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We discuss single adaptive measurements for the estimation of mixed quantum states of qubits. The results are compared to the optimal estimation schemes using collective measurements. We also demonstrate that the advantage of collective…

Quantum Physics · Physics 2009-11-06 Dietmar G. Fischer , Matthias Freyberger

We introduce the multistate iterative qubit coupled cluster (MS-iQCC) method, a quantum-inspired algorithm that runs efficiently on classical hardware and is designed to predict both ground and excited electronic states of molecules.…

Chemical Physics · Physics 2026-01-05 Robert A. Lang , Shashank G. Mehendale , Ilya G. Ryabinkin , Artur F. Izmaylov

Recently, it has been shown that the ground-state energy of a quantum many-body system can be written in terms of cumulants. In this paper we show that the energies of excited states can be expressed similarly. These representations are…

Condensed Matter · Physics 2007-05-23 T. Schork , P. Fulde

This paper explores the utility of the quantum phase estimation (QPE) in calculating high-energy excited states characterized by promotions of electrons occupying inner energy shells. These states have been intensively studied over the last…

The investigation of the dynamics of quantum many-body systems is a concerted effort involving computational studies of mathematical models and experimental studies of material samples. Some commonalities of the two tracks of investigation…

Strongly Correlated Electrons · Physics 2007-05-23 Gerhard Muller , Michael Karbach

We extend recently proposed variational coupled-cluster method to describe excitation states of quantum many-body interacting systems. We discuss, in general terms, both quasiparticle excitations and quasiparticle-density-wave excitations…

Other Condensed Matter · Physics 2009-11-13 Y. Xian

The prediction of electronic structure for strongly correlated molecules represents a promising application for near-term quantum computers. Significant attention has been paid to ground state wavefunctions, but excited states of molecules…

Quantum Physics · Physics 2025-01-08 Harper R. Grimsley , Francesco A. Evangelista

Calculating excited states in chemistry is crucial to provide insight into photoinduced molecular behavior beyond the ground state, enabling innovations in spectroscopy, material sciences, and drug design. While several approaches have been…

Quantum Physics · Physics 2025-10-14 Akilan Rajamani , Martin Beseda , Benjamin Lasorne , Bruno Senjean

We present a method for approximating the many-body density of states of a system of quantum identical particles, with a reduction of the computational cost by a combinatorial factor compared to the full calculation. This is carried out by…

Quantum Physics · Physics 2026-05-05 Hovan Lee , Rémi Lefèvre , Grégoire Ithier

Theoretical descriptions of excited states of molecular systems in high-energy regimes are crucial for supporting and driving many experimental efforts at light source facilities. However, capturing their complicated correlation effects…

Quenches are now routinely used in synthetic quantum systems to study a variety of fundamental effects, including ergodicity breaking, light-cone-like spreading of information, and dynamical phase transitions. It was shown recently that the…

Quantum Gases · Physics 2020-01-10 Louis Villa , Julien Despres , Laurent Sanchez-Palencia

Quantum Monte Carlo methods are first-principle approaches that approximately solve the Schr\"odinger equation stochastically. As compared to traditional quantum chemistry methods, they offer important advantages such as the ability to…

Chemical Physics · Physics 2020-02-11 Jonas Feldt , Claudia Filippi

Quantum computation can proceed solely through single-qubit measurements on an appropriate quantum state, such as the ground state of an interacting many-body system. We investigate a simple spin-lattice system based on the cluster-state…

Quantum Physics · Physics 2009-07-16 Andrew C. Doherty , Stephen D. Bartlett

The calculation of excited state energies of electronic structure Hamiltonians has many important applications, such as the calculation of optical spectra and reaction rates. While low-depth quantum algorithms, such as the variational…

Quantum Physics · Physics 2019-07-03 Oscar Higgott , Daochen Wang , Stephen Brierley

Computing excitation spectra of quantum many-body systems is a promising avenue to demonstrate the practical utility of current noisy quantum devices, especially as we move toward the ``megaquop'' regime. For this task, here we introduce a…

Quantum Physics · Physics 2026-04-16 Ji-Yao Chen , Bochen Huang , D. L. Zhou , Norbert Schuch , Chenfeng Cao , Muchun Yang

Measurement-based quantum computation has revolutionized quantum information processing, and the physical systems with which it can be implemented. One simply needs the ability to prepare a particular state, known as the cluster state, and…

Quantum Physics · Physics 2008-02-15 Dimitris G. Angelakis , Alastair Kay

Coupling a quantum many-body system to an external environment dramatically changes its dynamics and offers novel possibilities not found in closed systems. Of special interest are the properties of the steady state of such open quantum…

Quantum Physics · Physics 2021-03-30 Hendrik Weimer , Augustine Kshetrimayum , Román Orús

The methods of quantum chemistry and solid state theory to solve the many-body problem are reviewed. We start with the definitions of reduced density matrices, their properties (contraction sum rules, spectral resolutions, cumulant…

Strongly Correlated Electrons · Physics 2007-05-23 P. Ziesche , F. Tasnadi

We investigate different types of collective excitations in a quantum dot containing finite number of electrons at zero magnetic field. To estimate the excitation energies analytically we follow the energy weighted sum-rule approach. We…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 Subhasis Sinha

In classical computational chemistry, the coupled-cluster ansatz is one of the most commonly used $ab~initio$ methods, which is critically limited by its non-unitary nature. The unitary modification as an ideal solution to the problem is,…

Quantum Physics · Physics 2017-03-01 Yangchao Shen , Xiang Zhang , Shuaining Zhang , Jing-Ning Zhang , Man-Hong Yung , Kihwan Kim
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