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The BaCe0.8Y0.2O3-{\delta} proton conductor under hydration and under compressive strain has been analyzed with high pressure Raman spectroscopy and high pressure x-ray diffraction. The pressure dependent variation of the Ag and B2g bending…

A combination of first-principles density functional theory calculations and a search over structures predicts the stability of a proton-transfer modification of ammonia monohydrate with space group P4/nmm. The phase diagram is calculated…

We report our Raman studies of a new lead-free relaxor ferroelectrics, Ba0.85Ca0.15Ti0.9Zr0.1O3 (BCTZO). The Raman modes of BCTZO are compared with those of BaTi0.8Zr0.2O3 (BTZO), and BaTiO3 (BTO). Also, they are compared with the…

Materials Science · Physics 2013-05-08 Yu-Seong Seo , Jai Seok Ahn , Il-Kyoung Jeong

The structure of solid oxygen has been studied at pressures from 50 to 140~GPa using static structure search methods and molecular dynamics simulations with density functional theory and a hybrid exchange functional. Several crystalline…

Materials Science · Physics 2023-09-26 Sabri F. Elatresh , V. Askarpour , S. A. Bonev

The kinetic Monte Carlo method is applied to examine effects of hydrostatic pressure on the benzimidazolium azelate (BenAze) proton conductivity. Following the experimental indications the recently proposed model has been modified to…

Materials Science · Physics 2015-06-23 T. Masłowski , A. Drzewiński , P. Ławniczak , M. Zdanowska-Frączek , J. Ulner

The double proton transfer (DPT) reaction in hydrated formic acid dimer (FAD) is investigated at molecular-level detail. For this, a global and reactive machine learned (ML) potential energy surface (PES) is developed to run extensive (more…

Chemical Physics · Physics 2022-06-22 Kai Töpfer , Silvan Käser , Markus Meuwly

This paper investigates some of the successes and failures of density functional theory in the study of high-pressure solid hydrogen at low temperature. We calculate the phase diagram, metallization pressure, phonon spectrum, and proton…

Materials Science · Physics 2015-06-16 S. Azadi , W. M. C. Foulkes

In this study we employ Density Functional Theory (DFT) methods to investigate the surface energy barrier for electron emission (surface barrier) and thermodynamic stability of Ba and Ba-O species adsorption under conditions of high…

Materials Science · Physics 2016-07-08 Ryan M. Jacobs , John H. Booske , Dane Morgan

We employ quantum molecular dynamic simulations to investigate the behavior of benzene under shock conditions. The principal Hugoniot derived from the equation of state is determined. We compare our firs-principles results with available…

Materials Science · Physics 2015-05-14 Cong Wang , Ping Zhang

Adsorption of benzoic acid on the (110) surface of rutile, both unreconstructed and (1x2)- reconstructed ones, at saturation coverage of one benzoate per two adjacent five-coordinated Ti5c sites has been studied using DFT simulations, as…

Materials Science · Physics 2014-07-08 Xiang Zhao , David R. Bowler

Recent experiment reports that high thermal conductivity of ~1000 W/mK is observed in cubic boron arsenide crystal (BAs). In order to expand the scope of future applications, we use first-principles calculations to investigate the…

Materials Science · Physics 2018-10-29 Yanfeng Ge , Wenhui Wan , Yong Liu

$\delta$-AlOOH is of significant crystallochemical interest due to a subtle structural transition near 10 GPa from a $P2_1nm$ to a $Pnnm$ structure, the nature and origin of hydrogen disorder, the symmetrization of the O-H$\cdots$O hydrogen…

Materials Science · Physics 2021-10-14 Florian Trybel , Thomas Meier , Biao Wang , Gerd Steinle-Neumann

Measurements of temperature-dependent resistance and magnetization under hydrostatic pressures up to 2.13 GPa are reported for single-crystalline, superconducting BaBi$_3$. A temperature - pressure phase diagram is determined and the…

We use the two loop effective potential to study the first order electroweak phase transition in the minimial supersymmetric standard model. A global search of the parameter space is made to identify parameters compatible with electroweak…

High Energy Physics - Phenomenology · Physics 2009-10-31 J. M. Cline , G. D. Moore

We report the results of the X-ray diffraction study of B2O3 glass in the pressure interval up to 10 GPa in the 300-700 K temperature range, the results of in-situ volumetric measurements of the glass at pressures up to 9 GPa at room…

Disordered Systems and Neural Networks · Physics 2008-07-19 V. V. Brazhkin , Y. Katayama , K. Trachenko , O. B. Tsiok , A. G. Lyapin , Emilio Artacho , M. Dove , G. Ferlat , Y. Inamura , H. Saitoh

Yttrium substituted BaZrO3, with nominal composition BaZr0.9Y0.1O3, a ceramic proton conductor, was subject to impedance spectroscopy for temperatures 300 K < T < 715 K at mechanical pressures 1 GPa < p < 2 GPa. The activation energies Ea…

Strongly Correlated Electrons · Physics 2011-06-07 Qianli Chen , Artur Braun , Alejandro Ovalle , Cristian-Daniel Savaniu , Thomas Graule , Nikolai Bagdassarov

Density-functional theory calculations are performed to investigate hydrogen transport in the proton conductor BaSnO$_3$. Structural optimizations in the stable and saddle point configurations for transfer and reorientation allow…

Materials Science · Physics 2014-11-13 Grégory Geneste , Alistar Ottochian , Jessica Hermet , Guilhem Dezanneau

We report here the evidences of hydrogen bond symmetrization in the simplest amino acid- carboxylic acid complex, glycinium oxalate, at moderate pressures of 8 GPa using in-situ infrared and Raman spectroscopic investigations combined with…

A high statistics measurement of the pp --> ppeta reaction at an excess energy of Q = 15.5 MeV has been performed at the internal beam facility COSY-11. The stochastically cooled proton beam and the used detection system allowed to…

First-principles calculations and analysis of the thermodynamic, structural, and electronic properties of liquid SiO$_2$ characterize the bonded-to-atomic transition at 0.1--1.6 TPa and 10$^4$--10$^5$ K (1--7 eV), the high-energy-density…

Materials Science · Physics 2022-03-14 Shuai Zhang , Miguel A. Morales , Raymond Jeanloz , Marius Millot , S. X. Hu , Eva Zurek
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