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Molecular dynamics simulation methods are used to study the folding of polymer chains into packed cubic states. The polymer model, based on a chain of linked sites moving in the continuum, includes both excluded volume and torsional…

Soft Condensed Matter · Physics 2009-11-10 D. C. Rapaport

Mechanically bonded membranes of interlocked ring polymers are a significant generalization of conventional elastic sheets, where connectivity is provided by covalent bonding, and represent a promising class of topological meta-materials.…

Soft Condensed Matter · Physics 2024-06-21 Juan Luengo-Márquez , Salvatore Assenza , Cristian Micheletti

We investigate experimentally the distribution of configurations of a ring with an elementary topological constraint, a ``figure-8'' twist. Using vibrated granular chains, which permit controlled preparation and direct observation of such a…

Soft Condensed Matter · Physics 2015-07-22 M. B. Hastings , Z. A. Daya , E. Ben-Naim , R. E. Ecke

The conformations of topologically constrained double-folded ring polymers can be described as wrappings of randomly branched primitive trees. We extend previous work on the tree statistics under different (solvent) conditions to explore…

Soft Condensed Matter · Physics 2019-01-23 Angelo Rosa , Ralf Everaers

The non-equilibrium structural and dynamical properties of a flexible polymer tethered to a reflecting wall and subject to oscillatory linear flow are studied by numerical simulations. Polymer is confined in two dimensions and is modeled as…

Soft Condensed Matter · Physics 2024-07-30 A. Lamura

We model a macromolecule as an infinitely long Gaussian semi-flexible polymer chain and the conformations of the chain were realized in the nano cube using a cubic lattice. A modified version of the recursion relations is used to calculate…

Soft Condensed Matter · Physics 2022-01-11 Pramod Kumar Mishra

Ladder polymers, known for their rigid, ladder-like structures, exhibit exceptional thermal stability and mechanical strength, positioning them as candidates for advanced applications. However, accurately determining their structure from…

Soft Condensed Matter · Physics 2025-05-23 Lijie Ding , Chi-Huan Tung , Zhiqiang Cao , Zekun Ye , Xiaodan Gu , Yan Xia , Wei-Ren Chen , Changwoo Do

In the first part of this work a summary is provided of some recent experiments and theoretical results which are relevant in the research of systems of polymer rings in nontrivial topological conformations. Next, some advances in modeling…

Soft Condensed Matter · Physics 2014-02-04 Yani Zhao , Franco Ferrari

We investigate the internal structure of a polymer during collapse from an expanded coil to a compact globule. Collapse is more probable in local regions of high curvature, so a smoothing of the fractal polymer structure occurs that…

Soft Condensed Matter · Physics 2008-11-07 G. E. Crooks , B. Ostrovsky , Y. Bar-Yam

We used a coarse-grained model to study the geometric and dynamic properties of flexible entangled polymer chains dissolved in explicit athermal solvents. Our simulations successfully reproduced the geometrical properties including the…

Soft Condensed Matter · Physics 2023-06-16 Jiayi Wang , Ping Gao

Extensive molecular simulations are applied to characterize the equilibrium dynamics, entanglement topology, and nonlinear extensional rheology of symmetric ring-linear polymer blends with systematically varied ring fraction $\phi_R$.…

Soft Condensed Matter · Physics 2021-12-15 Thomas C. O'Connor , Ting Ge , Gary S. Grest

Monte Carlo computer simulations are used to study the segregation behaviour of two polymers under cylindrical confinement. Using a multiple-histogram method, the conformational free energy, F, of the polymers was measured as a function of…

Soft Condensed Matter · Physics 2018-05-24 James M. Polson , Deanna R. -M. Kerry

Using molecular dynamics simulations we examine the dynamics of a family of model polymers with varying chain length and torsional potential barriers. We focus on features of the dynamics of polymers that are seen experimentally but absent…

Soft Condensed Matter · Physics 2019-06-11 Daniel Fragiadakis , C. Michael Roland

The structure of polyelectrolytes is highly sensitive to small changes in the interactions between its monomers. In particular, interactions mediated by counterions play a significant role, and are affected by both specific molecular…

Soft Condensed Matter · Physics 2020-02-03 Pauline Bacle , Marie Jardat , Virginie Marry , Guillaume Mériguet , Guillaume Batôt , Vincent Dahirel

Obtaining reliable estimates of the statistical properties of complex macromolecules by computer simulation is a task that requires high computational effort as well as the development of highly efficient simulation algorithms. We present…

Soft Condensed Matter · Physics 2015-05-28 Hsiao-Ping Hsu , Wolfgang Paul

We analyze the statistics of loops formation in $f$-branched star polymers in an environment with structural defects, correlated at large distances $r$ according to a power law $\sim r^{-a}$. Applying the direct polymer renormalization…

Soft Condensed Matter · Physics 2017-10-04 K. Haydukivska , V. Blavatska

We present the exact solutions of various directed walk models of polymers confined to a slit and interacting with the walls of the slit via an attractive potential. We consider three geometric constraints on the ends of the polymer and…

Statistical Mechanics · Physics 2009-11-11 R Brak , A L Owczarek , A Rechnitzer , S G Whittington

This study focuses on comparing the individual polymer chain dynamics in an entangled polymeric liquid under different shear and extension rates. Polymer chains under various shear rates and extension rates were simulated using a…

Chemical Physics · Physics 2021-01-15 Behrouz Behdani , Tong Mou , Cody Spratt , Slava Butcovich , Ryan Gettler , Joontaek Park

Various authors have invoked discretized fractional Brownian (fBm) motion as a model for chain polymers with long range interaction of monomers along the chain. We show that for these, in contrast to the Brownian case, linear forces are…

Mathematical Physics · Physics 2019-07-24 Wolfgang Bock , Jinky Bornales , Ludwig Streit

Nanoscale and microscale confinement of biopolymers naturally occurs in cells and has been recently achieved in artificial structures designed for nanotechnological applications. Here, we present an extensive theoretical investigation of…

Soft Condensed Matter · Physics 2007-06-13 Frederik Wagner , Gianluca Lattanzi , Erwin Frey