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The electron-phonon coupling and the corresponding energy exchange was investigated experimentally and by ab initio theory in non-equilibrium states of the free-electron metal aluminium. The temporal evolution of the atomic mean squared…

Materials Science · Physics 2016-04-11 Lutz Waldecker , Roman Bertoni , Jan Vorberger , Ralph Ernstorfer

A short overview of theoretical models for the description of the relaxation processes in metals excited by a short laser pulse is presented. The main effort is given to description of different processes which are taking place after…

Strongly Correlated Electrons · Physics 2020-05-20 V. V. Kabanov

Electron-phonon coupling, being one of the most important parameters governing the material evolution after ultrafast energy deposition, yet remains the most unexplored one. In this work, we applied the dynamical coupling approach to…

Materials Science · Physics 2020-08-05 N. Medvedev , I. Milov

Electron-ion interactions play a central role for the energy relaxation processes and ultra-fast structure dynamics in laser-heated matter. The accurate prediction of the electron-ion energy exchange in a transient excited two-temperature…

Other Condensed Matter · Physics 2024-01-17 Jia Zhang , Rui Qin , Wenjun Zhu , Jan Vorberger

We determined electronic relaxation times via pump-probe optical spectroscopy using sub-15 fs pulses for the normal state of two different cuprate superconductors.We show that the primary relaxation process is the electron-phonon…

Multi-temperature models are nowadays often used to quantify the ultrafast electron-phonon (boson) relaxations and coupling strengths in advanced quantum solids. To test their applicability we study the time evolution of the electron…

Materials Science · Physics 2020-01-29 Manuel Obergfell , Jure Demsar

A theoretical approach using ab initio calculations has been applied to study the interaction of an ultra-short laser pulse with the metal alloy Fe$_{0.72}$Cr$_{0.18}$Ni$_{0.1}$ (AISI 304). The electronic structure is simulated by taking…

Materials Science · Physics 2016-04-20 Jan Winter , Jürgen Sotrop , Stephan Borek , Heinz P. Huber , Jan Minár

The low temperature electron-phonon (e-ph) relaxation near the surface of noble metals, Cu and Ag, is studied by using the density-functional theory approach. The appearance of the surface phonon mode can give rise to a strong enhancement…

Materials Science · Physics 2020-05-20 Shota Ono

We consider the deformation potential mechanism of the electron-phonon coupling in metal films and investigate the intensity of the associated heat transfer between the electron and phonon subsystems. The focus is on the temperature region…

Mesoscale and Nanoscale Physics · Physics 2016-03-31 S. Cojocaru , D. V. Anghel

The equilibration of electronic carriers in metals after excitation by an ultra-short laser pulse provides an important class of non-equilibrium phenomena in metals and allows measuring the effective electron-phonon coupling parameter.…

Materials Science · Physics 2022-10-06 Peter Kratzer , Laurenz Rettig , Irina Yu. Sklyadneva , Evgueni V. Chulkov , Uwe Bovensiepen

Coupling between electrons and phonons (lattice vibrations) drives the formation of the electron pairs responsible for conventional superconductivity. The lack of direct evidence for electron-phonon coupling in the electron dynamics of the…

We study the electron and phonon thermalization in simple metals excited by a laser pulse. The thermalization is investigated numerically by solving the Boltzmann transport equation taking into account all the relevant scattering mechanism:…

Materials Science · Physics 2018-02-28 Shota Ono

We present a theory for the rate of energy exchange between electrons and ions -- also known as the electron-ion coupling factor -- in physical systems ranging from hot solid metals to plasmas, including liquid metals and warm dense matter.…

Plasma Physics · Physics 2019-10-16 Jerome Daligault , Jacopo Simoni

Electron-electron thermalization and electron-phonon relaxation processes in laser-excited solids are often assumed to occur on different timescales. This is true for the majority of the conduction band electrons in a metal. However,…

Mesoscale and Nanoscale Physics · Physics 2019-06-05 Sebastian T. Weber , Baerbel Rethfeld

Electron-phonon coupling is a fundamental process that governs the energy relaxation dynamics of solids excited by ultrafast laser pulses. It has been found to strongly depend on electron temperature as well as on nonequilibrium effects.…

Materials Science · Physics 2023-08-03 Tobias Held , Sebastian T. Weber , Baerbel Rethfeld

We applied Time-Resolved Two-Photon Photoemission spectroscopy to probe the electron- phonon (e-ph) coupling strength in double-wall carbon nanotubes. The e-ph energy transfer rate G(Te,Tl) from the electronic system to the lattice depends…

Materials Science · Physics 2013-08-07 Ioannis Chatzakis

Using the Eliashberg theory of superconductivity we have examined several properties of a model in which electrons are coupled only to rattling phonon modes represented by a sharp peak in the electron-phonon coupling function. Our choice of…

Superconductivity · Physics 2018-07-13 Samin Tajik , Božidar Mitrović , Frank Marsiglio

Ultrafast laser measurements probe the non-equilibrium dynamics of excited electrons in metals with increasing temporal resolution. Electronic structure calculations can provide a detailed microscopic understanding of hot electron dynamics,…

Computational Physics · Physics 2016-08-12 Ana M. Brown , Ravishankar Sundararaman , Prineha Narang , William A. Goddard , Harry A. Atwater

Using full-potential, density-functional-based methods we have studied electron-phonon interaction in ZrB2 and TaB2 in P6/mmm crystal structure. Our results for phonon density of states and Eliashberg function show that the electron-phonon…

Superconductivity · Physics 2009-11-10 Prabhakar P. Singh

The theory of the electron relaxation in metals excited by an ultrashort optical pump is developed on the basis of the solution of the linearized kinetic equation. The kinetic equation includes both the electron-electron and the…

Strongly Correlated Electrons · Physics 2014-03-06 V. V. Baranov , V. V. Kabanov
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