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Strong Coulomb interactions can drive electrons to crystallize into a Wigner lattice. Achieving the bosonic analogue - a crystal of excitons - has remained elusive due to their short lifetimes and weaker interactions. Here, we report the…

Two-dimensional Mott insulators host antiferromagnetic (AFM) correlations that are predicted to enhance the attractive interaction between empty (holons) and doubly occupied (doublons) sites, creating a novel pathway for exciton formation.…

Strongly Correlated Electrons · Physics 2025-05-12 Omar Mehio , Yuchen Han , Xinwei Li , Honglie Ning , Zach Porter , Stephen D. Wilson , David Hsieh

Here we report on the low-energy excitations within the paramagnetic spin-orbit insulator Sr$_3$Ir$_2$O$_7$F$_2$ studied via resonant inelastic X-ray scattering, \textit{ab initio} quantum chemical calculations, and model-Hamiltonian…

Strongly Correlated Electrons · Physics 2022-09-26 Zach Porter , Paul M. Sarte , Thorben Petersen , Mary H. Upton , Liviu Hozoi , Stephen D. Wilson

The electronic properties of excitonic insulators have been examined precisely in recent years. Pictures of exciton condensation may be applied to the spin-state transition observed in perovskite cobalt oxides. We examine the crystal-field…

Strongly Correlated Electrons · Physics 2022-10-12 Koya Kitagawa , Hiroaki Matsueda

More than fifty years ago, excitonic insulators, formed by the pairing of electrons and holes due to Coulomb interactions, were first predicted. Since then, excitonic insulators have been observed in various classes of materials, including…

Using the projector-based renormalization method we investigate the formation of the excitonic insulator phase in the two-dimensional (2D) spinless Falicov-Kimball model with dispersive $f$ electrons and address the existence of excitonic…

Strongly Correlated Electrons · Physics 2015-05-27 Van-Nham Phan , Holger Fehske , Klaus W. Becker

Motivated by recent Raman and resonant inelastic X-ray scattering experiments performed for Mott insulators, which suggest formation of excitons in these systems, we present a theory of exciton formation in the upper Hubbard band. The…

Strongly Correlated Electrons · Physics 2009-11-07 P. Wrobel , R. Eder

Excitonic insulator is a coherent electronic phase that results from the formation of a macroscopic population of bound particle-hole pairs - excitons. With only a few candidate materials known, the collective excitonic behavior is…

Strongly Correlated Electrons · Physics 2021-05-27 Pavel A. Volkov , Mai Ye , Himanshu Lohani , Irena Feldman , Amit Kanigel , Girsh Blumberg

We probe the spectrum of elementary excitations in SrIrO$_3$ by using heterostructured [(SrIrO$_3$)$_m$/(SrTiO$_3$)$_l$] samples to approach the bulk limit. Our resonant inelastic x-ray scattering (RIXS) measurements at the Ir $L_3$-edge…

Many-body interactions can produce novel ground states in a condensed-matter system. For example, interacting electrons and holes can spontaneously form excitons, a neutral bound state, provided that the exciton binding energy exceeds the…

We study the conditions to realize an excitonic condensed phase in an electron-hole bilayer system with local Hubbard-like interactions at half-filling, where we can address the interplay with Mott localization. Using Dynamical Mean-Field…

Strongly Correlated Electrons · Physics 2025-12-15 Samuele Giuli , Adriano Amaricci , Massimo Capone

The excitonic insulator is an elusive electronic phase exhibiting a correlated excitonic ground state. Materials with such a phase are expected to have intriguing properties such as excitonic high-temperature superconductivity. However,…

Strongly Correlated Electrons · Physics 2021-12-07 Dominik Christiansen , Malte Selig , Mariana Rossi , Andreas Knorr

Excitonic insulators represent a unique quantum phase of matter, providing a rich ground for studying exotic quantum bosonic states. Strongly coupled electron-hole bilayers, which host stable dipolar exciton fluids with an exciton density…

We studied the possibility of exciton condensation in Mott insulating bilayers. In these strongly correlated systems an exciton is the bound state of a double occupied and empty site. In the strong coupling limit the exciton acts as a…

Strongly Correlated Electrons · Physics 2014-01-01 Louk Rademaker , Jeroen van den Brink , Jan Zaanen , Hans Hilgenkamp

First-principles calculations reveal an unusual electronic state (dubbed as half excitonic insulator) in monolayer 1T-MX2 (M = Co, Ni and X = Cl, Br). Its one spin channel has a many-body ground state due to excitonic instability, while the…

Materials Science · Physics 2019-06-19 Zeyu Jiang , Yuanchang Li , Wenhui Duan , Shengbai Zhang

An excitonic insulator$^{1,2}$ (EI) is a correlated many-body state of electron-hole pairs, potentially leading to high-temperature condensate and superfluidity$^{3-7}$. Despite ever-growing experiments suggesting possible EI states in…

Materials Science · Physics 2025-03-17 Fang Zhang , Jiawei Ruan , Gurjyot Sethi , Chen Hu , Steven G. Louie

The excitonic insulator, a quantum mechanical state arising from exciton condensation, was proposed theoretically many years ago but has yet to be experimentally confirmed. The discovery of correlated transition metal oxides based on $4d$…

Strongly Correlated Electrons · Physics 2024-10-18 Hidemaro Suwa , Shang-Shun Zhang , Cristian D. Batista

We consider the excitonic insulator state (often associated with electronic ferroelectricity), which arises on the phase diagram of an extended spinless Falicov--Kimball model (FKM) at half-filling. Within the Hartree--Fock approach, we…

Strongly Correlated Electrons · Physics 2015-03-20 D. I. Golosov

An excitonic insulator phase is expected to arise from the spontaneous formation of electron-hole pairs (excitons) in semiconductors where the exciton binding energy exceeds the size of the electronic band gap. At low temperature, these…

Strongly Correlated Electrons · Physics 2022-09-02 Selene Mor , Marc Herzog , Claude Monney , Julia Stähler

We re-examine the three-dimensional spinless Falicov-Kimball model with dispersive $f$ electrons at half-filling, addressing the dispute about the formation of an excitonic condensate, which is closely related to the problem of electronic…

Strongly Correlated Electrons · Physics 2015-05-14 B. Zenker , D. Ihle , F. X. Bronold , H. Fehske
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