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The lifetime $\tau$ of an isothermal and purely diffusively dissolving droplet in a host liquid scales as $\tau \sim R_0^2$ with its initial radius $R_0$ [Langmuir, Phys. Rev. 12, 368 (1919)]. For a droplet dissolving due to natural…

Fluid Dynamics · Physics 2022-02-15 Binglin Zeng , Yuliang Wang , Christian Diddens , Harold J. W. Zandvliet , Detlef Lohse

The dissolution process of small (initial (equivalent) radius $R_0 < 1$ mm) long-chain alcohol (of various types) sessile droplets in water is studied, disentangling diffusive and convective contributions. The latter can arise for high…

'A basic and basically unsolved problem in fluid dynamics is to determine the evolution of rising bubbles and falling drops of one miscible liquid in another' [1]. Here, we address this important literature gap and present the first theory…

Fluid Dynamics · Physics 2023-05-11 Jan Martin Nordbotten , Endre Joachim Lerheim Mossige

The Marangoni contraction of sessile droplets occurs when a binary mixture of volatile liquids is placed on a high-energy surface. Although the surface is wetted completely by the mixture and its components, a quasi-stationary non-vanishing…

Fluid Dynamics · Physics 2022-02-01 Olinka Ramirez-Soto , Stefan Karpitschka

Multicomponent liquid drops in a host liquid are very relevant in various technological applications. Their dissolution or growth dynamics is complex. Differences in solubility between the drop components combined with the solutal Marangoni…

When a mixture of propylene glycol and water is deposited on a clean glass slide, it forms a droplet of a given apparent contact angle rather than spreading as one would expect on such a high-energy surface. The droplet is stabilized by a…

Soft Condensed Matter · Physics 2017-12-04 Adrien Benusiglio , Nate Cira , Manu Prakash

We report here a peculiar dynamically ordered state of clustering droplets of a mixture of organic solvent. There droplets are driven by the solutal Marangoni effect on the surface of aqueous surfactant solution. They form temporal ring…

Soft Condensed Matter · Physics 2017-06-02 Shinpei Tanaka , Takeshi Kano

For a small sessile or pendant droplet it is generally assumed that gravity does not play any role once the Bond number is small. This is even assumed for evaporating binary sessile or pendant droplets, in which convective flows can be…

Fluid Dynamics · Physics 2020-05-29 Christian Diddens , Yaxing Li , Detlef Lohse

We experimentally investigate the dissolution of microscale sessile alcohol droplets in water under the influence of impermeable vertical confinement. The introduction of confinement suppresses the mass transport from the droplet to bulk…

Fluid Dynamics · Physics 2021-01-13 Saptarshi Basu , D. Chaitanya Kumar Rao , Ankur Chattopadhyay , Joita Chakraborty

The transport and aggregation of particles in suspensions is an important process in many physicochemical and industrial processes. In this work, we study the transport of particles in an evaporating binary droplet. Surprisingly, the…

When an evaporating water droplet is deposited on a thermally conductive substrate, the minimum temperature will be at the apex due to evaporative cooling. Consequently, density and surface tension gradients emerge within the droplet and at…

In this paper, the evaporation of neighbouring multi-component droplets or rivulets - often found in applications such as inkjet printing, spray cooling, and pesticide delivery - is studied numerically and theoretically. The proximity…

Fluid Dynamics · Physics 2026-04-01 Pim J. Dekker , Duarte Rocha , Christian Diddens , Detlef Lohse

Deformed droplets are ubiquitous in various industrial applications, such as inkjet printing, lab-on-a-chip devices, and spray cooling, and can fundamentally affect the involved applications both favorably and unfavorably. Here, we employ…

The evaporation of a binary sessile ethanol-water droplet on an inclined substrate is studied experimentally just below the critical sliding angles for different substrate temperatures. A customized goniometer equipped with a CMOS camera…

The evaporation of multi-component droplets is relevant to various applications but challenging to study due to the complex physicochemical dynamics. Recently, Li (2018) reported evaporation-triggered segregation in 1,2-hexanediol-water…

Fluid Dynamics · Physics 2020-08-26 Yaxing Li , Christian Diddens , Tim Segers , Herman Wijshoff , Michel Versluis , Detlef Lohse

Droplet evaporation of multicomponent droplets is essential for various physiochemical applications, e.g. in inkjet printing, spray cooling and microfabrication. In this work, we observe and study phase segregation of an evaporating sessile…

We study theoretically internal flows in a small oblate droplet suspended on the circular frame. Marangoni convection arises due to a vertical temperature gradient across the drop and is driven by the surface tension variations at the free…

Fluid Dynamics · Physics 2023-07-26 M. A. Shishkin , K. S. Kolegov , S. A. Pikin , B. I. Ostrovskii , E. S. Pikina

Experiments indicate that microdroplets undergoing micellar solubilization in the bulk of surfactant solution may excite Marangoni flows and self-propel spontaneously. Surprisingly, self-propulsion emerges even when the critical micelle…

Fluid Dynamics · Physics 2020-06-09 Matvey Morozov

For an immiscible oil drop immersed in a stably stratified ethanol-water mixture, a downwards solutal Marangoni flow is generated on the surface of the drop, owing to the concentration gradient, and the resulting propulsion competes against…

Fluid Dynamics · Physics 2021-12-06 Yanshen Li , Jochem G. Meijer , Detlef Lohse

The dissolution of a body into quiescent water leads to density stratifications at the interfaces that drive buoyant flows. Where the stratification is unstable, the flow destabilizes into convective solute plumes. By analogy with the…

Fluid Dynamics · Physics 2020-06-02 Caroline Cohen , Michael Berhanu , Julien Derr , Sylvain Courrech du Pont
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