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We present a new linear scaling method for the energy minimization step of semiempirical and first-principles Hartree-Fock and Kohn-Sham calculations. It is based on the self-consistent calculation of the optimum localized orbitals of any…

Materials Science · Physics 2009-11-10 Luis Seijo , Zoila Barandiaran

We present a low-complexity algorithm to calculate the correlation energy of periodic systems in second-order M\o ller-Plesset perturbation theory (MP2). In contrast to previous approximation-free MP2 codes, our implementation possesses a…

Chemical Physics · Physics 2017-03-16 Tobias Schäfer , Benjamin Ramberger , Georg Kresse

An efficient technique to generate ensembles of spins that are highly polarized by external magnetic fields is the Holy Grail in Nuclear Magnetic Resonance (NMR) spectroscopy. Since spin-half nuclei have steady-state polarization biases…

Quantum Physics · Physics 2007-05-23 Jose M. Fernandez , Seth Lloyd , Tal Mor , Vwani Roychowdhury

This paper aims at developing a clustering approach with spectral images directly from CASSI compressive measurements. The proposed clustering method first assumes that compressed measurements lie in the union of multiple low-dimensional…

Image and Video Processing · Electrical Eng. & Systems 2019-11-06 Jianchen Zhu , Tong Zhang , Shengjie Zhao , Carlos Hinojosa , Zengli Liu , Gonzalo R. Arce

Sparse linear prediction methods suffer from decreased prediction accuracy when the predictor variables have cluster structure (e.g. there are highly correlated groups of variables). To improve prediction accuracy, various methods have been…

Machine Learning · Statistics 2022-02-03 Rebecca Marion , Johannes Lederer , Bernadette Govaerts , Rainer von Sachs

While coupled cluster theory accurately models weakly correlated quantum systems, it often fails in the presence of strong correlations where the standard mean-field picture is qualitatively incorrect. In many cases, these failures can be…

Nuclear Theory · Physics 2020-05-14 Y. Qiu , T. M. Henderson , T. Duguet , G. E. Scuseria

We consider a new formulation of the stochastic coupled cluster method in terms of the similarity transformed Hamiltonian. We show that improvement in the granularity with which the wavefunction is represented results in a reduction in the…

Chemical Physics · Physics 2016-02-02 Ruth S. T. Franklin , James S. Spencer , Alberto Zoccante , Alex J. W. Thom

An approach to special relativistic dynamics using the language of spinors and twistors is presented. Exploiting the natural conformally invariant symplectic structure of the twistor space, a model is constructed which describes a…

High Energy Physics - Theory · Physics 2014-11-18 Andreas Bette

Downfolding coupled cluster (CC) techniques have recently been introduced into quantum chemistry as a tool for the dimensionality reduction of the many-body quantum problem. As opposed to earlier formulations in physics and chemistry based…

Quantum Physics · Physics 2022-03-23 Nicholas P. Bauman , Karol Kowalski

A differential cluster variation method (DCVM) is proposed for analysis of spinoidal decomposition in alloys. In this method, lattice symmetry operations in the presence of an infinitesimal composition gradient are utilized to deduce the…

Materials Science · Physics 2016-08-31 Zhi-Rong Liu , Huajian Gao

Quantum chemical methods dealing with challenging systems while retaining low computational costs have attracted attention. In particular, many efforts have been devoted to developing new methods based on the second-order perturbation that…

Chemical Physics · Physics 2023-10-30 Nhan Tri Tran , Hoang Thanh Nguyen , Lan Nguyen Tran

Subspace clustering is to find underlying low-dimensional subspaces and cluster the data points correctly. In this paper, we propose a novel multi-view subspace clustering method. Most existing methods suffer from two critical issues.…

Artificial Intelligence · Computer Science 2022-05-24 Mengyuan Zhang , Kai Liu

In electronic structure theory, restricted single-reference coupled cluster (CC) captures weak correlation but fails catastrophically under strong correlation. Spin-projected unrestricted Hartree-Fock (SUHF), on the other hand, misses weak…

Chemical Physics · Physics 2017-11-22 John A. Gomez , Thomas M. Henderson , Gustavo E. Scuseria

We propose a symmetric low-rank representation (SLRR) method for subspace clustering, which assumes that a data set is approximately drawn from the union of multiple subspaces. The proposed technique can reveal the membership of multiple…

Computer Vision and Pattern Recognition · Computer Science 2015-11-24 Jie Chen , Haixian Zhang , Hua Mao , Yongsheng Sang , Zhang Yi

The relativistic four-quark equations are found in the framework of the dispersion relation technique. The solutions of these equations using the method based on the extraction of leading singularities of the amplitudes are obtained. The…

High Energy Physics - Phenomenology · Physics 2009-10-31 S. M. Gerasyuta , V. I. Kochkin

When utilizing a cluster decomposible relativistic scattering formalism, it is most convenient that the covariant field equations take on a linear form with respect to the energy and momentum dispersion on the fields in the manner given by…

Mathematical Physics · Physics 2007-05-23 James Lindesay

Spectral clustering is one of the most popular clustering methods. However, the high computational cost due to the involved eigen-decomposition procedure can immediately hinder its applications in large-scale tasks. In this paper we use…

Machine Learning · Computer Science 2023-01-24 Yongyu Wang

This paper presents the derivation of a kinetic-balance condition for explicitly correlated basis functions employed in semi-classical relativistic calculations. Such a condition is important to ensure variational stability in algorithms…

Chemical Physics · Physics 2015-10-26 Benjamin Simmen , Edit Mátyus , Markus Reiher

The recent quantum information boom has effected a resurgence of interest in unitary coupled cluster (UCC) theory. Our group's interest in local energy landscapes of unitary ans\"atze prompted us to investigate the classical approach of…

Chemical Physics · Physics 2022-11-01 Harper R. Grimsley , Nicholas J. Mayhall

A low-rank transformation learning framework for subspace clustering and classification is here proposed. Many high-dimensional data, such as face images and motion sequences, approximately lie in a union of low-dimensional subspaces. The…

Computer Vision and Pattern Recognition · Computer Science 2014-03-11 Qiang Qiu , Guillermo Sapiro
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