generation (HHG) is a manifestation of the strongly nonlinear response of matter to intense laser fields and has, as the basis for coherent XUV sources a variety of applications. Recently, HHG from atoms in a phase and…

Optics · Physics 2020-05-20 Jonas Wätzel , Jamal Berakdar

We present studies of high-order harmonic generation (HHG) at laser intensities well above saturation. We use driving laser pulses which present a particular electron dynamics in the turn-on stage. Our results predict an increasing on the…

Atomic Physics · Physics 2015-06-19 J. A. Pérez-Hernández , M. F. Ciappina , M. Lewenstein , A. Zaïr , L. Roso

We investigate the case of phase-matched high-harmonic generation in a gas-filled capillary waveguide, comparing in detail theory with experiment. We observe three different regimes of phase matching: one where atomic dispersion balances…

Since the new millennium coherent extreme ultra-violet and soft x-ray radiation has revolutionized the understanding of dynamical physical, chemical and biological systems at the electron's natural timescale. Unfortunately, coherent…

A theoretical model is developed describing high-order harmonic generation (HHG) from a gas of multiply-charged ions driven by a laser field of relativistic intensity. Macroscopic propagation of harmonics is investigated in a relativistic…

Atomic Physics · Physics 2012-02-21 Markus C. Kohler , Karen Z. Hatsagortsyan

We present theoretical predictions of high-order harmonic generation (HHG) resulting from the interaction of short femtosecond laser pulses with metal nanotips. It has been demonstrated that high energy electrons can be generated using…