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We report the first quasiparticle calculations of the newly observed wurtzite polymorph of InAs and GaAs. The calculations are performed in the GW approximation using plane waves and pseudopotentials. For comparison we also report the study…

Materials Science · Physics 2009-11-11 Z. Zanolli , F. Fuchs , J. Furthmueller , U. von Barth , F. Bechstedt

This study presents a refined approach to computing the electronic structure of indium antimonide (InSb) using advanced \textit{ab initio} techniques with the In and Sb $4d^{10}$ semicore electrons included in the valence states. These…

Materials Science · Physics 2025-08-04 Ritwik Das , Anne-Sophie Grimault-Jacquin , Frédéric Aniel

We calculate the band gaps of 12 inorganic semiconductors and insulators composed of atoms from the first three rows of the periodic table using periodic equation-of-motion coupled-cluster theory with single and double excitations…

Materials Science · Physics 2023-10-09 Ethan A. Vo , Xiao Wang , Timothy C. Berkelbach

We report the calculated fundamental band gaps of \emph{wurtzite} ternary alloys Zn$_{1-x}$M$_x$O (M=Mg, Cd) and the band offsets of the ZnO/Zn$_{1-x}$M$_x$O heterojunctions, these II-VI materials are important for electronics and…

Materials Science · Physics 2017-01-26 Haitao Yin , Junli Chen , Yin Wang , Jian Wang , Hong Guo

Many-body perturbation theory methods, such as the $G_0W_0$ approximation, are able to accurately predict quasiparticle (QP) properties of several classes of materials. However, the calculation of the QP band structure of two-dimensional…

Materials Science · Physics 2022-06-23 Alberto Guandalini , Pino D'Amico , Andrea Ferretti , Daniele Varsano

We study the effect of semicore states on the self-energy corrections and electronic energy gaps of silicon, germanium and GaAs. Self-energy effects are computed within the GW approach, and electronic states are expanded in a plane-wave…

Materials Science · Physics 2009-11-10 Murilo L. Tiago , Sohrab Ismail-Beigi , Steven G. Louie

We present a systematic study that clarifies validity and limitation of current hybrid functionals in density functional theory for structural and electronic properties of various semiconductors and insulators. The three hybrid functionals,…

Materials Science · Physics 2015-03-19 Yu-ichiro Matsushita , Kazuma Nakamura , Atsushi Oshiyama

We present a plane wave implementation of the G0W0 approximation within the projector augmented wave method code GPAW. The computed band gaps of ten bulk semiconductors and insulators deviate on average by 0.2 eV (~ 5 %) from the…

Materials Science · Physics 2014-01-10 Falco Hüser , Thomas Olsen , Kristian S. Thygesen

The Semiempirical Pseudopotential Method (SEPM) has emerged as a valuable tool for accurately determining band structures, especially in the realm of low-dimensional materials. SEPM operates by utilizing atomic pseudopotentials, which are…

Materials Science · Physics 2024-06-25 Raj Kumar Paudel , Chung-Yuan Ren , Yia-Chung Chang

We present an accurate, first-principles study of the electronic structure and absorption spectrum of bulk copper within Density Functional Theory in the Local Density Approximation (DFT-LDA), including the study of intraband transitions.…

Materials Science · Physics 2009-11-07 Andrea Marini , Giovanni Onida , Rodolfo Del Sole

For materials of varying band gap, we compare energy levels of atomically localized defects calculated within a semilocal and a hybrid density-functional scheme. Since the latter scheme partially relieves the band gap problem, our study…

Materials Science · Physics 2008-07-30 Audrius Alkauskas , Peter Broqvist , Alfredo Pasquarello

The LDA-1/2 method expands Slater's half occupation technique to infinite solid state materials by introducing a self-energy potential centered at the anions to cancel the energy associated with electron-hole self-interaction. To avoid an…

Computational Physics · Physics 2016-03-07 Kan-Hao Xue , Leonardo R. C. Fonseca , Xiang-Shui Miao

We present an ab initio pseudopotential local density functional calculation for stoichiometric high-Tc cuprate YBa_2Cu_3O_7 using the plane-wave basis set. We have overcome well-known difficulties in applying pseudopotential methods to…

Condensed Matter · Physics 2009-10-22 Hanchul Kim , Jisoon Ihm

Multi-subband plasmon (MSP) modes in heavily doped InAs/GaSb broken-gap quantum wells grown via molecular beam epitaxy (MBE) are investigated. An $8$-band $\vec{k} \cdot \vec{p}$ semiclassical model accurately predicts ellipsometric…

In electronic structure calculations the optimized effective potential (OEP) is a method that treats exchange interactions exactly using a local potential within density-functional theory (DFT). We present a method using density functional…

Materials Science · Physics 2013-01-24 Tom W. Hollins , Stewart J. Clark , Keith Refson , Nikitas I. Gidopoulos

The density functional theory (DFT) approximations that are the most accurate for the calculation of band gap of bulk materials are hybrid functionals like HSE06, the MBJ potential, and the GLLB-SC potential. More recently, generalized…

The $GW$ approach of many-body perturbation theory (MBPT) has become a common tool for calculating the electronic structure of materials. However, with increasing number of published results, discrepancies between the values obtained by…

Materials Science · Physics 2016-08-03 Dmitrii Nabok , Andris Gulans , Claudia Draxl

We present an approach to calculate the electronic structure for a range of materials using the quasiparticle self-consistent GW method with vertex corrections included in the screened Coulomb interaction W. This is achieved by solving the…

Materials Science · Physics 2023-10-10 Brian Cunningham , Myrta Gruening , Dimitar Pashov , Mark van Schilfgaarde

Calculating the quasiparticle (QP) band structure of two-dimensional (2D) materials within the GW self-energy approximation has proven to be a rather demanding computational task. The main reason is the strong $\mathbf{q}$-dependence of the…

Materials Science · Physics 2016-10-12 Filip A. Rasmussen , Per S. Schmidt , Kirsten T. Winther , Kristian S. Thygesen

The $k \cdot p$ is a versatile technique that describes the semiconductor band structure in the vicinity of the bandgap. The technique can be extended to full Brillouin zone by including more coupled bands into consideration. For…

Other Condensed Matter · Physics 2007-05-23 C. Bulutay