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We consider the nonlinear terahertz response of n-doped monolayer graphene at room temperature using a microscopic theory of carrier dynamics. Our tight-binding model treats the carrier-field interaction in the length gauge, includes phonon…

Mesoscale and Nanoscale Physics · Physics 2019-03-27 L. G. Helt , M. M. Dignam

Graphene as a zero-bandgap two-dimensional semiconductor with a linear electron band dispersion near the Dirac points has the potential to exhibit very interesting nonlinear optical properties. In particular, third harmonic generation of…

Applied Physics · Physics 2018-01-31 Parvin Navaeipour , Ibraheem Al-Naib , Marc M. Dignam

Third harmonic generation of terahertz radiation is expected to occur in monolayer graphene due to the nonlinear relationship between the crystal momentum and the current density. In this work, we calculate the terahertz nonlinear response…

Applied Physics · Physics 2018-06-22 Parvin Navaeipour , Marc M. Dignam

We observe optical third harmonic generation from graphene and few-layer graphite flakes produced by exfoliation. The emission scales with the cube of the intensity of the incident near-infrared femtosecond pulses and has a wavelength that…

Mesoscale and Nanoscale Physics · Physics 2013-03-20 Nardeep Kumar , Jatinder Kumar , Chris Gerstenkorn , Rui Wang , Hsin-Ying Chiu , Arthur L. Smirl , Hui Zhao

We develop a density matrix formalism in the length gauge to calculate the nonlinear response of intrinsic monolayer graphene at terahertz frequencies. Employing a tight-binding model, we find that the interplay of the interband and…

Optics · Physics 2014-12-17 Ibraheem Al-Naib , J. E. Sipe , Marc M. Dignam

The low-energy (intraband) range of the third harmonic generation of graphene in the terahertz regime is governed by the damping terms induced by the interactions. A controlled many-body description of the scattering processes is thus a…

Mesoscale and Nanoscale Physics · Physics 2021-03-24 Habib Rostami , Emmanuele Cappelluti

Graphene has unique properties paving the way for groundbreaking future applications. Its large optical nonlinearity and ease of integration in devices notably makes it an ideal candidate to become a key component for all-optical switching…

The nonlinear responses of different materials provide useful mechanisms for optical switching, low noise amplification, and harmonic frequency generation. However, the nonlinear processes usually have an extremely weak nature and require…

Optics · Physics 2017-08-24 Boyuan Jin , Tianjing Guo , Christos Argyropoulos

We use an exact solution of the relaxation-time Boltzmann equation in a uniform AC electric field to describe the nonlinear optical response of graphene in the terahertz (THz). The cases of monolayer, bilayer and ABA-stacked trilayer…

Mesoscale and Nanoscale Physics · Physics 2014-09-23 N. M. R. Peres , Yu. V. Bludov , Jaime E. Santos , Antti-Pekka Jauho , M. I. Vasilevskiy

A density-matrix formalism within the length gauge is developed for the purpose of calculating the nonlinear response of intrinsic bilayer graphene at terahertz frequencies. Employing a tight-binding model, we find that interplay between…

Mesoscale and Nanoscale Physics · Physics 2016-12-07 Riley McGouran , Ibraheem Al-Naib , Marc M. Dignam

Graphene is a nonlinear material which can be used as a saturable absorber, frequency mixer and frequency multiplier. We investigate the third harmonic generation from graphene lying on different substrates, consisting of a dielectric…

Mesoscale and Nanoscale Physics · Physics 2017-02-09 N. A. Savostianova , S. A. Mikhailov

We study cascaded harmonic generation of hybrid surface plasmons in integrated planar waveguides composed of a graphene layer and a doped-semiconductor slab. We derive a comprehensive model of cascaded third harmonic generation through…

Optics · Physics 2015-10-14 Daria A. Smirnova , Alexander S. Solntsev

We report strong third-harmonic generation (THG) in monolayer graphene grown by chemical vapor deposition (CVD) and transferred to an amorphous silica (glass) substrate; the photon energy is in three-photon resonance with the…

Mesoscale and Nanoscale Physics · Physics 2013-06-12 Sung-Young Hong , Jerry I. Dadap , Nicholas Petrone , Po-Chun Yeh , James Hone , Richard M. Osgood

Achieving efficient, high-power harmonic generation in the terahertz spectral domain has technological applications, for example in sixth generation (6G) communication networks. Massless Dirac fermions possess extremely large terahertz…

We investigate through analytic calculations the surface plasmon dispersion relation for monolayer graphene sheets and a separated parallel pair of graphene monolayers. An approximate form for the dispersion relation for the monolayer case…

Mesoscale and Nanoscale Physics · Physics 2012-03-21 Choon How Gan , Hong Son Chu , Er Ping Li

We observe enhanced second-harmonic generation in monolayer graphene in the presence of an ultra-strong terahertz field pulse with a peak amplitude of 250 kV/cm. This is a strongly nonperturbative regime of light-matter interaction in which…

Graphene's exceptional nonlinear optical properties combined with resonant photonic structures offer a promising pathway for efficient nonlinear applications at terahertz (THz) frequencies. In this work, we propose and demonstrate a…

High-harmonic generation (HHG) in solids is an emerging method to probe ultrafast electron dynamics in solids at attosecond timescale. In this work, we study HHG from monolayer and bilayer graphene. Bilayer graphenes with AA and AB stacking…

Optics · Physics 2021-03-26 M. S. Mrudul , Gopal Dixit

Remarkable optical and electrical properties of two-dimensional (2D) materials, such as graphene and transition-metal dichalcogenide (TMDC) monolayers, offer vast technological potential for novel and improved optoelectronic nanodevices,…

Optics · Physics 2016-07-22 Martin Weismann , Nicolae C. Panoiu

Understanding how light interacts at the nanoscale with metals, semiconductors, or ordinary dielectrics is pivotal if one is to properly engineer nano-antennas, filters and, more generally, devices that aim to harness the effects of new…

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