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High harmonic generation(HHG) is one of the most commonly studied nonlinear optical phenomena, originating in the ultrafast dynamics of electrons in atomic gasses and semiconductors. It has attracted much attention because of its…

Optics · Physics 2023-09-08 Akira Kofuji , Robert Peters

We theoretically investigate correlated electron dynamics in high-harmonic generation (HHG), using all-electron \emph{ab initio} simulations for three-dimensional real alkali-metal atoms. The resulting harmonic spectra exhibit a plateau…

Atomic Physics · Physics 2019-04-10 Yang Li , Takeshi Sato , Kenichi L. Ishikawa

We show how many-body effects associated with background spin dynamics control the high-harmonic generation (HHG) in Mott insulators by analyzing the two-leg ladder Hubbard model. Spin dynamics activated by the interchain hopping $t_y$…

Strongly Correlated Electrons · Physics 2025-03-19 Yuta Murakami , Thomas Hansen , Shintaro Takayoshi , Lars Bojer Madsen , Philipp Werner

We study high-order harmonic generation (HHG) resulting from the illumination of plasmonic nanostructures with a short laser pulse. We show that both the inhomogeneities of the local electric field and the confinement of the electron motion…

Atomic Physics · Physics 2012-04-27 M. F. Ciappina , Srdjan S. Acimovic , T. Shaaran , J. Biegert , R. Quidant , M. Lewenstein

High harmonic generation (HHG) from semiconductors and insulators has become a very active area of research due to its great potential for developing compact HHG devices. Here we show that by growing monolayers (ML) of insulators on…

Atomic Physics · Physics 2016-12-28 Néstor F. Aguirre , Fernando Martín

Electronic structure and electron correlations of the Hubbard model on the Beta-Mn lattice have been investigated on the basis of the momentum dependent local ansatz wavefunction method. It is found that the electrons on the Beta-Mn lattice…

Strongly Correlated Electrons · Physics 2022-02-09 Yoshiro Kakehashi

The spectra produced by high-harmonic generation (HHG) typically exhibit well-defined peaks at odd integers times the laser frequency. However, in recent investigations of HHG from correlated materials, spectra exhibit signals at noninteger…

Atomic Physics · Physics 2024-06-05 Christian Saugbjerg Lange , Thomas Hansen , Lars Bojer Madsen

High-harmonic generation (HHG) involves the up-conversion of a high-intensity driving field into its harmonic orders. This process is intrinsically non-classical, requiring from quantum mechanics for a complete explanation as, under…

Quantum Physics · Physics 2024-09-25 Javier Rivera-Dean

Exciton effects on conjugated polymers and the resulting optical nonlinearities are investigated in soliton lattice states. We use the Su-Schrieffer-Heeger model with long-range Coulomb interactions for electrons. The third-harmonic…

Condensed Matter · Physics 2008-02-03 Kikuo Harigaya

We experimentally observe longer than long trajectory influence in high order harmonic generation (HHG) by varying the peak intensity of the driving laser field through either direct attenuation, or by chirping the laser pulse. Using a…

We perform a detailed analysis of high-order harmonic generation in diatomic molecules within the strong-field approximation, with emphasis on quantum-interference effects. Specifically, we investigate how the different types of electron…

Atomic Physics · Physics 2011-11-10 C. Figueira de Morisson Faria

High harmonic generation (HHG) provides a flexible framework for the development of coherent light sources in the extreme-ultraviolet and soft x-ray regimes. However it suffers from low conversion efficiencies as the control of the HHG…

Optics · Physics 2014-09-16 Alberto Castro , Angel Rubio , E. K. U. Gross

We consider noninteracting electrons coupled to laser fields, and study perturbatively the effects of the lattice potential involving disorder on the harmonic components of the electric current, which are sources of high-order harmonic…

Disordered Systems and Neural Networks · Physics 2020-01-15 Koki Chinzei , Tatsuhiko N. Ikeda

We reveal the crucial effect of strong spin-charge coupling on high-harmonic generation (HHG) in Mott insulators. In a system with antiferromagnetic correlations, the HHG signal is drastically enhanced with decreasing temperature, even…

Strongly Correlated Electrons · Physics 2022-10-06 Yuta Murakami , Kento Uchida , Akihisa Koga , Koichiro Tanaka , Philipp Werner

An accurate analytic model describing high-harmonic generation (HHG) in solids is derived. Extensive first-principles simulations within a time-dependent density-functional framework corroborate the conclusions of the model. Our results…

It is shown that electron backscattering can enhance high-harmonic generation in periodic systems with broken translational symmetry. Paradigmatically, we derive for a finite chain of atoms the harmonic cutoff due to electrons backscattered…

Atomic Physics · Physics 2022-04-13 Chuan Yu , Ulf Saalmann , Jan M. Rost

Since the discovery of high-order harmonic generation (HHG) in solids, much effort has been devoted to understanding its generation mechanism and both interband and intraband transitions are known to be essential. However, intraband…

We investigate the effect of dynamic electron correlation on high-harmonic generation in helium atoms using intense visible light (\lambda=390nm). Two complementary approaches are used which account for correlation in an approximate manner:…

Quantum Physics · Physics 2009-05-21 G. A. McKenna , R. Nepstad , J. F. McCann , D. Dundas

In this paper, we investigate the effects of full electronic correlation on the high harmonic generation in the helium atom subjected to laser pulses of extremely high intensity. To do this, we perform real-time propagations of the helium…

Chemical Physics · Physics 2022-05-18 Aleksander P. Woźniak , Michał Przybytek , Maciej Lewenstein , Robert Moszyński

We present a semiclassical model for plasmon-enhanced high-harmonic generation (HHG) in the vicinity of metal nanostructures. We show that both the inhomogeneity of the enhanced local fields and electron absorption by the metal surface play…

Optics · Physics 2015-07-29 A. Husakou , S. -J. Im , J. Herrmann