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We demonstrate optically pumped dynamic nuclear polarization of 29-Si nuclear spins that are strongly coupled to paramagnetic color centers in 4H- and 6H-SiC. The 99 +/- 1% degree of polarization at room temperature corresponds to an…

An experiment demonstrating the quantum simulation of a spin-lattice Hamiltonian is proposed. Dipolar interactions between nuclear spins in a solid state lattice can be modulated by rapid radio-frequency pulses. In this way, the effective…

Quantum Physics · Physics 2007-05-23 Georgios Roumpos , Cyrus P. Master , Yoshihisa Yamamoto

We experimentally demonstrate high degree of polarization of 13C nuclear spins weakly interacting with nitrogen-vacancy (NV) centers in diamond. We combine coherent microwave excitation pulses with optical illumination to provide controlled…

Quantum Physics · Physics 2019-10-25 Jiwon Yun , Kiho Kim , Dohun Kim

The nuclear-to-electron spin angular momentum conversion via hyperfine coupling in a normal metal (NM)/ferromagnet (FM) bilayer system is theoretically investigated by using the nonequilibrium Green's function method. The spin current…

Mesoscale and Nanoscale Physics · Physics 2018-09-10 Y. Ohnuma , S. Maekawa , M. Matsuo

We present a new concept for homonuclear dipolar recoupling in magic-angle-spinning (MAS) solid-state NMR experiments which avoids the problem of dipolar truncation. This is accomplished through the introduction of a new NMR pulse sequence…

Quantum Physics · Physics 2007-08-08 Navin Khaneja , Niels Chr. Nielsen

We analyze electron spin relaxation in electronic transport through coherently coupled double quantum dots in the spin blockade regime. In particular, we focus on hyperfine interaction as the spin relaxation mechanism. We pay special…

Mesoscale and Nanoscale Physics · Physics 2015-03-13 Carlos López-Monís , Jesús Iñarrea , Gloria Platero

Altermagnets (AMs) constitute a novel class of spin-compensated materials in which the symmetry connecting opposite-spin sublattices involves a spatial rotation. Here, we uncover a set of unique non-linear, light-driven properties that set…

Materials Science · Physics 2025-09-16 Amir Eskandari-asl , Jorge I. Facio , Oleg Janson , Adolfo Avella , Jeroen van den Brink

We propose a general protocol for on-demand generation of robust entangled states of nuclear and/or electron spins of ultracold $^1\Sigma$ and $^2\Sigma$ polar molecules using electric dipolar interactions. By encoding a spin-1/2 degree of…

Quantum Physics · Physics 2023-04-10 Timur V. Tscherbul , Jun Ye , Ana Maria Rey

Nuclear spins in certain solids couple weakly to their environment, making them attractive candidates for quantum information processing and inertial sensing. When coupled to the spin of an optically-active electron, nuclear spins can be…

Quantum Physics · Physics 2022-11-11 Alexander A. Wood , Russell M. Goldblatt , Robert E. Scholten , Andy M. Martin

We suggest a new spin orientation mechanism for localized electrons: $dynamic~electron~spin~polarization~provided~by~nuclear~spin~fluctuations$. The angular momentum for the electrons is gained from the nuclear spin system via the hyperfine…

Mesoscale and Nanoscale Physics · Physics 2020-10-14 D. S. Smirnov , T. S. Shamirzaev , D. R. Yakovlev , M. Bayer

Nuclear spins nearby nitrogen-vacancy (NV) centers in diamond are excellent quantum memory for quantum computing and quantum sensing, but are difficult to be initialized due to their weak interactions with the environment. Here we propose…

Quantum Physics · Physics 2019-09-04 Nanyang Xu , Yu Tian , Bing Chen , Jianpei Geng , Xiaoxiong He , Ya Wang , Jiangfeng Du

Nuclear-spin-dependent (NSD) parity violating (PV) effects can be strongly enhanced in diatomic molecules containing heavy atoms. Future measurements are anticipated to provide nuclear anapole moments and strength constants for PV nuclear…

Atomic Physics · Physics 2012-11-20 A. Borschevsky , M. Iliaš , V. A. Dzuba , K. Beloy , V. V. Flambaum , P. A. Schwerdtfeger

Quantum materials display exotic behaviours related to the interplay between temperature-driven phase transitions. Here, we study electron dynamics in one such material, CaFe2As2, a parent Fe-based superconductor, employing time and…

This study explores, both theoretically and experimentally, the photochemically induced dynamic nuclear polarization (photo-CIDNP) of 19F nuclei, the associated spin relaxation, cross-relaxation and cross-correlation effects, as well as…

Chemical Physics · Physics 2011-04-28 Ilya Kuprov

We present the results of experiments on dynamic nuclear polarization and relaxation of 75As in silicon crystals. Experiments are performed in strong magnetic fields of 4.6 T and temperatures below 1 K. At these conditions donor electron…

Materials Science · Physics 2016-11-15 J. Järvinen , J. Ahokas , S. Sheludyakov , O. Vainio , L. Lehtonen , S. Vasiliev , D. Zvezdov , L. Vlasenko

Resonant optical excitation of lowest-energy excitonic transitions in self-assembled quantum dots lead to nuclear spin polarization that is qualitatively different from the well known optical orientation phenomena. By carrying out a…

Mesoscale and Nanoscale Physics · Physics 2014-10-03 A. Högele , M. Kroner , C. Latta , M. Claassen , I. Carusotto , C. Bulutay , A. Imamoglu

Although 19F has high potential to serve as a background-free molecular marker in bioimaging, the molar amount of marker substance is often too small to enable 19F MR imaging or 19F NMR spectroscopy with a sufficiently high signal-to-noise…

Chemical Physics · Physics 2022-05-24 Johannes Bernarding , Christian Bruns , Isabell Prediger , Markus Plaumann

The available theoretical approaches aiming at describing Dynamic Nuclear spin Polarization (DNP) in solutions containing molecules of biomedical interest and paramagnetic centers are not able to model the behaviour observed upon varying…

Statistical Mechanics · Physics 2014-06-06 Sonia Colombo Serra , Marta Filibian , Pietro Carretta , Alberto Rosso , Fabio Tedoldi

Molecular nanostructures may constitute the fabric of future quantum technologies, if their degrees of freedom can be fully harnessed. Ideally one might use nuclear spins as low-decoherence qubits and optical excitations for fast…

Two dimensional heterostructures are likely to provide new avenues for the manipulation of magnetization that is crucial for spintronics or magnetoelectronics. Here, we demonstrate that optical spin pumping can generate a large effective…

Mesoscale and Nanoscale Physics · Physics 2018-12-26 Chongyun Jiang , Abdullah Rasmita , Weigao Xu , Atac Imamoğlu , Qihua Xiong , Wei-bo Gao