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The junction of a scanning tunneling microscope (STM) operating in the tunneling regime was irradiated with femtosecond laser pulses. A photo-excited hot electron in the STM tip resonantly tunnels into an excited state of a single molecule…

Mesoscale and Nanoscale Physics · Physics 2015-05-19 Shiwei Wu , Wilson Ho

Atomically thin layered van der Waals heterostructures feature exotic and emergent optoelectronic properties. With growing interest in these novel quantum materials, the microscopic understanding of fundamental interfacial coupling…

Understanding the interaction of kilojoule, picosecond laser pulse with long-scale length preplasma or homogeneous near critical density (NCD) plasma is crucial for guiding experiments at national short-pulse laser facilities. Using full…

Plasma Physics · Physics 2022-10-12 X. F. Shen , A. Pukhov , O. N. Rosmej , N. E. Andreev

Manipulating spin in antiferromagnetic (AFM) materials has great potential in AFM opto-spintronics. Laser pulses can induce a transient ferromagnetic (FM) state in AFM metallic systems, but have never been proven in two-dimensional (2D) AFM…

Materials Science · Physics 2022-03-11 Shuo Li , Junjie He , Thomas Frauenheim

We show theoretically that coherent light can be completely absorbed in a two-dimensional or three-dimensional metallic nanostructure by matching the frequency and field pattern of an incident wave to that of a localized surface plasmon…

Optics · Physics 2015-05-30 Heeso Noh , Yidong Chong , A. Douglas Stone , Hui Cao

We present an experimental observation of non-linear up- and down-converted optical luminescence of graphene and thin graphite subject to picosecond infrared laser pulses. We show that the excitation yields to a high density electron-hole…

Materials Science · Physics 2010-10-01 Rainer J. Stoehr , Roman Kolesov , Jens Pflaum , Joerg Wrachtrup

All-organic-based photovoltaic solar cells have attracted considerable attention because of their low-cost processing and short energy payback time. In such systems the primary dissociation of an optical excitation into a pair of…

Two-dimensional (2D) nanoparticle films are a new class of materials with interesting physical properties and applications ranging from nanoelectronics to sensing and photonics. The importance of conducting nanoparticle films makes the…

Materials Science · Physics 2022-04-12 Lianhua Zhang , Jian Chen , Fei Liu , Zhengyang Du , Yilun Jiang , Min Han , Guanghou Wang

The theory of energy transfer dynamics of a pair of donor and acceptor molecules located in the plasmonic hot spots is developed by means of the master equation approach and the electromagnetic Green's tensor technique. A nonlocal effect…

Optics · Physics 2017-12-29 Jun Ren , Tian Chen , Bo Wang , Xiangdong Zhang

Understanding the stress transfer mechanisms from a polymer matrix to two-dimensional reinforcements is essential for the preparation of high performance nanocomposites. In this study, the interfacial stress transfer from a flexible polymer…

Materials Science · Physics 2022-10-19 Ming Dong , Robert J. Young , David J. Dunstan , Dimitrios G. Papageorgiou

Shift current---a photocurrent induced by light irradiating noncentrosymmetric materials in the absence of any bias voltage or built-in electric field---is one of the mechanisms of the so-called bulk photovoltaic effect. It has been…

Mesoscale and Nanoscale Physics · Physics 2019-03-28 U. Bajpai , B. S. Popescu , P. Plechac , B. K. Nikolic , L. E. F. Foa Torres , H. Ishizuka , N. Nagaosa

The design of low-dimensional organic-inorganic interfaces for the next generation of opto-electronic applications requires an in-depth understanding of the microscopic mechanisms ruling electronic interactions in these systems. In this…

The interest in monomolecular films as electric conductors arises from the search for innovative materials. The utility of non-covalently bonded films is limited because they are mechanically unstable and consist of poorly connected…

Materials Science · Physics 2007-05-23 Dmitry Zaslavsky , Andrei Pakoulev , Vladimir Burtman

The strong light-matter interaction in monolayer transition metal dichalcogenides (TMDs) is promising for nanoscale optoelectronics with their direct band gap nature and the ultra-fast radiative decay of the strongly bound excitons these…

Mesoscale and Nanoscale Physics · Physics 2019-05-27 Medha Dandu , Rabindra Biswas , Sarthak Das , Sangeeth Kallatt , Suman Chatterjee , Mehak Mahajan , Varun Raghunathan , Kausik Majumdar

We investigate the relaxation dynamics of photogenerated carriers in silicon nanowires consisting of a crystalline core and a surrounding amorphous shell, using femtosecond time-resolved differential reflectivity and transmission…

Mesoscale and Nanoscale Physics · Physics 2012-12-24 Sunil Kumar , M. Khorasaninejad , M. M. Adachi , K. S. Karim , S. S. Saini , A. K. Sood

Singly ionized nitrogen molecules in ambient air pumped by near-infrared femtosecond laser give rise to superradiant emission. Here we demonstrate coherent control of this superradiance by injecting a pair of resonant seeding pulses inside…

Semiconducting monolayer of 2D material are able to concatenate multiple interesting properties into a single component. Here, by combining opto-mechanical and electronic measurements, we demonstrate the presence of a partial 2H-1T phase…

Photosystem II (PSII) reaction center is a unique protein-chromophore complex that is capable of efficiently separating electronic charges across the membrane after photoexcitation. In the PSII reaction center, the primary energy- and…

The rate at which matter emits or absorbs light can be modified by its environment, as dramatically exemplified by the widely-studied phenomenon of superradiance. The reverse process, superabsorption, is harder to demonstrate due to the…

We report a strong nonlinear optical response of 2D MoSe$_2$ nanoflakes (NFs) through spatial self-phase modulation (SSPM) and cross-phase modulation (XPM) induced by nonlocal coherent light-matter interactions. The coherent interaction of…

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