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Graphite is a ubiquitous electrode material with particular promise for use in e.g., energy storage and desalination devices, but very little is known about the properties of the graphite-electrolyte double layer at technologically relevant…

Materials Science · Physics 2021-09-03 Aaron R. Finney , Ian J. McPherson , Patrick R. Unwin , Matteo Salvalaglio

Ionic Seebeck effect of electrolytes has shown promising applications in harvesting energy from low-grade waste-heat sources with small temperature difference from the environment, which can power sensors and Internet-of-Things devices.…

Soft Condensed Matter · Physics 2022-02-03 Xin Qian , Te-Huan Liu , Ronggui Yang

One prominent structural feature of ionic liquids near surfaces is formation of alternating layers of anions and cations. However, how this layering responds to applied potential is poorly understood. We focus on the structure of…

Ionic liquids are promising candidates for electrolytes in energy-storage systems. We demonstrate that mixing two ionic liquids allows to precisely tune their physical properties, like the dc conductivity. Moreover, these mixtures enable…

Soft Condensed Matter · Physics 2018-02-27 E. Thoms , P. Sippel , D. Reuter , M. Weiß , A. Loidl , S. Krohns

Hypothesis: Ionic liquids have various applications in catalytic reaction environments. In those systems, their interaction with interfaces is key to their performance as a liquid phase. We hypothesize that the way a monolayer ionic liquid…

Soft Condensed Matter · Physics 2024-03-14 Kevin Höllring , Nataša Vučemilović-Alagić , David M. Smith , Ana-Sunčana Smith

Nanopores made with low dimensional semiconducting materials, such as carbon nanotubes and graphene slit pores, are used in supercapacitors. In theories and simulations of their operation, it is often assumed that such pores screen ion-ion…

Materials Science · Physics 2017-01-24 Alpha A. Lee , Dominic Vella , Alain Goriely

We present a comparative computer simulation study of the phase diagrams and anomalous behavior of two-dimensional ($2D$) and quasi-two-dimensional ($q2D$) classical particles interacting with each other through isotropic core-softened…

Soft Condensed Matter · Physics 2019-06-14 Yu. D. Fomin , E. N. Tsiok , V. N. Ryzhov

We study theoretically an influence of the near-interfacial insulator traps and electron-hole puddles on the small-signal capacitance and conductance characteristics of the gated graphene structures. Based on the self-consistent…

Mesoscale and Nanoscale Physics · Physics 2011-06-29 G. I. Zebrev , E. V. Melnik , A. A. Tselykovskiy

We perform a comprehensive analysis of the spectrum of graphene plasmons which arise when a pair of sheets are confined between conducting materials. The associated enhanced local fields may be employed in the manipulation of light on the…

Mesoscale and Nanoscale Physics · Physics 2017-09-05 Godfrey Gumbs , Dipendra Dahal , Antonios Balassis

Graphene, as a passivation layer, can be used to protect the black phosphorus from the chemical reaction with surrounding oxygen and water. However, black phosphorus and graphene heterostructures have low efficiency of heat dissipation due…

Materials Science · Physics 2019-03-28 Yang Chen , Yingyan Zhang , Kun Cai , Jinwu Jiang , Jin-cheng Zheng , Junhua Zhao , Ning Wei

The effect of an axial temperature gradient on the flow profile and the induced streaming potential of a pressure-driven symmetric electrolyte in a slit channel is investigated. Based on the non-isothermal Nernst-Planck equations as well as…

Fluid Dynamics · Physics 2020-06-26 Mathias Dietzel , Steffen Hardt

We show that the huge Seebeck coefficients observed recently for ionic conductors, arise from a ratchet effect where activated jumps between neighbor sites are rectified by a temperature gradient, thus driving mobile ions towards the cold.…

Soft Condensed Matter · Physics 2021-02-17 Alois Würger

Electrical double layers play a key role in a variety of electrochemical systems. The mean free path of secondary electrons in aqueous solutions is on the order of a nanometer, making them suitable for probing of ultrathin electrical double…

We consider the effect of electron-electron interactions on a voltage biased quantum point contact in the tunneling regime used as a detector of a nearby qubit. We model the leads of the quantum point contact as Luttinger liquids,…

Mesoscale and Nanoscale Physics · Physics 2017-05-10 Gleb Skorobagatko , Anton Bruch , Silvia Viola Kusminskiy , Alessandro Romito

It is generally accepted that the hydrophilic property of graphene can be affected by the underlying substrate. However, the role of intrinsic vs. substrate contributions and the related mechanisms are vividly debated. Here we show that the…

New interlayer intermolecular potential model was proposed and it represented ``ABAB'' staking of graphite. Hydrogen atom sputtering on graphite surface was investigated using molecular dynamics simulation. In the initial short time period,…

Materials Science · Physics 2007-11-26 Atsushi Ito , Hiroaki Nakamura

We present computer simulations of a simple bead-spring model for polymer melts with intramolecular barriers. By systematically tuning the strength of the barriers, we investigate their role on the glass transition. Dynamic observables are…

Soft Condensed Matter · Physics 2015-05-14 Marco Bernabei , Angel J. Moreno , Juan Colmenero

Morphology of polymer electrolytes membranes (PEM), e.g., Nafion, inside PEM fuel cell catalyst layers has significant impact on the electrochemical activity and transport phenomena that determine cell performance. In those regions, Nafion…

Materials Science · Physics 2015-01-27 Daiane Damasceno Borges , Gerard Gebel , Alejandro A. Franco , Kourosh Malek , Stefano Mossa

Ionic liquids, salts in the liquid state under ambient conditions, are of great interest as precision lubricants. Ionic liquids form layered structures at surfaces, yet it is not clear how this nano-structure relates to their lubrication…

Materials Science · Physics 2017-09-13 Alexander M. Smith , Kevin R. J. Lovelock , Nitya Nand Gosvami , Tom Welton , Susan Perkin

A generalization of the mean-field approach will be derived that will take into account the ion-ion as well as ion-surface non-electrostatic effects on an equal footing, being based on the bulk and surface equations of state in the absence…

Soft Condensed Matter · Physics 2018-06-20 Rudolf Podgornik
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