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Using the finite-element discrete variable representation of the nonequilibrium Green's function (NEGF) we extend previous work [K.~Balzer et al., Phys. Rev. A \textbf{81}, 022510 (2010)] to nonequilibrium situations and compute---from the…

Atomic Physics · Physics 2010-11-29 K. Balzer , S. Bauch , M. Bonitz

We present a real-time second-order Green's function (GF) method for computing excited states in molecules and nanostructures, with a computational scaling of $O(N_{\rm e}^3$), where $N_{\rm e}$ is the number of electrons. The cubic scaling…

Chemical Physics · Physics 2024-01-29 Leopoldo Mejía , Jia Yin , David R. Reichman , Roi Baer , Chao Yang , Eran Rabani

Despite recent advances, systematic quantitative treatment of the electron correlation problem in extended systems remains a formidable task. Systematically improvable Green's function methods capable of quantitatively describing weak and…

Chemical Physics · Physics 2016-11-15 Alexander A. Rusakov , Dominika Zgid

In recent years, Green's function methods have garnered considerable interest due to their ability to target both charged and neutral excitations. Among them, the well-established $GW$ approximation provides accurate ionization potentials…

Chemical Physics · Physics 2023-08-31 Enzo Monino , Pierre-François Loos

We report an implementation of self-consistent Green's function many-body theory within a second-order approximation (GF2) for application with molecular systems. This is done by iterative solution of the Dyson equation expressed in matrix…

Chemical Physics · Physics 2016-11-15 Jordan J. Phillips , Dominika Zgid

We have developed a time propagation scheme for the Kadanoff-Baym equations for general inhomogeneous systems. These equations describe the time evolution of the nonequilibrium Green function for interacting many-body systems in the…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 Adrian Stan , Nils Erik Dahlen , Robert van Leeuwen

In the nonequilibrium Green's function approach, the approximation of the correlation self-energy at the second-Born level is of particular interest, since it allows for a maximal speed-up in computational scaling when used together with…

Computational Physics · Physics 2019-11-11 Riku Tuovinen , Fabio Covito , Michael A. Sentef

We have implemented time-propagation of the non-equilibrium Green function for atoms and molecules, by solving the Kadanoff-Baym equations within a conserving self-energy approximation. We here demonstrate the usefulnes of time-propagation…

Materials Science · Physics 2007-05-23 Nils Erik Dahlen , Robert van Leeuwen

The theory of Nonequilibrium Green functions (NEGF) has seen a rapid development over the recent three decades. Applications include diverse correlated many-body systems in and out of equilibrium. Very good agreement with experiments and…

Strongly Correlated Electrons · Physics 2026-04-02 Michael Bonitz , Jan-Philip Joost , Christopher Makait , Erik Schroedter , Tim Karsberger , Karsten Balzer

The time-dependent variational principle proposed by Balian and Veneroni is used to provide the best approximation to the generating functional for multi-time Green's functions of a set of (bosonic) observables $Q_{\mu)$. By suitably…

High Energy Physics - Theory · Physics 2016-09-06 Mohamed Benarous

Using the Kadanoff-Baym non-equilibrium Green's function formalism, we derive kinetic equations for the non-condensate atoms at finite temperatures which include the effect of binary collisions between atoms. The effect of collisions is…

Condensed Matter · Physics 2017-08-23 Milena Imamovic-Tomasovic , Allan Griffin

The second-order Green's function method (GF2) was shown recently to be an accurate self-consistent approach for electronic structure of correlated systems since the self-energy accounts for both the weak and some of the strong correlation.…

Chemical Physics · Physics 2016-03-31 Daniel Neuhauser , Roi Baer , Dominika Zgid

The non-equilibrium Green's function gives access to one-body observables for quantum systems. Of particular interest are quantities such as density, currents, and absorption spectra which are important for interpreting experimental results…

Computational Physics · Physics 2025-05-02 Thomas Blommel , David J. Gardner , Carol S. Woodward , Emanuel Gull

We present an approach to renormalized second-order Green's function perturbation theory (GF2) which avoids all dependency on continuous variables, grids or explicit Green's functions, and is instead formulated entirely in terms of static…

Chemical Physics · Physics 2020-06-26 Oliver J. Backhouse , Max Nusspickel , George H. Booth

For a minimal Hubbard-type system at different interaction strengths U, we investigate the density-response for an excitation beyond the linear regime using the generalized Kadanoff-Baym ansatz (GKBA) and the second Born (2B) approximation.…

Strongly Correlated Electrons · Physics 2015-06-12 K. Balzer , S. Hermanns , M. Bonitz

Linear density response functions are calculated for symmetric nuclear matter of normal density by time-evolving two-time Green's functions in real time. Of particular interest is the effect of correlations. The system is therefore…

Nuclear Theory · Physics 2016-05-04 H. S. Köhler , N. H. Kwong

Real-time Green's function simulations of molecular junctions (open quantum systems) are typically performed by solving the Kadanoff-Baym equations (KBE). The KBE, however, impose a serious limitation on the maximum propagation time due to…

Mesoscale and Nanoscale Physics · Physics 2015-06-17 S. Latini , E. Perfetto , A. -M. Uimonen , R. van Leeuwen , G. Stefanucci

A nonequilibrium Green's functions (NEGF) approach for spatially inhomogeneous, strongly correlated artificial atoms is presented and applied to compute the time-dependent properties while starting from a (correlated) initial few-electron…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 K Balzer , M Bonitz

To explore whether the density-functional theory non-equilibrium Green's function formalism (DFT-NEGF) provides a rigorous framework for quantum transport, we carried out time-dependent density functional theory (TDDFT) calculations of the…

Materials Science · Physics 2011-07-01 ChiYung Yam , Xiao Zheng , GuanHua Chen , Yong Wang , Thomas Frauenheim , Thomas A. Niehaus

We have developed a method based on the embedded Kadanoff-Baym equations to study the time evolution of open and inhomogeneous systems. The equation of motion for the Green's function on the Keldysh contour is solved using different…

Mesoscale and Nanoscale Physics · Physics 2011-11-28 Petri Myöhänen , Adrian Stan , Gianluca Stefanucci , Robert van Leeuwen
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