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Battery electrode surfaces are generally coated with electronically insulating solid films of thickness 1-50 nm. Both electrons and Li+ can move at the electrode-surface film interface in response to the voltage, which adds complexity to…

Materials Science · Physics 2015-07-10 Kevin Leung , Andrew Leenheer

We formulate the continuum field equations and constitutive equations that govern deformation, stress, and electric current flow in a Li-ion half-cell. The model considers mass transport through the system, deformation and stress in the…

Computational Physics · Physics 2011-08-01 Allan F. Bower , Pradeep R. Guduru , Vijay A. Sethuraman

Ultrahigh rate performance of active particles used in lithium-ion battery electrodes has been revealed by single-particle measurements, which indicates a huge potential for developing high-power batteries. However, the charging/discharging…

Chemical Physics · Physics 2022-07-25 Ruoyu Xiong , Mengyuan Zhou , Longhui Li , Jia Xu , Maoyuan Li , Bo Yan , Dequn Li , Yun Zhang , Huamin Zhou

This article examines the problem of Lithium-Sulfur (Li-S) battery state estimation. Such estimation is important for the online management of this energy-dense chemistry. The literature uses equivalent circuit models (ECMs) for Li-S state…

Systems and Control · Electrical Eng. & Systems 2021-02-17 Chu Xu , Timothy Cleary , Daiwei Wang , Guoxing Li , Christopher Rahn , Donghai Wang , Rajesh Rajamani , Hosam K. Fathy

We present a physics-based model that accurately predicts the performance of Medtronic's implantable medical device battery lithium/carbon monofluoride (CF$_x$) - silver vanadium oxide (SVO) under both low-rate background monitoring and…

The applied potential governs lithium-intercalation and electrode passivation reactions in lithium ion batteries, but are challenging to calibrate in condensed phase DFT calculations. In this work, the "anode potential" of charge-neutral…

Materials Science · Physics 2015-02-03 Kevin Leung

We perform phase-field simulations of the electrodeposition process that forms dendrites within metal-anode batteries including anisotropic representation. We describe the evolution of a phase field, the lithium-ion concentration, and an…

Understanding battery degradation in electric vehicles (EVs) under real-world conditions remains a critical yet under-explored area of research. Central to this investigation is the challenge of estimating the specific degradation modes in…

Optimization and Control · Mathematics 2024-05-20 Raja Abhishek Appana , Faissal El Idrissi , Prashanth Ramesh , Marcello Canova , Chun Yong Kang , Kimoon Um

Controlling nanostructure from molecular, crystal lattice to the electrode level remains as arts in practice, where nucleation and growth of the crystals still require more fundamental understanding and precise control to shape the…

Battery short-term electrical impedance behavior varies between linear, linear time-varying, or nonlinear at different operating conditions. Data-based electrical impedance modeling techniques often model the battery as a linear…

Systems and Control · Computer Science 2018-05-17 Rishi Relan , Koen Tiels , Jean-Marc Timmermans , Johan Schoukens

The degradation process of lithium-ion batteries is intricately linked to their entire lifecycle as power sources and energy storage devices, encompassing aspects such as performance delivery and cycling utilization. Consequently, the…

Machine Learning · Computer Science 2023-08-16 Yue Xiang , Bo Jiang , Haifeng Dai

We present a mechanistic theory for predicting void evolution in the Li metal electrode during the charge and discharge of all-solid-state battery cells. A phase field formulation is developed to model vacancy annihilation and nucleation,…

Materials Science · Physics 2022-08-31 Y. Zhao , R. Wang , E. Martínez-Pañeda

For many practical applications, fully coupled three-dimensional models describing the behaviour of lithium-ion pouch cells are too computationally expensive. However, owing to the small aspect ratio of typical pouch cell designs, such…

Computational Physics · Physics 2020-08-11 Scott G. Marquis , Robert Timms , Valentin Sulzer , Colin P. Please , S. Jon Chapman

We have investigated the lithium capacity of the 2H phase of niobium sulphide (NbS2) using density functional theory calculations and experiments. Theoretically, this material is found to allow the intercalation of a double layer of Li in…

We consider the mathematical treatment of a system of nonlinear partial differential equations based on a model, proposed in 1972 by J. Newman, in which the coupling between the Lithium concentration, the phase potentials and temperature in…

Analysis of PDEs · Mathematics 2022-02-23 Jesús Ildefonso Díaz , David Gómez-Castro , Angel Manuel Ramos

Battery thermal management systems (BTMSs) are critical for efficient and safe operation of lithium-ion batteries (LIBs), especially for fast charging/discharging applications that generate significant heating within the cell. Forced…

Fluid Dynamics · Physics 2025-02-04 Piyush Mani Tripathi , Amy M. Marconnet

This paper presents findings on dynamic cell modeling for state-of-charge (SOC) estimation in an autonomous electric vehicle (AEV). The studied cells are Lithium-Ion Polymer-based with a nominal capacity of around 8Ah, optimized for…

Systems and Control · Electrical Eng. & Systems 2023-06-21 Qasim Ajao , Lanre Sadeeq

We introduce "bond-counting" potentials, which provide an elementary description of covalent bonding. These simplistic potentials are intended for studies of the mechanisms behind a variety of phase transitions in elemental melts, including…

Chemical Physics · Physics 2021-04-09 Shlomi Matityahu , Nathan Argaman

The use of floating bipolar electrodes in copper electro-winning cells represents an emerging technology that promises economic and operational impacts. This article presents a computational tool designed for the simulation and analysis of…

Graphics · Computer Science 2026-01-08 César Mena , Ricardo Sánchez , Lautaro Salazar

Alkali metal ion batteries, and in particular Li-ion batteries, have become a key technology for current and future energy storage, already nowadays powering many devices of our daily lives. Due to the inherent complexity of batteries and…

Materials Science · Physics 2021-12-14 Holger Euchner , Axel Groß