Related papers: THz non-linear optical response in cuprates: predo…
The recent observation of a transmitted Thz pulse oscillating at three times the frequency of the incident light paves the way to a new protocol to access resonant excitations in a superconductor. Here we show that this non-linear optical…
We present a detailed theoretical investigation of the linear and non-linear optical response in a model system for a disordered d-wave superconductor, showing that for both quantities the gap symmetry considerably changes the paradigm of…
The presence of optical polarization anisotropies, such as Faraday/Kerr effects, linear birefringence, and magnetoelectric birefringence are evidence for broken symmetry states of matter. The recent discovery of a Kerr effect using near-IR…
Recent experiments with strong THz fields in both conventional and unconventional superconductors have clearly evidenced a marked third-harmonic generation below the superconducting temperature $T_c$. Its interpretation challenged…
Recent advances in time-domain terahertz (THz) spectroscopy have unveiled that resonantly-enhanced strong THz third-harmonic generation (THG) mediated by the collective Higgs amplitude mode occurs in s-wave superconductors, where…
We have performed an angle-resolved photoemission study of the nodal quasi-particle spectra of the high-Tc cuprate tri-layer Bi2Sr2Ca2Cu3O10+d (Tc~ 110 K). The spectral weight Z of the nodal quasi-particle increases with decreasing…
Although cuprate superconductors have been intensively studied for the past decades, there is no consensus regarding the microscopic origin of their superconductivity. In this work, we measure the low-energy electrodynamic response of…
Unconventional superconductivity in the cuprates emerges from, or coexists with, other types of electronic order. However, these orders are sometimes invisible because of their symmetry. For example, the possible existence of superfluid…
Terahertz nonlinear optics is a viable method to interrogate collective phenomena in quantum materials spanning ferroelectrics, charge-density waves, and superconductivity. In superconductors this includes the Higgs amplitude and Josephson…
A pivotal step toward understanding unconventional superconductors would be to decipher how superconductivity emerges from the unusual normal state upon cooling. In the cuprates, traces of superconducting pairing appear above the…
We investigated the terahertz (THz)-pulse driven nonlinear response in the d-wave cuprate superconductor Bi2Sr2CaCu2O8+x (Bi2212) using a THz pump near-infrared probe scheme in the time domain. We have observed an oscillatory behavior of…
Measuring terahertz waveforms in terahertz spectroscopy often relies on electrooptic sampling employing a ZnTe crystal. Although the nonlinearities in such zincblende semiconductors induced by intense terahertz pulses have been studied at…
A puzzling phenomenon has been recently revealed in terahertz nonlinear optical response experiments: A third harmonic generation (THG) signal, identified only in the superconducting (SC) phase in a conventional BCS superconductor, is found…
Josephson plasmons in layered superconductors represent a natural source of optical non-linearity, thanks to their intrinsically anharmonic nature. Here we derive the selection rules behind non-linear plasmonics showing its dependence on…
In multiband superconductors, multiple collective modes exist associated with the multiple order parameters. Oscillations of the amplitude and the relative phase of the order parameters are called Higgs and Leggett modes, respectively.…
In a superconductor the third-harmonic generation (THG) of a strong THz pulse is enhanced below Tc by the resonant excitation of lattice-modulated charge fluctuations (LCF), which modulate the response according to the polarization of the…
We report on the first experimental observation of a very strong nonlinear response in crystalline quartz in the terahertz (THz) frequency region through THz time-domain spectroscopy (THz-TDS). Theoretical modelling is presented and…
High-temperature superconductivity (HTS) of cuprates represents a challenge to the conventional theory. Here I review a multi-polaron approach to the problem based on our extension of the BCS theory to the strong-coupling regime. Since…
We study the nonlinear optical response in a superconducting NbN thin film with strong terahertz (THz)wave. Besides the expected third harmonic generation, we observe a new transient oscillation which softensin frequency with temperature…
Recent experiments on K$_3$C$_{60}$ and layered copper-oxide materials have reported substantial changes in the optical response following application of an intense THz pulse. These data have been interpreted as the stimulation of a…