Related papers: Spectroscopy on the eEDM-sensitive states of ThF$^…
We report ab initio relativistic correlation calculations of potential curves and spectroscopic constants for four lowest-lying electronic states of the lead monofluoride. We also calculated parameters of the spin-rotational Hamiltonian for…
We report high-precision measurements on the thallium fluoride $\tilde{J} = 1$ hyperfine manifold of the $B^3\Pi_1$ ($\nu = 0$) state. This state is of special interest because it is central to an optical cycling scheme that is envisioned…
A precise theoretical study of the electronic structure of heavy atom diatomic molecules is of key importance to interpret the experiments in the search for violation of time-reversal (T) and spatial-parity (P) symmetries of fundamental…
This paper is a theoretical work in support of a newly proposed experiment (R. Stutz and E. Cornell, Bull. Am. Soc. Phys. 89, 76 2004) that promises greater sensitivity to measurements of the electron's electric dipole moment (EDM) based on…
We present progress towards a new measurement of the electron electric dipole moment using a cold supersonic beam of YbF molecules. Data are currently being taken with a sensitivity of $10^{-27}\textrm{e.cm}/\sqrt{\textrm{day}}$. We…
The g-factors for $J = 1$, $F=3/2$, $|M_F|=3/2$ hyperfine levels of the ground electronic state $^3\Delta_1$ of the $^{232}$ThF$^+$ cation are calculated as functions of the external electric field. These calculations are necessary for the…
Heavy polar diatomic molecules are the primary tools for searching for the T-violating permanent electric dipole moment of the electron (eEDM). Valence electrons in some molecules experience extremely large effective electric fields due to…
We propose using matrix-isolated paramagnetic diatomic molecules to search for the electric dipole moment of electron (eEDM). As was suggested by Shapiro in 1968, the eEDM leads to a magnetization of a sample in the external electric field.…
Permanent electric dipole moments (EDMs) of fundamental particles such as the electron are signatures of parity and time-reversal violation due to physics beyond the standard model. EDM measurements probe new physics at energy scales well…
A recently implemented relativistic four-component configuration interaction approach to study ${\cal{P}}$- and ${\cal{T}}$-odd interaction constants in atoms and molecules is employed to determine the electron electric dipole moment…
Measurement of a non-zero electric dipole moment (EDM) of the electron within a few orders of magnitude of the current best limit of |d_e| < 1.05 e -27 e cm would be an indication of physics beyond the Standard Model. The ACME Collaboration…
The T-odd phenomenon of induction of the magnetic field by a static electric field provides to study the electron EDM and constants of T-odd, P-odd interaction of an electron with a nucleus. Measurement of this magnetic field for…
The most sensitive measurements of the electron electric dipole moment d_e have previously been made using heavy atoms. Heavy polar molecules offer a greater sensitivity to d_e because the interaction energy to be measured is typically 10^3…
The current constraint on the electron electric dipole moment ($e$EDM), $|d_e|<4.1\times 10^{-30}$ ${e {\cdotp} {\rm cm}}$ (90\% confidence), was recently established using the trapped $^{180}$Hf$^{19}$F$^+$ molecular ions in the $J=1$…
Measurements of the electron's electric dipole moment (eEDM) are demanding tests of physics beyond the Standard Model. We describe how ultracold YbF molecules could be used to improve the precision of eEDM measurements by two to three…
The best upper limit for the electron electric dipole moment was recently set by the ACME collaboration. This experiment measures an electron spin-precession in a cold beam of ThO molecules in their metastable $H~(^3\Delta_1)$ state.…
The electric dipole moment of an electron (eEDM) is one of the sensitive probes of physics beyond the standard model. The possible existence of the eEDM gives rise to an experimentally observed energy shift, which is proportional to the…
Heavy polar diatomic molecules are the leading candidates in searches for the permanent electric dipole moment of the electron (eEDM). Next-generation eEDM search experiments ideally require extremely large coherence times, in large…
Efficient quantum-state detection is crucial for many precision control experiments, such as the ongoing effort to probe the electron's electric dipole moment using trapped molecular $^{232}\mathrm{ThF}^+$ ions at JILA. While quantum state…
We use the technique of chopped nonlinear magneto-optic rotation (NMOR) in a room temperature $^{133}$Cs vapor cell to measure the permanent electric dipole moment (EDM) in the atom. The cell has paraffin coating on the walls to increase…