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Two frequency combs can be used to measure the full complex response of a sample in a configuration which can be alternatively viewed as the equivalent of a dispersive Fourier transform spectrometer, infrared time domain spectrometer, or a…

Optics · Physics 2015-05-18 I. Coddington , W. C. Swann , N. R. Newbury

The femtosecond laser frequency comb has enabled the 21st century revolution in optical synthesis and metrology. A particularly compelling technique that relies on the broadband coherence of two laser frequency combs is dual-comb…

Optics · Physics 2023-07-19 Vicente Duran , Santiago Tainta , Victor Torres-Company

Molecular spectroscopy in the mid-infrared portion of the electromagnetic spectrum (3--25 um) has been a cornerstone interdisciplinary analytical technique widely adapted across the biological, chemical, and physical sciences. Applications…

Instrumentation and Detectors · Physics 2018-09-18 Abijith S. Kowligy , Henry Timmers , Alex Lind , Ugaitz Elu , Flavio C. Cruz , Peter G. Schunemann , Jens Biegert , Scott A. Diddams

Time-resolved near-infrared absorption spectroscopy of single non-repeatable transient events is performed at high spectral resolution with a dual-comb interferometer using a continuous-wave laser followed by a single electro-optic…

Dual Comb Spectroscopy proved its versatile capabilities in molecular fingerprinting in different spectral regions, but not yet in the ultraviolet (UV). Unlocking this spectral window would expand fingerprinting to the electronic energy…

On-chip spectroscopy that could realize real-time fingerprinting with label-free and high-throughput detection of trace molecules is one of the 'holy grails" of sensing. Such miniaturized spectrometers would greatly enable applications in…

Ultrabroadband electro-optic sampling with few-cycle optical pulses is known to be an extremely sensitive technique to detect electric field amplitudes. By combining this method with dual-comb spectroscopy and with a new class of ultrafast…

A laser frequency combs is a broad spectrum composed of equidistant narrow lines. Initially invented for frequency metrology, such combs enable new approaches to spectroscopy over broad spectral bandwidths, of particular relevance to…

Optics · Physics 2019-03-01 Nathalie Picqué , Theodor W. Hänsch

We introduce a new parallelized approach to photothermal microscopy that utilizes mid-infrared dual-comb lasers, enabling simultaneous measurements at hundreds of wavelengths. This technology allows for high-speed, label-free chemical…

We demonstrate a high-accuracy dual-comb spectrometer centered at 3.4 \mu m. The amplitude and phase spectra of the P, Q, and partial R-branch of the methane {\nu}3 band are measured at 25 MHz to 100 MHz point spacing with ~kHz resolution…

Dual-comb spectroscopy allows for the rapid, multiplexed acquisition of high-resolution spectra without the need for moving parts or low-resolution dispersive optics. This method of broadband spectroscopy is most often accomplished via…

The optical frequency comb has made a significant impact in precision spectroscopy and on our ability to probe atomic, molecular and, recently, nuclear transitions to further our understanding of their fundamental properties and how their…

Optics · Physics 2026-02-17 John J. McCauley , DylanP. Tooley , R. Jason Jones

Dual comb spectroscopy allows for high-resolution spectra to be measured over broad bandwidths, but an essential requirement for coherent integration is the availability of a phase reference. Usually, this means that the combs' phase and…

Optics · Physics 2016-06-01 David Burghoff , Yang Yang , Qing Hu

We present a new type of dual optical frequency comb source capable of scaling applications to high measurement speeds while combining high average power, ultra-low noise operation, and a compact setup. Our approach is based on a…

Dual-comb spectroscopy has emerged as an indispensable analytical technique in applications that require high resolution and broadband coverage within short acquisition times. Its experimental realization, however, remains hampered by…

Instrumentation and Detectors · Physics 2019-12-02 Łukasz A. Sterczewski , Aleksandra Przewłoka , Wawrzyniec Kaszub , Jarosław Sotor

Dual-comb spectroscopy is a powerful technique to measure optical spectra in a wide spectral range with high-frequency resolution. The development of compact systems operating in the long-wave infrared wavelength range is of high interest…

Dual-comb ranging has emerged as an effective technology for long-distance metrology, providing absolute distance measurements with high speed, precision, and accuracy. Here, we demonstrate a dual-comb ranging method that utilizes a…

Optical frequency combs emit narrow pulses of light with a stable repetition rate. Equivalently, the generated light spectrum consists of many discrete frequencies spaced by this same repetition rate. These precision light sources have…

Optics · Physics 2024-02-05 N. J. Lambert , L. S. Trainor , H. G. L. Schwefel

We present quasi-real-time dual-comb spectroscopy (DCS) using two Yb:fiber combs with ~750 MHz repetition rates. A computational coherent averaging technique is employed to correct timing and phase fluctuations of the measured dual-comb…

As a potent greenhouse gas and ozone depleting agent, nitrous oxide (N$_2$O) plays a critical role in the global climate. Effective mitigation relies on understanding global sources and sinks which can be supported through isotopic…

Instrumentation and Detectors · Physics 2020-10-21 D. Michelle Bailey , Gang Zhao , Adam J. Fleisher